Abstract
A quantization scheme is developed for the radiation and higher order electromagnetic fields in one dimensional periodic, dispersive and absorbing dielectric medium. For this structure, the Green function is solved based on the plane wave expansion method, thus the photon operators, commutation relations and quantum Langevin equations are given and studied based on the Green function approach, moreover, the input-output relations are also derived. It is proved that this quantum theory can be reduced back to that of the predecessors’ study on the homogenous dielectric. Based on this method, we find that the transformation of the photon state through the lossy grating is non-unitary and that the notable non-unitary transformation can be obtained by tuning the imaginary part of the permittivity, we also discussed the excellent quantum optical properties for the grating which are similar to the classical optical phenomena. We believe our work is very beneficial for the control and regulation of the quantum light based on gratings.
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Introduction
In recent years, a significant effort has been devoted to the study on the theory and application of metastructure and metasurface, which are artificial periodic structures with their periodicity perpendicular to the incident direction of light1. Based on the dimension of the periodicity, they can be classified as one dimensional (1D) grating2 and two dimensional variation of such structures. A lot of fundamental study on these structures has been conducted, including band structure3,4,5, scattering6,7, absorption8,9, nonlinear optical effects10,11,12, and so on. The extraordinary features, like guided resonance, light bound states in the continuum (BICs)13,14,15, and so on, enable these structure to be applied to many optical processes, for example, hollow-core waveguide16, high-Q resonators17, surface-normal coupler18, vertical-cavity surface-emitting lasers19, high-NA planar lenses20, surface-normal second-harmonic emission21, and so on.
The previous study of metastructure and metasurface focuses on the classical optical properties and presents various and meaningful application in classical optics, but an important question is noticeable, how these structures regulate the quantum electromagnetic (EM) field? To solve this problem we should accomplish the the first two basic tasks which are the EM field quantization in those periodic artificial structures and getting the corresponding input-output relation. There has been extensive research on EM quantization22,23,24,25,26. In ref. 27, a fully canonical quantization scheme which is based on the Hopfield model28 of a dielectric for the macroscopic EM field in a linear harmonic oscillator bulk material is developed, the EM field is coupled to a harmonic-oscillator polarization field that interacts with a continuum of harmonic oscillator reservoir fields. Another method-the Green function approach-is introduced to solve the quantization problem for the dielectric including loss, which can be regarded as a natural extension of the familiar method of the mode expansion to arbitrary Kramers-Kronig consistent media. The quantization of the radiation field is based on the classical Green function representation of the vector potential, identifying the external sources therein with the noise sources that are necessarily associated with the loss in the medium. However, so far there has not been specific EM quantization theory for the medium with periodic structure.
In our work, the plane-wave expansion (PWE) method29,30,31, which is applied previously to deal with the classical optical problems for the periodic structures, and the Green function approach are used to accomplish the EM field quantization for 1D periodic, dispersive, and lossy medium. The EM fields in plane wave expansion is introduced to the quantum Maxwell equation and then the Green function in the corresponding bulk system can be calculated, on the basis of these the photon annihilators will be obtained. Moreover, we can study the input-output relation and get more quantum properties by applying this relation. Here the method we used is developed from the mode expansion of photon operators32,33,34.
Theory and Method
Solution of quantum Maxwell equations for 1D grating
We consider 1D periodic structure (1D photonic crystal) as shown in Fig. 1. In order to quantize the eletromagnetic field in this structure we will resolve the quantum Maxwell equations22,23,24,25 using PWE method. Here the relative permittivity is periodic along the x direction and uniform along the y and z direction, we consider the transverse electric (TE) modes in which the electric field is polarized in the uniform y direction, all possible nonzero EM fields are denoted by \(({\hat{H}}_{x},{\hat{E}}_{y},{\hat{H}}_{z})\). The unit vectors of the primitive lattice and the corresponding reciprocal lattice can be introduced a = aex and \({\boldsymbol{b}}=b{{\boldsymbol{e}}}_{x}=2\pi /a{\overrightarrow{{\boldsymbol{e}}}}_{x}\), respectively. The operator EM fields can be written as the superposition of plane waves based on the PWE method
Noise current density \({\hat{J}}_{y}({\boldsymbol{r}},\omega )\) and corresponding bosonic vector field \({\hat{f}}_{y}({\boldsymbol{r}},\omega )\) can be expressed in a similar way. The periodic relative permittivity can be also expanded as \(\varepsilon (x,y,z,\omega )=\sum _{j}{\varepsilon }_{j}(\omega ){e}^{i{G}_{j}x}\). Here the wave vector is kjx = kx + Gj, Gj = jb. The integer j in all the previous expressions is taken as j = 0, −1, 1, …, −N, N. In principle, the indices j should run from −∞ to +∞, but in numerical practice, truncation over a certain order is necessary. The number of the values of j is \(M=2N+1\), \({\hat{E}}_{jy}(z,\omega )\) and \({\hat{H}}_{j\xi }(z,\omega )\) are expansion coefficients of the electric and magnetic fields, \({\varepsilon }_{j}(x,\omega )\), \({\hat{J}}_{jy}(z,\omega )\) and \({\hat{f}}_{jy}(z,\omega )\) represent expansion coefficients of the relative permittivity, noise current density and corresponding bosonic vector field. It is implicit in equations (1) that the Bloch theorem is satisfied for the one dimensional periodic medium.
The classical EM fields in the one dimensional periodic structures have already been studied in many previous works29,30,31. We borrow the ideas from these works to solve the quantum Maxwell equations, substitute the operator EM fields in quantum Maxwell equations for the plane waves expansion, thereby we find that the electric field \({\hat{E}}_{my}(z,\omega )\) obeys the partial differential equation
In order to solve the electric field in this equation, we rewrite it as the following matrix form
where P(ω) is M × M matrix, \({\hat{E}}_{y}(z,\omega )\) and \({\hat{J}}_{y}(z,\omega )\) are both one column matrixes, \({\hat{E}}_{y}(z,\omega )=({\hat{E}}_{0y}(z,\omega ),{\hat{E}}_{-1y}(z,\omega ),\) \({\hat{E}}_{1y}(z,\omega ),\cdots {\hat{E}}_{Ny}(z,\omega ){)}^{T}\) and \({\hat{E}}_{y}(z,\omega )=({\hat{E}}_{0y}(z,\omega ),{\hat{E}}_{-1y}(z,\omega ),\) \({{\hat{E}}_{1y}(z,\omega ),\cdots {\hat{E}}_{Ny}(z,\omega ))}^{T}\), the superscript T means the transpose of the matrixes. We use the Green function method to solve the electric field \({\hat{E}}_{y}(z,\omega )\) in Eq. (3), the Green function35 G(z, z’, ω) is a M × M matrix, in order to solve it, the Fourier transforms of \({\hat{E}}_{y}(\kappa ,\omega )\) and \({\hat{J}}_{y}(\kappa ,\omega )\) of \({\hat{E}}_{y}(z,\omega )\) and \({\hat{J}}_{y}(z,\omega )\) should be introduced. Then we substitute these Fourier decomposition into Eq. (3) and obtain an equation in Fourier space shown as follows
The corresponding Green function G(κ, κ′, ω) for this equation satisfies
here the Green function G(κ, κ′, ω) is also a M × M matrix which is the Fourier transform of G(z, z′, ω), I is the identity matrix, \({\hat{E}}_{y}(\kappa ,\omega )\) and \({\hat{J}}_{y}(\kappa ,\omega )\) are one column matrixes. The eigenvalues of the matrix P(ω) and the M × M matrix S(ω), whose σ th column (S0σ(ω), S−1σ(ω), S1σ(ω), …, S−Nσ(ω), SNσ(ω))T is the eigenvector corresponding to the eigenvalue −κσ2(ω), can be obtained simultaneously, κσ(ω) is the wavevector along z direction. The matrix S(ω) satisfies
Then the Green function \(G(\kappa ,\kappa ^{\prime} ,\omega )\) in Eq. (5) can be calculated based on Eq. (6)
where δ is a positive infinitesmal, the dependence on ω is implicit for κσ(ω) and S(ω). The Green function G(z, z’, ω) can be calculated by integrating G(κ, κ′, ω) over κ and κ′
the residue theorem is used in the calculation of this integral. Based on this Green function the field \(\hat{E}\)my(z, ω) can be solved
here the amplitude operators \({\hat{o}}_{\sigma y}^{+}(z,\omega )\) and \({\hat{o}}_{\sigma y}^{-}(z,\omega )\) are introduced, which propagate forward (along +z direction) and backward (along −z direction), respectively,
where we assume the wave vector κσ = βσ + iγσ, βσ and γσ are the real and imaginary parts of κσ.
Annihilation and creation operators
Based on the explicit expressions of amplitude operators, we have also studied the spatial evolution of the amplitude operators which is governed by quantum Langevin equations (see Supplementary Material), where the quantum noise associated with the damping is taken into account by operator Langevin noise sources. After consideration of the commutation relations of the operator noise current densities, we can get the commutation relations of the amplitude operators (see Supplementary Material), from the results we can see that the commutation relations of the amplitude operators with different orders may not be zero. A special case is considered z = z’ and then we define a matrix Umn(ω) in this case
The commutation relations of the photon annihilation operators with different orders should be equal to zero, so we introduce the photon annihilation operators \({\hat{a}}_{my}^{+}(z,\omega )\) and \({\hat{a}}_{my}^{-}(z,\omega )\), which are the linear superposition of the amplitude operators \({\hat{o}}_{my}^{+}(z,\omega )\) and \({\hat{o}}_{my}^{-}(z,\omega )\), respectively,
The matrixes of superposition coefficients X+ (ω) and X−(ω) are determined by the commutation relations of the bosonic photon annihilation and creation operators
Substituting in the left of the commutation relations in Eq. (13) for the photon operators the superposition forms (12), the coefficients X+ (ω) and X−(ω) can be determined by U(ω)
It is clearly seen from Eq. (14) that X+ (ω) is equal to X−(ω) (X+ (ω) = X−(ω) = X(ω)).
So far, The EM field quantization in one-dimensional photonic crystal is fully completed, the final form of the electric field can be written as in matrix
Here\({e}^{\pm i\beta z}\) are the diagonal matrixes \(diag({e}^{\pm i{\beta }_{0}z},\,{e}^{\pm i{\beta }_{-1}z},{e}^{\pm i{\beta }_{1}z}\cdots {e}^{\pm i{\beta }_{N}z})\) which describe the propagation of the quantum light, \({\hat{a}}_{y}^{\pm }(z,\omega )\) are one column matrixes \({({\hat{a}}_{0y}(z,\omega ),{\hat{a}}_{-1y}(z,\omega ),{\hat{a}}_{1y}(z,\omega ),\cdots {\hat{a}}_{Ny}(z,\omega ))}^{T}\). Here \({\hat{a}}_{0y}(z,\omega )\) is the radiation order and the others are high orders. The matrix S connects the amplitude operators in different orders with the electric field operators in different orders, it is not unity matrix in the grating, which reveal that there is interaction between different orders in this case. When the model degenerates to the homogeneous case, the matrix S is unity and X is diagonal, then our theory can degenerate successfully to the the corresponding results of the previous work36,37,38 of other authors who considered the EM quantization in the radiation order in the normal propagation case (see Supplementary Material).
Quantum optical input-output relation for grating
Now we turn to the problem of propagation of the quantized field39 through 1D periodic dielectric slab—1D grating—embedded in two semi-infinite homogeneous dielectrics, which is shown in Fig. 2. The dielectric function is expressed as
the superscripts 1, 2, 3 represent three corresponding regions.
The input-output relation of annihilation operators in transfer matrix form for the grating can be obtained by using EM boundary condition and solution of quantum Langevin equation (see Supplementary Material)
here the columns \({\hat{g}}^{+}(\omega )\) and \({\hat{g}}^{-}(\omega )\) are associated with the grating.
The commutation relations of \({\hat{G}}^{\pm }(\omega )\) with different orders may not be zero, in light of mentioned theoretical discussion we construct the new operators \({\hat{g}}_{n}^{+}(\omega )\) and \({\hat{g}}_{n}^{-}(\omega )\) associated with the slab which satisfy the bosonic commutation relations. Firstly, we define \({\hat{G}}_{n}^{0+}(\omega )\) and \({\hat{G}}_{n}^{0-}(\omega )\) to ensure that they commute with each other
After some calculation, the related commutation relations are listed in the following, moreover, the matrix V is introduced further
Secondly, we construct new operators \({\hat{g}}_{m}^{+}(\omega )\) and \({\hat{g}}_{n}^{-}(\omega )\) as linear superposition of operators \({\hat{G}}_{n}^{0+}(\omega )\) and \({\hat{G}}_{n}^{0-}(\omega )\) in the similar way to construct the photon operators
The new operators should fulfill the bosonic commutation relations
Similarly, the coefficients of Y+ (ω) and Y− (ω) can be determined from the above equations by substituting the Eqs. (20) into (21)
Finally, the quantum optical input-output relation expressed in the transfer matrix form can be transformed to the scattering matrix Qmn(mn = 11, 12, 21, 22)
So far we construct the relation between the output annihilation operators \({\hat{a}}^{3+}(l/2,\omega )\), \({\hat{a}}^{1-}(-l/2,\omega )\) and the input annihilation operators \({\hat{a}}^{1+}(-l/2,\omega )\), \({\hat{a}}^{3-}(l/2,\omega )\) and the bosonic excitations associated with the slab \({\hat{g}}^{+}(\omega )\), \({\hat{g}}^{-}(\omega )\). The new operators \({\hat{g}}^{+}(\omega )\) and \({\hat{g}}^{-}(\omega )\) play the role of the noise sorces associated with the damping in the input-output relation. When we consider the special case of homogeneous dielectric, the input-output relation and related commutation relations can be also derived back to the previous study37,38.
Then we can derive the commutation relations between the output photon operators based on the input-output relation together with the known commutation relations between the input photon operators. After deliberate and straightforward calculation the results can be written in matrix form
Here the matrixes shown in the above equation are defined as \({c}_{11,mn}=[{\hat{a}}_{m}^{3+}(l/2,\omega ),{\hat{a}}_{n}^{3+\dagger }(l/2,\omega )],{c}_{12,mn}=\) \([{\hat{a}}_{m}^{3+}(l/2,\omega ),{\hat{a}}_{n}^{1-\dagger }(-l/2,\omega )]\), \({c}_{21,mn}=[{\hat{a}}_{m}^{1-}(-l/2,\omega ),{\hat{a}}_{n}^{3+\dagger }(l/2,\omega )]\) and \({c}_{22,mn}=[{\hat{a}}_{m}^{1-}(-l/2,\omega ),\) \({\hat{a}}_{n}^{1-\dagger }(-l/2,\omega )]\). In the following we give the results about the values of commutation relations for the uniform slab and grating immersed in air. The grating refers to alternating dielectric bar and air, the period and bar width of the grating are denoted by Λ and w, the relative permittivity of the dielectric bar is marked by ε, the thicknesses of the uniform slab and grating are both denoted by l, the wavelength and incident angle of the EM field are represented by λ and θ. Because of the symmetry of this model, c11,mn = c22,mn, c12,mn = c21,mn.
The diagonal elements of matrixes c11, c12, c21 and c22 are real number which can be seen from Eq. (24). For the uniform dielectric the matrix X is diagonal, if the uniform dielectric is lossless, the coefficients Xmn approach zero for higher orders (m ≠ 0), so only the radiated (m = 0) annihilation and creation operators are physically significant. Hence, we are interested in c11,00, c12,00, c21,00 and c22,00 in radiation order for our model.
In Fig. 3 we consider the transmission and values of commutation relations, c11,00 and c22,00, for the lossless uniform slab and lossless grating as a function of the reduced wavelength λ/Λ. The corresponding case of lossy layer is shown in Fig. 4. For uniform slab, no matter it is lossless or lossy, c11,00 = 1 and c12,00 = 0 hold, which can be seen from Figs. 3(b), 4(b,c), that means the output photons satisfy bosonic commutation relation and the annihilation operators for different channels commute with each other, these results coincide with the former work. For grating, only when it is lossless, c11,00 = 1 and c12,00 = 0, which can be seen from Fig. 3(d), when it is lossy, these equations are not true in this case, that is to say, c11,00 ≠ 1 and c12,00 ≠ 0, which can be seen from 4(e,f). After comparing the four different models, we find that the physical origin of this inequality is that the excitations, \({\hat{g}}_{m}^{+}(\omega )\) and \({\hat{g}}_{m}^{-}(\omega )\), in different orders interact with each other. Not only that, from Fig. 4(d–f) we also find that near the guided resonance, which is the Fano resonance in our optical model, obvious resonance and deviation of c11,00 and c12,00, the deviation means that the departure of c11,00 value from 1 and c12,00 value from 0. It can be also clearly seen that at the reduced wavelength λ/a > 1.5, there is no guided resonance, while there is also no resonance for c11,00 and c12,00 and the deviation decreases.
The Heisenberg picture is implied in the quantization theory, when the theory is converted to Schördinger picture, we can understand the phenomenon further, which is the deviation of the bosonic commutation relations for the output photon operators in the lossy grating. In the Schördinger picture, the evolution operator is no longer unitary with respect to the radiated order which can be derived from the input-output relation40,41, so the transformation of the quantum states is non-unitary. From Fig. 4(e,f) we can see that the phenomenon of deviation is very small (~10−3).
Now we tune c11,00 and c12,00, which describe the transformation of the photon states, by change the parameters in our model. Compared to the classical optics the Fano resonance can appear in the grating for quantum light which can be seen from Fig. 5(a,d), near the resonant absorption is notable. The peak and valley of c11,00 and c12,00 are coincident with the resonant absorption, the sign of c12,00 is opposite to that near the adjacent resonant curve. We can see that the deviations of c11,00 from 1 and c12,00 from 0 are closely related to the Fano resonance in the grating. It is clearly seen in Fig. 5 that these deviations are very weak (~10−3) due to the weak absorption (the imaginary part of the relative permittivity is only \({\varepsilon }_{I}=0.1\)). In Fig. 6 it is implied that the deviation of c11,00 from 1 rises by increasing the imaginary part of the relative permittivity which is closely related to the effect of absorption, this devation can reach about 0.4. When εI is located at (0.3, 1.5) the deviation of c12,00 from 0 can be increased about 1 order of magnitude (~10−2). εI variation leads to notable effect of \({\hat{g}}_{m}^{+}(\omega )\) and \({\hat{g}}_{m}^{-}(\omega )\) in higher orders on the output photon operators in radiation order, so we can enhance the effect of the nonunitary evolution obviously by changing the imaginary part of the relative permittivity of the grating.
We have also calculated the transmission, reflection and absorption for photon number density, which are equal to that in classical optics. The sharp resonance, guided resonance, which appears in the grating for classical light can also emerge for quantum light. At the resonance, 100% relative numbers of the outgoing photons in output channels are exhibited and near 100% absorption is realized for the lossy grating, the Q factor is high and the lifetime is long. From the asymptotic behavior of the resonance, some embedded resonances with zero linewidth can be found, these embedded resonances possess infinite high Q factor and infinite long lifetime, and are called light bound states in the continuum (BICs) which have attracted much attention in recent years in classical optics13,14,15. In our work, we also find the light BICs in quantum optics in theory. In classical optics, many applications of the grating are developed because of their excellent optical properties42,43, we believe that the grating can be applied in various areas of quantum optics, such as propagation of non-classical light, quantum state transformation, spontaneous emission of a nearby scatter and so on, these will be our next tasks.
Conclusion
We give the Green function and the EM field quantization for 1D periodic, dispersive and absorbing dielectric bulk medium firstly. The EM field are expanded in plane waves and are inserted to the quantum Maxwell equations, the Green function is solved, furthermore the electric field is quantized and the amplitude annihilators are established. The commutation relations of these amplitude operators in our periodic bulk system are calculated out based on the previous known commutation relations of the operator noise current density, we find that the amplitude operator don’t commute with the its Hermite operator with different order, which is quite different from the homogeneous dielectric case. Then we construct the photon annihilation operators by linear superposition of the amplitude operators. The quantum Langevin equations which determine the spatial evolution of the amplitude operators in our bulk system are provided and studied.
The quantum input-output relation for the grating is also derived, the output field operators can be described in terms of input field operators and noise sources associated with the loss in the gratings. We find that the conventional commutation relations are satisfied, \({c}_{11,00}=[{\hat{a}}_{0}^{3+}(l/2,\omega ),{\hat{a}}_{0}^{3+\dagger }(l/2,\omega )]=1\) and \({c}_{12,00}=[{\hat{a}}_{0}^{3+}(l/2,\omega ),\), \({\hat{a}}_{0}^{1-\dagger }(-l/2,\omega )]=0\)for uniform slab or lossless grating, but for lossy grating, these relations do not hold, these phenomena originate from the interaction between the output photon in radiation order and the excitations in higher orders. The excellent quantum optical properties of the grating are also found and discussed. We believe our work is very beneficial for the control and regulation of the quantum light based on gratings.
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Acknowledgements
This work was supported by the Science and Technology Innovation Planning Project in Universities and Colleges of Shanxi Province of China under Grant No. 2019L0019.
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Wang, T. Electromagnetic field quantization and quantum optical input-output relation for grating. Sci Rep 9, 19992 (2019). https://doi.org/10.1038/s41598-019-56197-1
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DOI: https://doi.org/10.1038/s41598-019-56197-1
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