Abstract
A harmonically driven cavity QED system consisting of two cavities and a two-level qubit is shown to enable the generation of a vast class of maximally entangled states suitable for measurements with a Heisenberg-limit precision. As one of its modalities, this system can serve as a quantum beam splitter, converting an |N〉 ⊗ |0〉 input into a maximally entangled N00N state (|N〉 ⊗ |0〉 + |0〉 ⊗ |N〉)/\(\sqrt{{\bf{2}}}\) at its output. A network of such quantum beam splitters is shown to provide a source of multimode N00N-type entanglement.
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Introduction
Quantum physics leads us to rethink and redefine the limits of precision in a physical measurement. When applied to an estimation of a parameter \(\phi \) by sampling a system N times, suitably tailored quantum states can overcome the classical shot-noise limit (SNL) of parameter-estimation error, \(\Delta \phi \propto 1/\sqrt{N}\), taking it to a new level of precision, limited only by the Heisenberg limit, \(\Delta \phi \propto 1/N\)1,2.
Maximally entangled quantum states \((|N\rangle \otimes |0\rangle +|0\rangle \otimes |N\rangle )/\sqrt{2}\), referred to as N00N states3,4,5, stand out as a conceptually and methodologically important example of quantum entanglement that enables measurements with a Heisenberg-limit (HL) precision1,5. Generation of such states in a realistic experimental setting is, however, anything but trivial. As a result, the values of N attainable with the existing experimental methods of N00N-state generation6 are rather low compared to the N values that have been achieved for other prominent classes of quantum states broadly used in photonic quantum technologies. Indeed, while coherent states with N \(\simeq \) 100, N = 15 Fock states, and N = 10 Greenberger–Horne–Zeilinger (GHZ) states are all experimentally attainable7,8,9, N00N states with N > 5 photons are still beyond the capabilities of currently existing technologies.
As a promising direction toward practical sources of N00N-type states for HL measurements, a quantum interferometer with a nonlinear phase shift in one of its arms has been shown10,11 to provide a quantum beam-splitter-type scheme whereby an \(|N\rangle \otimes |0\rangle \) state at the input can be converted into a N00N-state output. Implementation of this elegant concept in an all-optical format calls for systems with enhanced optical nonlinearities. Recent experiments suggest that a breakthrough to this much-needed nonlinearity enhancement may be achieved in systems with electromagnetically induced transparency (EIT)12,13,14 or resonance-enhanced Kerr effect15,16 inside an atom trap14, an optical cavity17, or a hollow waveguide13,15,16.
Here, in search for the ways to enhance the performance of a quantum beam splitter as source of quantum entanglement, we examine a generic harmonically driven cavity QED system consisting of two cavities and a two-level qubit. We show that such a system offers an interesting extension of the quantum beam-splitter concept that does not require an all-optical nonlinearity for multipartite entanglement generation. Instead, it is a periodic modulation of the parameters of the two-cavity–qubit system, that enables a control over the phase of quantum interference, needed to steer its output toward a N00N-type state. Effective-Hamiltonian analysis of such a system reveals physically insightful parallels with the Hamiltonians of both an ordinary beam splitter and a Kerr-nonlinearity-enabled quantum beam splitter. A network of such harmonically driven two-cavity–qubit quantum beam splitters is shown to provide a source of multimode N00N-type entanglement.
The Magic of a Quantum Beam Splitter
We start by briefly examining a generic ordinary beam splitter as an important point of reference. When fed with a single-photon state \(|1\rangle \) and a vacuum state \(|0\rangle \) through its two input ports, a standard beam splitter will deliver \((|1\rangle \otimes |0\rangle +|0\rangle \otimes |1\rangle )/\sqrt{2}\), that is, a N00N state with N = 1, at its output. However, when a single-photon state \(|1\rangle \) at the input of a beam splitter is replaced with a larger N-photon state \(|N\rangle \), the state produced as an output of the beam splitter cannot be reduced to a N00N state.
With an ordinary beam splitter being unable to deliver a pure N00N-state output, we come to realize that it takes a kind of a “magic” beam splitter18 to generate N00N states with N > 1, from the input \(|N\rangle \otimes |0\rangle \) state. The Kerr-type optical nonlinearity has been shown10,11 to lend such a magic touch, providing a physical mechanism whereby a suitable nonlinear phase shift can be induced in one of the arms of a quantum interferometer, referred to as a quantum beam splitter (QBS), enabling N00N-state generation at its output.
In this work, in search for the ways to enhance the field–matter coupling – the key factor in control of the QBS performance – beyond the limitations of the purely optical Kerr effect, we explore the cavity-QED extension of the QBS concept. This approach, as will be shown below in this paper, opens the routes toward enhanced QBS performance due to a much stronger field–matter coupling attainable in the cavity QED setting. As a specific example of a cavity QED system, we consider a two-level qubit coupled to two cavities. The effective Hamiltonian of such a system, as we show in this work, can be written as
where \(\kappa \) is the cavity–qubit coupling coefficient, \({a}_{i}^{\dagger }\) and ai are the photon creation and annihilation operators for the ith cavity field, and \({\sigma }_{z}=|e\rangle \langle e|-|g\rangle \langle g|\), \(|e\rangle \) and \(|g\rangle \) being the two states of the two-level qubit.
The Hamiltonian of Eq. (1) is in many ways instructive as it bears a pleasing resemblance of both – the Hamiltonian of an ordinary beam splitter and the Hamiltonian of a quantum beam splitter based on the Kerr effect. We articulate that the scope of Eq. (1) goes way beyond a specific cavity-QED QBS implementation, as this equation, in fact, sets up the effective Hamiltonian for a generic QBS source of N00N states, converting an \(|N\rangle |0\rangle \) input into a N00N-state output. We therefore intend to focus first on the properties of the Hamiltonian (1) as a generic source of N00N states, providing its consistent derivation later, where Eq. (1) will be shown to define the effective Hamitonian for a specific, two-cavity–qubit cavity-QED system.
When used jointly with the Heisenberg evolution equation, the Hamiltonian (1) leads to the following evolution equations for the fields:
The solution to Eq. (2) is
With \(\kappa t=\pi /4\), Eq. (3) give
These fields are then transmitted through a 50:50 beam splitter (see Fig. 1), providing a two-mode unitary transformation \(U=\exp [\,-\,\pi /4({a}_{1}^{\dagger }{a}_{2}-{a}_{2}^{\dagger }{a}_{1})]\) and yielding
An overall transformation of the input fields provided by the two-cavity–qubit system and the 50:50 beam splitter is
These transformations are central to understanding the entanglement-generation capability of our qubit–two-cavity system. Equations (4) and (5) dictate the following transformation of a \(|\psi \rangle =|N\rangle |0\rangle (|g\rangle +|e\rangle )/\sqrt{2}\) input: \(|\psi \rangle \to \frac{1}{\sqrt{2}}(|N\rangle |0\rangle |e\rangle +|0\rangle |N\rangle |g\rangle )/\sqrt{2}\).
With an Hadamard gate applied to the qubit (Fig. 1), e.g., by an external π/2 pulse, the output state becomes \([(|N\rangle |0\rangle +|0\rangle |N\rangle )|e\rangle +(|N\rangle |0\rangle -|0\rangle |N\rangle )|g\rangle ]/2\). A measurement of the qubit state will then yield a N00N state. Specifically, the detection of the qubit in its ground and excited states \(|g\rangle \) and \(|e\rangle \) gives the N00N states \((|N\rangle |0\rangle -|0\rangle |N\rangle )/\sqrt{2}\) and \((|N\rangle |0\rangle +|0\rangle |N\rangle )/\sqrt{2}\), respectively. Either of these output N00N states will enable parameter estimation with the HL precision.
In an earlier study, Yang et al.19 have proposed an elegant circuit QED source of enhanced quantum entanglement based on a four-level qubit coupled to two cavities. The cavity QED scheme considered in this work, on the other hand, employs a two-level qubit, which helps avoid difficulties related to the second-order detuning term in the effective Hamiltonian, which tends to weaken qubit–cavity coupling, making the entangled-state output prone to decoherence.
Enhanced Entanglement Beyond N00N States
In this section, we will demonstrate that the ability of the considered two-cavity–qubit system to generate enhanced quantum entanglement is not limited to a N00N-state output, but extends to a much broader class of quantum states. To this end, we take the input of the first cavity in the form of a coherent state20, \(|\alpha \rangle ={e}^{-\frac{|\alpha {|}^{2}}{2}}\,{\sum }_{n=0}^{\infty }\,\frac{{\alpha }^{n}}{\sqrt{n!}}|n\rangle \), α being an arbitrary complex number. Then, with \(|0\rangle \) at the second input port, the initial state of the system is \(|\psi \rangle =|\alpha \rangle |0\rangle \,(|g\rangle +|e\rangle )/\sqrt{2}\). Quantum evolution of this state dictated by Eqs (4) and (5) yields \((|\alpha \rangle |0\rangle |e\rangle +|0\rangle |\alpha \rangle |g\rangle )/\sqrt{2}\). Applying an Hadamard gate to this state and performing a measurement on the qubit, we arrive at
where, the minus or plus sign is taken depending on whether the qubit is detected in its ground or excited state. The state \(|{\phi }^{+}\rangle \) is known to have important applications in quantum metrology21. With a squeezed state at its input, our system can yield a squeezed-state–vacuum entanglement.
For a general-form initial state \(|\psi \rangle =|{\psi }_{1}\rangle |{\psi }_{2}\rangle \,(|g\rangle +|e\rangle )/\sqrt{2}\), with \(|{\psi }_{1}\rangle ={\sum }_{n=0}^{{d}_{1}}\,{b}_{n}|n\rangle \) and \(|{\psi }_{2}\rangle ={\sum }_{n=0}^{{d}_{2}}\,{c}_{n}|n\rangle \), our two-cavity–qubit system will create an antisymmetric or symmetric entangled-state output,
depending on whether the atom is detected in its ground or excited state.
With a properly tailored input, our cavity-QED QBS can also help generate superpositions composed of two coherent states (\(|\alpha \rangle \) and \(|\beta \rangle \)), \((|\alpha \rangle |\beta \rangle \pm |\beta \rangle |\alpha \rangle )/\sqrt{2\pm 2|\langle \alpha |\beta \rangle {|}^{2}}\), two squeezed states (\(|{\xi }_{1}\rangle \) and \(|{\xi }_{2}\rangle \)), \((|{\xi }_{1}\rangle |{\xi }_{2}\rangle \pm \)\(|{\xi }_{2}\rangle |{\xi }_{1}\rangle )/\sqrt{2\pm 2|\langle {\xi }_{1}|{\xi }_{2}\rangle {|}^{2}}\), or hybrid-entanglement combinations of Fock, coherent, and squeezed states, \((|\alpha \rangle |{\xi }_{1}\rangle \pm \)\(|{\xi }_{1}\rangle |\alpha \rangle )/\sqrt{2\pm 2|\langle {\xi }_{1}|\alpha \rangle {|}^{2}}\), \((|\alpha \rangle |N\rangle \pm |N\rangle |\alpha \rangle )/\sqrt{2\pm 2|\langle N|\alpha \rangle {|}^{2}}\), or \((|{\xi }_{1}\rangle |N\rangle \pm |N\rangle |{\xi }_{1}\rangle )/\)\(\sqrt{2\pm 2|\langle N|{\xi }_{1}\rangle {|}^{2}}\). Such states can help overcome the SNL in quantum metrology and promise interesting options for quantum information processing.
The entanglement of \(|{\psi }^{\pm }\rangle \) can be quantified in terms of the concurrence22, defined as
where σy is the spin flip operator and \(|{\psi }^{\ast }\rangle \) is the complex conjugate of \(|\psi \rangle \). When applied to \(|{\psi }^{\pm }\rangle \), Eq. (9) gives
with the plus and minus signs taken for \(|{\psi }^{+}\rangle \) and \(|{\psi }^{-}\rangle \), respectively. Notably, while the maximum entanglement of \(|{\psi }^{-}\rangle \) is achieved with any input state, \(|{\psi }^{+}\rangle \) is maximally entangled if and only if the input states are orthogonal states, with \(\langle {\psi }_{1}|{\psi }_{2}\rangle =0\). The maximum entanglement of the \(|{\psi }^{-}\rangle \) output makes our two-cavity–qubit QBS a powerful resource not only for quantum sensing and parameter estimation, but also for quantum computing and information processing.
As an important example, with an \(|N\rangle |M\rangle \) state at its input, our QBS will produce a maximally entangled state \((|N\rangle |M\rangle \pm |M\rangle |N\rangle )/\sqrt{2}\), as its output. With \(M=0\), this output reduces to a N00N state.
The Effective Hamiltonian
In this section, we will consider specific examples of cavity-QED systems that can be described in terms of the effective Hamiltonian (1). Our analysis will be focused on a system consisting of two cavities with frequencies \({\omega }_{1}\) and \({\omega }_{2}\) and a two-level qubit whose levels are separated by an energy \(\hslash {\omega }_{0}\). The qubit is coupled to the first and second cavities with coupling strengths g1 and g2. We will show below in this section that, when the cavity frequencies or the qubit–cavity coupling strengths in such a system are modulated periodically in time23,24, the quantum evolution of the system can be described in terms of the effective Hamiltonian (1), enabling the generation of a vast class of maximally entangled states suitable for measurements with an HL precision.
Two-cavity–qubit system with a modulated coupling strength
We first consider a system of two cavities and a two-level qubit in which the coupling strengths g1 and g2 are harmonic functions of time, \({g}_{j}={g}_{0}\,\cos ({\upsilon }_{d}t+{\phi }_{j})\), \(j=1,2\). Such harmonically modulated coupling terms are found in Hamiltonians describing superconducting-circuit magnetic field synthesizers23,25,26 and photonic resonator lattices exhibiting effective magnetic fields for photons23,25,26. We represent the full Hamiltonian of such a system as a sum \(H={H}_{0}+{H}_{I}\) with
and
We set, with an appropriate choice of the system of units, \(\hslash =1\) and assume the free Hamiltonian defined as \({V}_{0}=\frac{\omega }{2}{\sigma }_{z}+\omega {a}_{1}^{\dagger }{a}_{1}+\omega {a}_{2}^{\dagger }{a}_{2}\). In the frame rotating with V0, the Hamiltoninan can be given as
where \({U}_{0}(t)=\exp [\,-\,i{V}_{0}t]\) is the unitary evolution operator. Noting that \([{H}_{0},{V}_{0}]=0\), the resultant Hamiltonian reduces to
where \({\delta }_{0}={\omega }_{0}-\omega \), \({\delta }_{1}={\omega }_{1}-\omega \) and \({\delta }_{2}={\omega }_{2}-\omega \).
Equation (14) can be rewritten as
Defining an operator \({h}_{j}={g}_{0}({\sigma }^{+}{a}_{j}+{a}_{j}^{\dagger }{\sigma }^{-}){e}^{i{\phi }_{j}}\), we reduce HI to a Floquet Hamiltonian24,27,28,29, \({H}_{I}={\delta }_{0}{\sigma }_{z}/2+{\delta }_{1}{a}_{1}^{\dagger }{a}_{1}+{\delta }_{2}{a}_{2}^{\dagger }{a}_{2}++\,{\sum }_{j=1}^{2}\,{h}_{j}^{\dagger }{e}^{i{\upsilon }_{d}t}+{h}_{j}{e}^{-i{\upsilon }_{d}t}\). Considering the condition \({\upsilon }_{d}\gg \sqrt{N}{g}_{0}\) with N being the number of the input photons, we can find the effective Floquet Hamiltonian by adiabatically eliminating the fast oscillating terms24. Thus, using the commutation relations \([{h}_{j},{h}_{j}^{\dagger }]=0\) we find for the effective Hamiltonian24,27,28,29
As can be seen from Eq. (15), the coupling term of the effective Hamiltonian is controlled by the phase difference \({\phi }_{1}-{\phi }_{2}\). To maximize this term, we choose \({\phi }_{1}-{\phi }_{2}=\pi /2\). Equation (15) then becomes
where \(\kappa =\frac{2{g}_{0}^{2}}{{\upsilon }_{d}}\).
Note that σz commutes with the rest of the Hamiltonian, thus, on a resonance condition on the cavities, Eq. (16) reduces to the sought-for effective Hamiltonian of Eq. (1).
Two-cavity–qubit system with modulated cavity frequencies
We now assume that the coupling strength in our two-cavity–qubit QBS is constant, but the cavity frequencies are harmonic functions of time, \({\omega }_{j}(t)=\nu +\Delta \,\sin ({\nu }_{d}t-{\phi }_{j})\), j = 1, 2. The Hamiltonian of the system is then written as
On a resonance, \({\omega }_{0}=\nu \), we find for HI in the rotating-wave approximation
where \(\zeta =\Delta /{\nu }_{d}\).
We can now use the identity \({e}^{i\zeta \cos ({\nu }_{d}t+{\phi }_{j})}=\mathop{\sum }\limits_{n=-\infty }^{\infty }\,{J}_{n}(\zeta ){e}^{in({\nu }_{d}t+{\phi }_{j})}\), \({J}_{n}(\zeta )\) being the nth-order Bessel function of the first kind, to reduce HI to a Floquet Hamiltonian, \({H}_{I}={H}_{0}+{\sum }_{n=1}^{\infty }\,{H}_{n}{e}^{in{\nu }_{d}t}\), with
and
The interaction Hamiltonian of this form leads to an effective Hamiltonian28,29
Combining Eqs (18)–(20), we derive24,27,28,29
where \(\Omega ={g}^{2}\chi /{\nu }_{d}\) and \(\chi ={\sum }_{n=1}^{\infty }\,2{J}_{n}{(\zeta )}^{2}\,\sin (n({\phi }_{1}-{\phi }_{2}))/n\).
Choosing \(\zeta \) such that \({J}_{0}(\zeta )\approx 0\) (\(\zeta \approx 2.405\)), we find
The effective coupling coefficient \(\Omega \) can be maximized with an appropriate choice of \({\phi }_{1}-{\phi }_{2}\). Specifically, \({\phi }_{1}-{\phi }_{2}\approx \pi /3\) leads to \(\chi \approx 0.628\). Qubit–resonator coupling as strong as \(\simeq \)100 MHz can be achieved for a flux qubit coupled to a pair of superconductor cavities30,31, providing \(\kappa \simeq \Omega \simeq 10-100\,{\rm{MHz}}\). Specifically, with \({\upsilon }_{d}=8{g}_{0}\) and \({g}_{0}\simeq 50\,{\rm{MHz}}\) in Eq. (16), we arrive at \(\kappa \simeq 12.5\,{\rm{MHz}}\), which is well above the decoherence rates of the cavities and the qubit, typically estimated as \(\simeq \)1 MHz32.
Multimode Entanglement
We are going to show now that, when connected into a network, cavity-QED QBS systems examined in the previous sections can help confront a challenge of multimode N00N-type entanglement generation. To this end, we consider an array of two-cavity units (Fig. 2) with a qubit set to consecutively interact with each pair of cavities within a time interval \(t=\pi /(4{\kappa }_{0})\), where \({\kappa }_{0}=\kappa \) for a two-cavity–qubit system with a modulated coupling strength and \({\kappa }_{0}=\Omega \) for a two-cavity–qubit system with modulated cavity frequencies. Output cavity photons are sent to 50:50 beam splitters (Fig. 2).
When applied to an initial state \(|\psi \rangle =|N,0\rangle \otimes |N,0\rangle \otimes \ldots \otimes |N,0\rangle \,(|g\rangle +|e\rangle )/\sqrt{2}\), this cavity QED array will yield \((|N,0\rangle \mathrm{...}|N,0\rangle |e\rangle +|0,N\rangle \ldots |0,N\rangle |g\rangle )/\sqrt{2}\) as its output. To illustrate, let us consider the input state with two cavity pairs as \(|\psi \rangle =|N,0\rangle \otimes |N,0\rangle \otimes (|g\rangle +|e\rangle )/\sqrt{2}\). First, the qubit interacts with the first cavity pair resulting in \((|N,0\rangle |e\rangle +|0,N\rangle |g\rangle )/\sqrt{2}\otimes |N,0\rangle \). Then, the qubit interacts with the second cavity pair which prepares \((|N,0\rangle |N,0\rangle |e\rangle +|0,N\rangle |0,N\rangle |g\rangle )/\sqrt{2}\) as its output. With a π/2 pulse applied to the qubit and following a measurement, this output becomes a double-N00N state \((|N,0\rangle |N,0\rangle \pm |0,N\rangle |0,N\rangle )/\sqrt{2}\). Therefore, with the cavity QED array above, we can generate a multi-N00N state \((|N,0\rangle \ldots |N,0\rangle \pm |0,N\rangle \ldots |0,N\rangle )/\sqrt{2}\).
An array of M cavity pairs arranged in this scheme will then provide a phase resolution \(\Delta \phi \propto 1/(MN)\). Achieving this level of Δ\(\phi \) with ordinary N00N states would have required MN photons in each of the entangled modes. For large M and N, this requirement is difficult to fulfill in practice. To appreciate this, let us take \(m=2\), for simplicity. In this case, the generated state reduces to the double N00N state \((|N,0\rangle |N,0\rangle \pm |0,N\rangle |0,N\rangle )/\sqrt{2}\) introduced in33. Applying the phase shift \(\phi \) on the second and the fourth modes of the state, the phase shift of 2N\(\phi \) is accumulated which results in \(\Delta \phi \propto 1/(2N)\). This is equivalent to the phase estimation with a N00N state of the form \((|2N,0\rangle +|0,2N\rangle )/\sqrt{2}\)33. Considering the fact that number states of more than N = 15 are feasible with the current technology7,9, preparing two pairs of N = 15 photons in cavity pairs can result in estimation with a phase resolution \(\Delta \phi \propto 1/30\). Achieving such a big phase estimation number with an ordinary N00N state is far beyond the latest achievements with the current technology which is limited to a few photons. It is notable that our approach of double N00N state generation is different from the one introduced in33 in principle. In the setup proposed in33, N + 2 operational steps is required for generating a double N00N state; however, in our system, we can produce a double N00N state in just a few operational steps, which is independent of the number of the photons, once the initial state is given. Furthermore, our structure is even capable of generating multi-N00N states that can facilitate quantum phase estimation techniques. That being said, we can generate a vast class of multi-mode entangled state by preparing each resonator in our specific state of interest. It is notable that in most of the recently introduced schemes, generating a N00N state requires a linear number of operations with N, which is usually greater than N34,35. The large operational steps required makes it challenging to generate such states experimentally, as decoherence is introduced to the system in each step of the operation. Thus, generation of multimode N00N state can be useful for overcoming this challenge.
Conclusion
To summarize, we have shown that a harmonically driven cavity QED system consisting of two cavities and a two-level qubit enables the generation of a vast class of maximally entangled states suitable for measurements with an HL precision. As one of its modalities, this system can serve as a quantum beam splitter, converting an \(|N\rangle \otimes |0\rangle \) input into a maximally entangled N00N state \((|N\rangle \otimes |0\rangle +|0\rangle \otimes |N\rangle )/\sqrt{2}\) at its output. A network of such quantum beam splitters is shown to provide a source of multimode N00N-type entanglement.
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Acknowledgements
This research was supported in part by the Russian Foundation for Basic Research (projects nos. 18-29-20031, 19-02-00473, 18-52-00025), Welch Foundation (grant no. A-1801-20180324), and the Ministry of Education and Science of the Russian Federation (project 14.Z50.31.0040, February 17, 2017). Research into the quantum optics of microstructure fibers was supported by the Russian Science Foundation (project no. 17-12-01533).
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Y.M. conceived the project, performed the analysis, carried out the calculations, analyzed the results, and wrote the paper. A.M.Z. analyzed the results, and wrote the paper.
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Maleki, Y., Zheltikov, A.M. A high-N00N output of harmonically driven cavity QED. Sci Rep 9, 16780 (2019). https://doi.org/10.1038/s41598-019-49465-7
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DOI: https://doi.org/10.1038/s41598-019-49465-7
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