Enhanced triple-α reaction reduces proton-rich nucleosynthesis in supernovae

Abstract

The rate of the triple-α reaction that forms 12C affects1,2 the synthesis of heavy elements in the Ga–Cd range in proton-rich neutrino-driven outflows of core-collapse supernovae3,4,5. Initially, these outflows contain only protons and neutrons; these later combine to form α particles, then 12C nuclei via the triple-α reaction, and eventually heavier nuclei as the material expands and cools. Previous experimental work6,7 demonstrated that despite the high temperatures encountered in these environments, the reaction is dominated by the well characterized Hoyle state resonance in 12C nuclei. At sufficiently high nucleon densities, however, proton- and neutron-scattering processes may alter the effective width of the Hoyle state8,9. This raises the questions of what the reaction rate in supernova outflows is, and how changes affect nucleosynthesis predictions. Here we report that in proton-rich core-collapse supernova outflows, these hitherto neglected processes enhance the triple-α reaction rate by up to an order of magnitude. The larger reaction rate suppresses the production of heavy proton-rich isotopes that are formed by the νp process3,4,5 (where ν is the neutrino and p is the proton) in the innermost ejected material of supernovae10,11,12,13. Previous work on the rate enhancement mechanism9 did not anticipate the importance of this enhancement for proton-rich nucleosynthesis. Because the in-medium contribution to the triple-α reaction rate must be present at high densities, this effect needs to be included in supernova nucleosynthesis models. This enhancement also differs from earlier sensitivity studies that explored variations of the unenhanced rate by a constant factor1,2, because the enhancement depends on the evolving thermodynamic conditions. The resulting suppression of heavy-element nucleosynthesis for realistic conditions casts doubt on the νp process being the explanation for the anomalously high abundances of 92,94Mo and 96,98Ru isotopes in the Solar System1,3,14 and for the signatures of early Universe element synthesis in the Ga–Cd range found in the spectra of ancient metal-poor stars15,16,17,18,19,20.

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Fig. 1: Enhancement of seed nuclei production.
Fig. 2: The total in-medium enhanced triple-α reaction rate.
Fig. 3: Nucleosynthesis results.
Fig. 4: Nucleosynthesis results with the rate enhancement at the upper end of the estimated nuclear uncertainty.
Fig. 5: Effect of the enhancement on p-nuclide production.

Data availability

The simulation data that support these findings is available from the corresponding author upon reasonable request.

Code availability

The reaction network library SkyNet used for this work is publicly available at https://bitbucket.org/jlippuner/skynet. The code used to run and analyse the simulations described here (which relies on the SkyNet library) is publicly available at https://bitbucket.org/lroberts/triplealphainmediumenhancement.

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Acknowledgements

We thank A. Arcones, J. Bliss, H. O. U. Fynbo, G. M. Hale, D. Lee and H. Weller for discussions. We acknowledge support from NSF awards PHY-1430152 (JINA Center for the Evolution of the Elements), PHY-1913554 and PHY-1102511. S.J. is supported by CSC-FRIB Postdoctoral Fellowship grant 201600090331. L.F.R. was partially supported by the US Department of Energy through the Advanced Computing (SciDAC) programme under award number DE-SC0017955.

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S.J. and L.F.R. carried out the calculations and analysis. S.M.A. carried out enhancement factor calculations. All authors contributed to the motivation, analysis and interpretation as well as the writing of the manuscript.

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Correspondence to Luke F. Roberts.

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Jin, S., Roberts, L.F., Austin, S.M. et al. Enhanced triple-α reaction reduces proton-rich nucleosynthesis in supernovae. Nature 588, 57–60 (2020). https://doi.org/10.1038/s41586-020-2948-7

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