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An increase in the 12C + 12C fusion rate from resonances at astrophysical energies

A Publisher Correction to this article was published on 28 June 2018

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Abstract

Carbon burning powers scenarios that influence the fate of stars, such as the late evolutionary stages of massive stars1 (exceeding eight solar masses) and superbursts from accreting neutron stars2,3. It proceeds through the 12C + 12C fusion reactions that produce an alpha particle and neon-20 or a proton and sodium-23—that is, 12C(12C, α)20Ne and 12C(12C, p)23Na—at temperatures greater than 0.4 × 109 kelvin, corresponding to astrophysical energies exceeding a megaelectronvolt, at which such nuclear reactions are more likely to occur in stars. The cross-sections4 for those carbon fusion reactions (probabilities that are required to calculate the rate of the reactions) have hitherto not been measured at the Gamow peaks4 below 2 megaelectronvolts because of exponential suppression arising from the Coulomb barrier. The reference rate5 at temperatures below 1.2 × 109 kelvin relies on extrapolations that ignore the effects of possible low-lying resonances. Here we report the measurement of the 12C(12C, α0,1)20Ne and 12C(12C, p0,1)23Na reaction rates (where the subscripts 0 and 1 stand for the ground and first excited states of 20Ne and 23Na, respectively) at centre-of-mass energies from 2.7 to 0.8 megaelectronvolts using the Trojan Horse method6,7 and the deuteron in 14N. The cross-sections deduced exhibit several resonances that are responsible for very large increases of the reaction rate at relevant temperatures. In particular, around 5 × 108 kelvin, the reaction rate is boosted to more than 25 times larger than the reference value5. This finding may have implications such as lowering the temperatures and densities8 required for the ignition of carbon burning in massive stars and decreasing the superburst ignition depth in accreting neutron stars to reconcile observations with theoretical models3.

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Fig. 1: Excitation functions from THM experimental yields.
Fig. 2: 12C + 12C astrophysical S(E)* factors.
Fig. 3: 12C + 12C reaction rate ratio.

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Change history

  • 28 June 2018

    In equation (1) of this Letter, the closing bracket was missing; in Extended Data Fig. 1 and the accompanying legend, ‘Φ(pd)’ should have been ‘Φ2(pd)’, and in the Methods the text “Odd J assignments are uncertain by ±1.” has been added. These errors have all been corrected online.

References

  1. Woosley, S. E., Heger, A. & Weaver, T. A. The evolution and explosion of massive stars. Rev. Mod. Phys. 74, 1015–1071 (2002).

    Article  ADS  CAS  Google Scholar 

  2. Keek, L. et al. First superburst from a classical low-mass X-ray binary transient. Astron. Astrophys. 479, 177–188 (2008).

    Article  ADS  CAS  Google Scholar 

  3. Cooper, R. L. et al. Possible resonances in the 12C + 12C fusion rate and superburst ignition. Astrophys. J. 702, 660–671 (2009).

    Article  ADS  CAS  Google Scholar 

  4. Iliadis, C. Nuclear Physics of Stars. (Wiley, Weinheim, 2007).

    Book  Google Scholar 

  5. Caughlan, G. R. & Fowler, W. A. Thermonuclear reaction rates V. At. Data Nucl. Data Tables 40, 283–334 (1988).

    Article  ADS  CAS  Google Scholar 

  6. Spitaleri, C. et al. The Trojan Horse Method in nuclear astrophysics. Phys. At. Nucl. 74, 1725–1739 (2011).

    Article  CAS  Google Scholar 

  7. Tribble, R. et al. Indirect techniques in nuclear astrophysics: a review. Rep. Prog. Phys. 77, 106901–106950 (2014).

    Article  MathSciNet  PubMed  ADS  CAS  Google Scholar 

  8. Pignatari, M. et al. The 12C + 12C reaction and the impact on nucleosynthesis in massive stars. Astrophys. J. 762, 31–54 (2013).

    Article  ADS  CAS  Google Scholar 

  9. Abegg, R. & Davis, C. A. 12Mg states observed via 20Ne(α,α0)20Ne. Phys. Rev. C 43, 2523–2540 (1991).

    Article  ADS  CAS  Google Scholar 

  10. Itoh, K. et al. Electroexcitation of giant multipole resonances in 24Mg. Phys. Rev. C 23, 945–959 (1981).

    Article  ADS  CAS  Google Scholar 

  11. Yang, G. C. et al. Isoscalar multipole strength in 24Mg through inelastic α scattering. Phys. Rev. C 13, 1376–1387 (1976).

    Article  ADS  CAS  Google Scholar 

  12. Vanhoy, J. R. et al. Proton resonances in 24Mg from E x = 12.7 to 15.7 MeV. Phys. Rev. C 36, 920–932 (1987).

    Article  ADS  CAS  Google Scholar 

  13. Bertrand, F. E. et al. Giant quadrupole resonance in 24,26Mg: a comparison of inelastic-scattering and α-capture experiments. Phys. Rev. Lett. 40, 635–638 (1978).

    Article  ADS  CAS  Google Scholar 

  14. Becker, H. W., Kettner, K. U., Rolfs, C. & Trautvetter, H. P. The 12C + 12C reaction at sub-Coulomb energies (II). Z. Phys. A 303, 305–312 (1981).

    Article  ADS  CAS  Google Scholar 

  15. Spillane, T. et al. 12C + 12C fusion reactions near the Gamow Energy. Phys. Rev. Lett. 98, 122501–122505 (2007).

    Article  PubMed  ADS  CAS  Google Scholar 

  16. Lane, A. M. & Thomas, R. G. R-matrix theory of nuclear reactions. Rev. Mod. Phys. 30, 257–353 (1958).

    Article  MathSciNet  ADS  Google Scholar 

  17. Aguilera, E. F. et al. New γ-ray measurements for 12C + 12C sub-Coulomb fusion: toward data unification. Phys. Rev. C 73, 064601–064612 (2006).

    Article  ADS  CAS  Google Scholar 

  18. Mazarakis, M. G. & Stephens, W. E. Experimental measurements of the 12C + 12C nuclear reactions at low energies. Phys. Rev. C 7, 1280–1287 (1973).

    Article  ADS  CAS  Google Scholar 

  19. High, M. D. & Cujec, B. The 12C + 12C sub-Coulomb fusion cross section. Nucl. Phys. A 282, 181–188 (1977).

    Article  ADS  Google Scholar 

  20. Kettner, K. U., Lorenz-Wirzba, H. & Rolfs, C. The 12C + 12C reaction at subcoulomb energies. Z. Phys. A 298, 65–75 (1980).

    Article  ADS  CAS  Google Scholar 

  21. Barrón-Palos, L. et al. Absolute cross sections measurement for the 12C + 12C system at astrophysically relevant energies. Nucl. Phys. A 779, 318–332 (2006).

    Article  ADS  CAS  Google Scholar 

  22. Caciolli, A. et al. Proton elastic scattering and proton induced γ-ray emission cross-sections on 23Na from 2 to 5 MeV. Nucl. Instrum. Meth. Phys. Res. B 266, 1392–1396 (2008).

    Article  ADS  CAS  Google Scholar 

  23. Zickefoose, J. 12C + 12C Fusion: Measurement and Advances Toward the Gamow Energy. PhD thesis, Univ. of Connecticut (2011); https://pqdtopen.proquest.com/doc/908637546.html?FMT=AI.

  24. Jiang, C. L. et al. Reaction rate for carbon burning in massive stars. Phys. Rev. C 97, 012801–012806 (2018).

    Article  ADS  Google Scholar 

  25. Thielemann, F.-K., Arnould, M. & Truran, J. W. Thermonuclear reactions rate from statistical model calculations. In Advances in Nuclear Astrophysics (2nd IAP Workshop) (ed. Vangioni-Flam, E.) 525 (Les Editions Frontières, Gif sur Yvette, 1987).

  26. Schatz, H. et al. Strong neutrino cooling by cycles of electron capture and β - decay in neutron star crust. Nature 505, 62–65 (2014).

    Article  PubMed  ADS  CAS  Google Scholar 

  27. Bravo, E. et al. Type Ia supernovae and the 12C + 12C reaction rate. Astron. Astrophys. 535, A114 (2011).

    Article  CAS  Google Scholar 

  28. Straniero, O., Piersanti, L. & Cristallo, S. Do we really know Mup (i.e. the transition mass between type Ia and core-collapse supernova progenitors)? J. Phys. Conf. Ser. 665, 012008 (2016).

    Article  Google Scholar 

  29. Strieder, F., Rolfs, C., Spitaleri, C. & Corvisiero, P. Electron-screening effects on fusion reactions. Naturwissenschaften 88, 461–467 (2001).

    Article  ADS  CAS  Google Scholar 

  30. Spitaleri, C. et al. Indirect 7Li(p,α)4He reaction at astrophysical energies. Phys. Rev. C 60, 055802–055809 (1999).

    Article  ADS  Google Scholar 

  31. Lamia, L. et al. An updated 6Li(p,α)3He reaction rate at astrophysical energies with the Trojan horse method. Astrophys. J. 768, 65–73 (2013).

    Article  ADS  CAS  Google Scholar 

  32. Tumino, A. et al. New determination of the 2H(d,p)3H and 2H(d,n)3He reaction rates at astrophysical energies. Astrophys. J. 785, 96–113 (2014).

    Article  ADS  CAS  Google Scholar 

  33. Pizzone, R. G. et al. First measurement of the 19F(α,p)22Ne reaction at energies of astrophysical relevance. Astrophys. J. 836, 57–63 (2017).

    Article  ADS  CAS  Google Scholar 

  34. Spitaleri, C. et al. Measurement of the 10B(p,α 0)7Be cross section from 5 keV to 1.5 MeV in a single experiment using the Trojan horse method. Phys. Rev. C 95, 035801–035814 (2017).

    Article  ADS  Google Scholar 

  35. Mukhamedzhanov, A. M. et al. Trojan Horse as an indirect technique in nuclear astrophysics. Resonance reactions. J. Phys. G 35, 014016–014022 (2008).

    Article  ADS  CAS  Google Scholar 

  36. La Cognata, M. et al. On the measurement of the 13C(α,n)16O S-factor at negative energies and its influence on the s-process. Astrophys. J. 777, 143–164 (2013).

    Article  ADS  CAS  Google Scholar 

  37. La Cognata, M. et al. Effect of high-energy resonances on the 18O(p, α)15N reaction rate at AGB and post-AGB relevant temperatures. Astrophys. J. 723, 1512–1522 (2010).

    Article  ADS  CAS  Google Scholar 

  38. Mukhamedzhanov, A. M. et al. Theory of deuteron stripping. From surface integrals to generalized R-matrix approach. Phys. Rev. C 84, 044616–044622 (2011).

    Article  ADS  CAS  Google Scholar 

  39. La Cognata, M. et al. The fluorine destruction in stars: first experimental study of the 19F(p0)16O reaction at astrophysical energies. Astrophys. J. 739, L54–L60 (2011).

    Article  ADS  CAS  Google Scholar 

  40. Zurmühle, R. W. et al. Observation of 12C cluster transfer by angular correlation measurements. Phys. Rev. C 49, 2549–2554 (1994).

    Article  ADS  Google Scholar 

  41. Belyaeva, T. L., Zelenskaya, N. S. & Aguero Granados, M. Investigation of quasimolecular states in 24Mg*Mg through the analysis of the angular dα correlations in the 12C(14N,d)24Mg(α)20Ne reaction. Phys. At. Nucl. 65, 1616–1627 (2002).

    Article  CAS  Google Scholar 

  42. Blatt, J. M. & Biedenharn, L. C. The angular distribution of scattering and reaction cross sections. Rev. Mod. Phys. 24, 258–272 (1952).

    Article  MATH  ADS  CAS  Google Scholar 

  43. Jiang, C. L. et al. Origin and consequences of 12C + 12C fusion resonances at deep sub-barrier energies. Phys. Rev. Lett. 110, 072701–072705 (2013).

    Article  PubMed  ADS  CAS  Google Scholar 

  44. La Cognata, M. et al. A Trojan Horse approach to the production of 18F in novae. Astrophys. J. 846, 65–71 (2017).

    Article  ADS  CAS  Google Scholar 

  45. Patterson, J. R., Winkler, H. & Zaidins, C. S. Experimental investigation of the stellar nuclear reaction 12C + 12C at low energies. Astrophys. J. 157, 367–373 (1969).

    Article  ADS  CAS  Google Scholar 

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Acknowledgements

We thank V. Z. Goldberg for having inspired the idea of the experiment and for discussions and assistance. We thank A. M. Mukhamedzhanov for having developed the theoretical framework of the THM. The aid of the technical staff of INFN-LNS during the preparation of the experiment is gratefully acknowledged. We thank M. Wiescher and F. X. Timmes for comments.

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Authors and Affiliations

Authors

Contributions

A.T. and C.S. proposed the experiment. A.T., C.S., M.L.C., G.L.G., I.I., L.L., R.G.P., S.M.R.P., R.S. and G.G.R. set up and ran the experiment, which lasted about one month. S.C., M.G., S.H., H.P., M.L.S., S.R. and L.T. participated in the data collection. A.T. performed the data reduction and analysis. M.L.C. developed the modified R-matrix code for the one-level many-channel case. A.T. and M.L.C. performed the statistical analysis. A.T. performed R-matrix calculations, interpreted the results, prepared the figures and wrote the manuscript. C.S. and M.L.C. contributed on the interpretation of the results. M.L.C. assisted with the figure preparation. L.L., R.G.P. and R.S. assisted with the astrophysical interpretation. A.T., C.S., M.L.C., S.C., G.L.G., I.I., L.L., R.G.P., G.G.R., R.S., S.R. and L.T. revised the manuscript.

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Correspondence to A. Tumino.

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Extended data figures and tables

Extended Data Fig. 1 Deuteron momentum distribution.

The experimental distribution Φ2(pd) is shown as filled black circles. Error bars represent standard 1σ uncertainties. The black line represents the theoretical shape (see text for details).

Extended Data Fig. 2 Pole diagram describing the quasi-free mechanism in the A(a,bB)s reaction.

The upper vertex refers to the break-up of a and the lower vertex shows the A(x,b)B process. Colours help to highlight the role of individual particles in the mechanism.

Extended Data Fig. 3 Typical ∆E–E spectrum.

The strongest loci from the bottom to the top correspond to p, d and α. ADC, analogue-to-digital converter.

Extended Data Fig. 4 Q-value as a function of the α detection angle Θα for the 12C(14N,α20Ne)2H reaction.

Blue and red solid lines cross the Q-value axis at −5.65 MeV and −7.28 MeV, highlighting the contributions of the ground and first excited states, respectively.

Extended Data Table 1 Resonance parameters of 24Mg levels entering the R-matrix fit and total plus partial widths resulting from the fit
Extended Data Table 2 Reaction rate of the 12C + 12C fusion reaction

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Tumino, A., Spitaleri, C., La Cognata, M. et al. An increase in the 12C + 12C fusion rate from resonances at astrophysical energies. Nature 557, 687–690 (2018). https://doi.org/10.1038/s41586-018-0149-4

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