Abstract
Some magnetic systems feature spin textures, real-space patterns in the orientation of spins that can topologically form non-trivial configurations. Among them, a vortex-like spin swirling texture known as a magnetic skyrmion has attracted particular attention. Lattices of skyrmions form in the helimagnet MnSi with a periodicity of 18 nm, which makes them amenable to investigation by Lorentz transmission electron microscopy in real space and by small-angle neutron scattering in momentum space. However, the dynamics of the skyrmion lattice are difficult to measure at the microelectronvolts energy scale at small wavevectors. Here we examine the low-energy excitations of the skyrmion state in MnSi by using the neutron spin-echo technique under small-angle neutron scattering conditions. We observe an asymmetric dispersion of the phason excitations of the lattice because of the string-like structure of the skyrmion cores.
This is a preview of subscription content, access via your institution
Access options
Access Nature and 54 other Nature Portfolio journals
Get Nature+, our best-value online-access subscription
$29.99 / 30 days
cancel any time
Subscribe to this journal
Receive 12 print issues and online access
$259.00 per year
only $21.58 per issue
Buy this article
- Purchase on SpringerLink
- Instant access to full article PDF
Prices may be subject to local taxes which are calculated during checkout
Similar content being viewed by others
Change history
02 October 2023
A Correction to this paper has been published: https://doi.org/10.1038/s41567-023-02241-x
References
Nagaosa, N. & Tokura, Y. Topological properties and dynamics of magnetic skyrmions. Nat. Nanotechnol. 8, 899–911 (2013).
Mühlbauer, S. et al. Skyrmion lattice in a chiral magnet. Science 323, 915–919 (2009).
Yu, X. Z. et al. Real-space observation of a two-dimensional skyrmion crystal. Nature 465, 901–904 (2010).
Neubauer, A. et al. Topological Hall effect in the A phase of MnSi. Phys. Rev. Lett. 102, 186602 (2009).
Grigoriev, S. V. et al. Interplay between crystalline chirality and magnetic structure in Mn1−xFexSi. Phys. Rev. B 81, 012408 (2010).
Tonomura, A. et al. Real-space observation of skyrmion lattice in helimagnet MnSi thin samples. Nano Lett. 12, 1673–1677 (2012).
Sato, T. J. et al. Magnon dispersion shift in the induced ferromagnetic phase of noncentrosymmetric MnSi. Phys. Rev. B 94, 144420 (2016).
Janoschek, M. et al. Helimagnon bands as universal excitations of chiral magnets. Phys. Rev. B 81, 214436 (2010).
Kugler, M. et al. Band structure of helimagnons in MnSi resolved by inelastic neutron scattering. Phys. Rev. Lett. 115, 097203 (2015).
Weber, T. et al. Field dependence of nonreciprocal magnons in chiral MnSi. Phys. Rev. B 97, 224403 (2018).
Pappas, C. et al. Magnetic fluctuations, precursor phenomena, and phase transition in MnSi under a magnetic field. Phys. Rev. Lett. 119, 047203 (2017).
Weber, T. et al. Topological magnon band structure of emergent Landau levels in a skyrmion lattice. Science 375, 1025–1030 (2022).
Garst, M. et al. Collective spin excitations of helices and magnetic skyrmions: review and perspectives of magnonics in non-centrosymmetric magnets. J. Phys. D: Appl. Phys 50, 293002 (2017).
Zang, J., Mostovoy, M., Han, J. H. & Nagaosa, N. Dynamics of skyrmion crystal in metallic thin films. Phys. Rev. Lett. 107, 136804 (2011).
Hoshino, S. & Nagaosa, N. Theory of magnetic skyrmion glass. Phys. Rev. B 97, 024413 (2018).
Waizner, J. Spin Wave Excitations in Magnetic Helices and Skyrmion Lattices. PhD Thesis, Univ. of Cologne (2017).
Koshibae, W. & Nagaosa, N. Dynamics of skyrmion in disordered chiral magnet of thin film form. Sci. Rep. 9, 5111 (2019).
Tatara, G. & Fukuyama, H. Phasons and excitations in skyrmion lattice. J. Phys. Soc. Jpn 83, 104711 (2014).
Onose, Y., Okamura, Y., Seki, S., Ishiwata, S. & Tokura, Y. Observation of magnetic excitations of skyrmion crystal in a helimagnetic insulator Cu2OSeO3. Phys. Rev. Lett. 109, 037603 (2012).
Kindervater, J. et al. Weak crystallization of fluctuating skyrmion textures in MnSi. Phys. Rev. X 9, 041059 (2019).
Weber, T. et al. Non-reciprocal magnons in non-centrosymmetric MnSi. AIP Adv. 8, 101328 (2018).
Weber, T. et al. Polarized inelastic neutron scattering of nonreciprocal spin waves in MnSi. Phys. Rev. B 100, 060404(R) (2019).
Mühlbauer, S. et al. Kinetic small angle neutron scattering of the skyrmion lattice in MnSi. New J. Phys. 18, 075017 (2016).
Blume, M. Polarization effects in the magnetic elastic scattering of slow neutrons. Phys. Rev. 130, 1670–1676 (1963).
Mochizuki, M. Spin-wave modes and their intense excitation effects in skyrmion crystals. Phys. Rev. Lett. 108, 017601 (2012).
Kataoka, M. Spin waves in systems with long period helical spin density waves due to the antisymmetric and symmetric exchange interactions. J. Phys. Soc. Jpn 56, 3635–3647 (1987).
Hayashida, S. et al. Inelastic neutron scattering on multiferroics NdFe3(BO3)4. Phys. Proc. 75, 127–133 (2015).
Forgan, E. M. et al. Institut Laue-Langevin (ILL) https://doi.org/10.5291/ILL-DATA.4-01-1584 (2018).
Forgan, E. M. et al. Institut Laue-Langevin (ILL) https://doi.org/10.5291/ILL-DATA.4-01-1645 (2021).
Acknowledgements
We greatly appreciate the fruitful discussions with W. Koshibae, G. Tatara and S. Hoshino. We thank K. Beauvois for providing access to OrientExpress, the test Laue neutron diffractometer at the Institut Laue-Langevin. Travel expenses for the neutron experiment performed using IN15 at ILL, France, were supported by the General User Program for Neutron Scattering Experiments, Institute for Solid State Physics, The University of Tokyo (proposal no. 18812), at JRR-3, Japan Atomic Energy Agency, Tokai, Japan. The work was supported by JST, CREST, grant no. JPMJCR20T1, Japan. The work was supported by Czech Ministry of Education, Youth and Sports (MEYS), project LTT20014.
Author information
Authors and Affiliations
Contributions
M.S. and H.K.-F. planned the neutron scattering experiments. M.S., E.M.F., E.B., V.R., I.H., E.C. and H.K.-F. carried out the neutron spin-echo experiments. Data analysis was done by M.S. in discussion with E.M.F. and E.B. The samples were grown by A.K. The paper was written by M.S., with additional material from E.M.F. and E.B. All other co-authors actively contributed to the final version.
Corresponding author
Ethics declarations
Competing interests
The authors declare no competing interests.
Peer review
Peer review information
Nature Physics thanks J. R. Stewart, D. Cabra and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.
Additional information
Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Supplementary information
Supplementary Information
Supplementary Sections 1–4, Figs. 1–5, Tables 1 and 2 and source data list.
Supplementary Data
Expected phase shifts for Supplementary Fig. 2. Variations in the echo phase shift for Supplementary Fig. 3. Energy estimated from the phase shift in the helical state for Supplementary Fig. 5.
Supplementary Code
Expected phase shifts for Supplementary Fig. 2. Proposed dispersion curve for Supplementary Fig. 4. Intermediate scattering function and phase shift for Fig. 3.
Source data
Source Data Fig. 1
Source data for graph and contour plot.
Source Data Fig. 2
Source data for graph and contour plot.
Source Data Fig. 3
Source data for graph.
Source Data Fig. 5
Source data for graph.
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Soda, M., Forgan, E.M., Blackburn, E. et al. Asymmetric slow dynamics of the skyrmion lattice in MnSi. Nat. Phys. 19, 1476–1481 (2023). https://doi.org/10.1038/s41567-023-02120-5
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1038/s41567-023-02120-5