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Subcycle squeezing of light from a time flow perspective

Abstract

Light as a carrier of information and energy plays a fundamental role in both general relativity and quantum physics, linking these areas that are still not fully compliant with each other. Usually the quantum nature of light is described in the frequency domain. Even for broadband quantum states with a well-defined carrier frequency, a quasi-continuous-wave picture is still applicable. However, recent access to subcycle quantum features of electromagnetic radiation promises a new class of time-dependent quantum states of light. Paralleled with the developments in attosecond science, these advances motivate an urgent need for a theoretical framework that treats arbitrary wavepackets of quantum light intrinsically in the time domain. Here, we formulate a consistent time-domain theory of the generation and sampling of few-cycle and subcycle pulsed squeezed states, leading to a relativistic interpretation in terms of induced changes in the local flow of time. Our theory enables the use of such states as a resource for novel ultrafast applications in quantum optics and quantum information.

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Fig. 1: Scheme of the generation and detection set-up and the corresponding evolution of the MIR quantum field \(\hat \varepsilon (z,t)\) inside the nonlinear crystal for a half-cycle MIR driving field with effective squeezing strength r = 5.
Fig. 2: Behaviour of the conformal time with respect to the laboratory time illustrated for the half-cycle pulse (see equation (7)) with r = 5 and Γ0/(2π) = 26 THz.
Fig. 3: RDV as a function of the strength of the half-cycle driving field and probe pulse duration.
Fig. 4: Pulsed squeezing for single-cycle driving.

Data availability

The data that support the plots within this paper and other findings of this study are available from the corresponding author upon reasonable request.

References

  1. 1.

    Dorfman, K. E., Schlawin, F. & Mukamel, S. Nonlinear optical signals and spectroscopy with quantum light. Rev. Mod. Phys. 88, 045008 (2016).

    ADS  MathSciNet  Article  Google Scholar 

  2. 2.

    Knill, E., Laflamme, R. & Milburn, G. J. A scheme for efficient quantum computation with linear optics. Nature 409, 46–52 (2001).

    ADS  Article  Google Scholar 

  3. 3.

    Weedbrook, C. et al. Gaussian quantum information. Rev. Mod. Phys. 84, 621–669 (2012).

    ADS  Article  Google Scholar 

  4. 4.

    Broome, M. A. et al. Photonic boson sampling in a tunable circuit. Science 339, 794–798 (2013).

    ADS  Article  Google Scholar 

  5. 5.

    Boto, A. N. et al. Quantum interferometric optical lithography: exploiting entanglement to beat the diffraction limit. Phys. Rev. Lett. 85, 2733–2736 (2000).

    ADS  Article  Google Scholar 

  6. 6.

    D’Angelo, M., Chekhova, M. V. & Shih, Y. Two-photon diffraction and quantum lithography. Phys. Rev. Lett. 87, 013602 (2001).

    ADS  Article  Google Scholar 

  7. 7.

    Jones, D. J. et al. Carrier-envelope phase control of femtosecond mode-locked lasers and direct optical frequency synthesis. Science 288, 635–639 (2000).

    ADS  Article  Google Scholar 

  8. 8.

    Holzwarth, R. et al. Optical frequency synthesizer for precision spectroscopy. Phys. Rev. Lett. 85, 2264–2267 (2000).

    ADS  Article  Google Scholar 

  9. 9.

    Corkum, P. B. & Krausz, F. Attosecond science. Nat. Phys. 3, 381–387 (2007).

    Article  Google Scholar 

  10. 10.

    Krausz, F. & Ivanov, M. Attosecond physics. Rev. Mod. Phys. 81, 163–234 (2009).

    ADS  Article  Google Scholar 

  11. 11.

    Moskalenko, A. S., Zhu, Z.-G. & Berakdar, J. Charge and spin dynamics driven by ultrashort extreme broadband pulses: a theory perspective. Phys. Rep. 672, 1–82 (2017).

    ADS  MathSciNet  Article  Google Scholar 

  12. 12.

    Riek, C. et al. Direct sampling of electric-field vacuum fluctuations. Science 350, 420–423 (2015).

    ADS  MathSciNet  Article  Google Scholar 

  13. 13.

    Moskalenko, A. S., Riek, C., Seletskiy, D. V., Burkard, G. & Leitenstorfer, A. Paraxial theory of direct electro-optic sampling of the quantum vacuum. Phys. Rev. Lett. 115, 263601 (2015).

    ADS  Article  Google Scholar 

  14. 14.

    Benea-Chelmus, I.-C. et al. Subcycle measurement of intensity correlations in the terahertz frequency range. Phys. Rev. A 93, 043812 (2016).

    Article  Google Scholar 

  15. 15.

    Riek, C. et al. Subcycle quantum electrodynamics. Nature 541, 376–379 (2017).

    ADS  Article  Google Scholar 

  16. 16.

    Benea-Chelmus, I.-C., Settembrini, F. F., Scalari, G. & Faist, J. Electric field correlation measurements on the electromagnetic vacuum state. Nature 568, 202–206 (2019).

    ADS  Article  Google Scholar 

  17. 17.

    Breitenbach, G., Schiller, S. & Mlynek, J. Measurement of the quantum states of squeezed light. Nature 387, 471–475 (1997).

    ADS  Article  Google Scholar 

  18. 18.

    Lvovsky, A. I. in Photonics: Scientific Foundations, Technology and Applications Vol. 1 (ed. Andrews, D. L.) 121–163 (John Wiley & Sons, 2015).

  19. 19.

    Chekhova, M., Leuchs, G. & Żukowski, M. Bright squeezed vacuum: entanglement of macroscopic light beams. Opt. Commun. 337, 27–43 (2015).

    ADS  Article  Google Scholar 

  20. 20.

    Caves, C. M. Quantum-mechanical noise in an interferometer. Phys. Rev. D 23, 1693–1708 (1981).

    ADS  Article  Google Scholar 

  21. 21.

    Xiao, M., Wu, L.-A. & Kimble, H. J. Precision measurement beyond the shot-noise limit. Phys. Rev. Lett. 59, 278–281 (1987).

    ADS  Article  Google Scholar 

  22. 22.

    Grangier, P., Slusher, R. E., Yurke, B. & LaPorta, A. Squeezed-light–enhanced polarization interferometer. Phys. Rev. Lett. 59, 2153–2156 (1987).

    ADS  Article  Google Scholar 

  23. 23.

    Abadie, J. et al. A gravitational wave observatory operating beyond the quantum shot-noise limit. Nat. Phys. 7, 962–965 (2011).

    Article  Google Scholar 

  24. 24.

    Aasi, J. et al. Enhanced sensitivity of the LIGO gravitational wave detector by using squeezed states of light. Nat. Photon. 7, 613–619 (2013).

    ADS  Article  Google Scholar 

  25. 25.

    Abbott, B. P. et al. Observation of gravitational waves from a binary black hole merger. Phys. Rev. Lett. 116, 061102 (2016).

    ADS  MathSciNet  Article  Google Scholar 

  26. 26.

    Blow, K. J., Loudon, R., Phoenix, S. J. D. & Shepherd, T. J. Continuum fields in quantum optics. Phys. Rev. A 42, 4102–4114 (1990).

    ADS  Article  Google Scholar 

  27. 27.

    Anderson, M. E., McAlister, D. F., Raymer, M. G. & Gupta, M. C. Pulsed squeezed-light generation in χ (2) nonlinear waveguides. J. Opt. Soc. Am. B 14, 3180–3190 (1997).

    ADS  Article  Google Scholar 

  28. 28.

    Slusher, R. E., Grangier, P., LaPorta, A., Yurke, B. & Potasek, M. J. Pulsed squeezed light. Phys. Rev. Lett. 59, 2566–2569 (1987).

    ADS  Article  Google Scholar 

  29. 29.

    Wasilewski, W., Lvovsky, A. I., Banaszek, K. & Radzewicz, C. Pulsed squeezed light: simultaneous squeezing of multiple modes. Phys. Rev. A 73, 063819 (2006).

    ADS  Article  Google Scholar 

  30. 30.

    Harris, S. E. Chirp and compress: toward single-cycle biphotons. Phys. Rev. Lett. 98, 063602 (2007).

    ADS  Article  Google Scholar 

  31. 31.

    Horoshko, D. B. & Kolobov, M. I. Towards single-cycle squeezing in chirped quasi-phase-matched optical parametric down-conversion. Phys. Rev. A 88, 033806 (2013).

    ADS  Article  Google Scholar 

  32. 32.

    Christ, A., Brecht, B., Mauerer, W. & Silberhorn, C. Theory of quantum frequency conversion and type-II parametric down-conversion in the high-gain regime. New J. Phys. 15, 053038 (2013).

    ADS  MathSciNet  Article  Google Scholar 

  33. 33.

    Shaked, Y. et al. Lifting the bandwidth limit of optical homodyne measurement with broadband parametric amplification. Nat. Commun. 9, 609 (2018).

    ADS  Article  Google Scholar 

  34. 34.

    Sharapova, P. R., Tikhonova, O. V., Lemieux, S., Boyd, R. W. & Chekhova, M. V. Bright squeezed vacuum in a nonlinear interferometer: frequency and temporal Schmidt-mode description. Phys. Rev. A 97, 053827 (2018).

    ADS  Article  Google Scholar 

  35. 35.

    Planken, P. C. M., Nienhuys, H.-K., Bakker, H. J. & Wenckebach, T. Measurement and calculation of the orientation dependence of terahertz pulse detection in ZnTe. J. Opt. Soc. Am. B 18, 313–317 (2001).

    ADS  Article  Google Scholar 

  36. 36.

    Loudon, R. The Quantum Theory of Light (Oxford Univ. Press, 2000).

  37. 37.

    Boyd, R. W. Nonlinear Optics 3rd edn (Academic, 2008).

  38. 38.

    Brabec, T. & Krausz, F. Nonlinear optical pulse propagation in the single-cycle regime. Phys. Rev. Lett. 78, 3282–3285 (1997).

    ADS  Article  Google Scholar 

  39. 39.

    Keiber, S. et al. Electro-optic sampling of near-infrared waveforms. Nat. Photon. 10, 159–162 (2016).

    ADS  Article  Google Scholar 

  40. 40.

    Virally, S. & Reulet, B. Unidimensional time domain quantum optics. Preprint at arXiv https://arxiv.org/abs/1810.06932 (2018).

  41. 41.

    Shen, Y. R. Principles of Nonlinear Optics (Wiley-Interscience, 1984).

  42. 42.

    Powers, P. E. Fundamentals of Nonlinear Optics (Taylor & Francis, 2011).

  43. 43.

    Guedes, T. L. M. et al. Spectra of ultrabroadband squeezed pulses and the finite-time Unruh–Davies effect. Phys. Rev. Lett. 122, 053604 (2019).

    ADS  Article  Google Scholar 

  44. 44.

    Belgiorno, F. et al. Dielectric black holes induced by a refractive index perturbation and the Hawking effect. Phys. Rev. D 83, 024015 (2011).

    ADS  Article  Google Scholar 

  45. 45.

    Mukhanov, V. Physical Foundations of Cosmology (Cambridge Univ. Press, 2005).

  46. 46.

    Gallot, G. & Grischkowsky, D. Electro-optic detection of terahertz radiation. J. Opt. Soc. Am. B 16, 1204–1212 (1999).

    ADS  Article  Google Scholar 

  47. 47.

    Glauber, R. J. The quantum theory of optical coherence. Phys. Rev. 130, 2529–2539 (1963).

    ADS  MathSciNet  Article  Google Scholar 

  48. 48.

    Kawada, Y., Yasuda, T. & Takahashi, H. Carrier envelope phase shifter for broadband terahertz pulses. Opt. Lett. 41, 986–989 (2016).

    ADS  Article  Google Scholar 

  49. 49.

    Riek, C., Sulzer, P., Seeger, M., Seletskiy, D. V. & Leitenstorfer, A. Simultaneous sampling of electric field quadratures in the time domain. In Conference on Lasers and Electro-Optics, OSA Technical Digest paper SM1L.1 (Optical Society of America, 2016).

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Acknowledgements

We thank P. Sulzer and R. Haussmann for discussions. Support by the DFG via SFB767, by Baden-Württemberg Stiftung via the Elite programme for Postdocs (project ‘Fundamental aspects of relativity and causality in time-resolved quantum optics’) and by the Young Scholar Fund of the University of Konstanz is acknowledged. M.K. is indebted to the LGFG PhD fellowship programme of the University of Konstanz.

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A.S.M., D.V.S. and G.B. conceived the idea. A.S.M. managed the project and supervised the research. M.K. found the exact analytical solution in the time domain, performed numerical calculations and prepared the figures. T.L.d.M.G. obtained the perturbative analytic solution via the squeezing operator in the frequency domain. M.K., T.L.d.M.G. and A.S.M. wrote the first version of the paper. D.V.S. and A.L. provided several important physical insights and interpretations. All authors discussed the results and contributed to the writing of the final manuscript.

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Correspondence to Andrey S. Moskalenko or Guido Burkard.

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Peer review information: Nature Physics thanks Mikhail Fedorov, Avi Pe’er, Dmitry Strekalov and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.

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Supplementary text, Supplementary Figs. 1–5 and Supplementary references.

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Kizmann, M., Guedes, T.L.d.M., Seletskiy, D.V. et al. Subcycle squeezing of light from a time flow perspective. Nat. Phys. 15, 960–966 (2019). https://doi.org/10.1038/s41567-019-0560-2

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