Ultrafast preparation and detection of ring currents in single atoms

Abstract

Quantum particles can penetrate potential barriers by tunnelling1. If that barrier is rotating, the tunnelling process is modified2,3. This is typical for electrons in atoms, molecules or solids exposed to strong circularly polarized laser pulses4,5,6. Here we measure how the transmission probability through a rotating tunnel depends on the sign of the magnetic quantum number m of the electron and thus on the initial direction of rotation of its quantum phase. We further show that our findings agree with a semiclassical picture, in which the electron keeps part of that rotary motion on its way through the tunnel by measuring m-dependent modification of the electron emission pattern. These findings are relevant for attosecond metrology as well as for interpretation of strong-field electron emission from atoms and molecules7,8,9,10,11,12,13,14 and directly demonstrate the creation of ring currents in bound states of ions with attosecond precision. In solids, this could open a way to inducing and controlling ring-current-related topological phenomena15.

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Fig. 1: Experimental preparation of ring currents by m-dependent tunnel-ionization.
Fig. 2: Detection of ring currents by momentum-resolved m-dependent tunnel-ionization.
Fig. 3: Energy-resolved electron spectra showing ring current transport during tunnelling.

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Acknowledgements

This work was supported by the DFG Priority Programme ‘Quantum Dynamics in Tailored Intense Fields’ (projects DO 604/29-1, BA 5623/1-1, IV 156/6-1, SM 292/5-1).

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S.E., M.K., M.R., A.H., J.R., F.T., K.F., N.S., K.H., L.Ph.H.S., T.J., M.S. and R.D. contributed to the experiment. S.E., M.K., M.R., K.L., I.B., J.K., F.M., M.I., O.S. and R.D. contributed to the theoretical results. S.E., M.K., T.J., M.S. and R.D. performed the analysis of the experimental data. All authors contributed to the manuscript.

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Correspondence to Sebastian Eckart or Reinhard Dörner.

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Eckart, S., Kunitski, M., Richter, M. et al. Ultrafast preparation and detection of ring currents in single atoms. Nature Phys 14, 701–704 (2018). https://doi.org/10.1038/s41567-018-0080-5

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