Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • Article
  • Published:

Brilliant femtosecond-laser-driven hard X-ray flashes from carbon nanotube plasma

Abstract

Brilliant X- and γ-ray sources with ultrashort duration are widely pursued in fundamental science, industry and medicine. Compact femtosecond X-ray sources based on relativistic electrons accelerated by the laser wakefield in gases have performed outstandingly. Their energy conversion efficiency from laser to hard X-ray photons (>10 keV) is, however, limited to 10−7–10−5. Here we report the high-yield generation of hard X-ray flashes from targets made of carbon nanotubes, instead of gases. Orders-of-magnitude more electrons, accelerated to relativistic energy, are strongly wiggled inside a micrometre-scale, near-critical density plasma formed by the nanotube target, emitting 1012 high-energy photons per shot. The yield of hard X-rays exceeds 1010 photons per joule, corresponding to an unprecedented efficiency of 10−3. Irradiated by upcoming 10-PW-class lasers, such targets can deliver 10-MeV photons with brightness outperforming existing sources by two orders of magnitude.

This is a preview of subscription content, access via your institution

Access options

Buy this article

Prices may be subject to local taxes which are calculated during checkout

Fig. 1: Evolution of a CNT target interacting with the rising edge of the petawatt laser pulse.
Fig. 2: Schematic drawing and the measured photon spectra.
Fig. 3: X-rays from the NCD plasmas.
Fig. 4: DLA electrons and scaling law in the CS regime.
Fig. 5: Performance of typical X-ray sources.

Similar content being viewed by others

Data availability

The main data that support the findings of this study are available within the paper and its Supplementary Information. Extra data are available from the corresponding authors upon request.

Code availability

The open-source code EPOCH was used and the detailed set-up of the simulations that support the plots and other findings of this study are presented in the Supplementary Information.

References

  1. Albert, F. L. & Thomas, A. G. R. Applications of laser wakefield accelerator-based light sources. Plasma Phys. Control. Fusion 58, 103001 (2016).

    Article  ADS  Google Scholar 

  2. Wang, W. et al. Free-electron lasing at 27 nanometres based on a laser wakefield accelerator. Nature 595, 516–520 (2021).

    Article  ADS  Google Scholar 

  3. Phuoc, K. T. et al. All-optical Compton gamma-ray source. Nat. Photon. 6, 308–311 (2012).

    Article  ADS  Google Scholar 

  4. Powers, N. et al. Quasi-monoenergetic and tunable X-rays from a laser-driven Compton light source. Nat. Photon. 8, 28–31 (2014).

    Article  ADS  Google Scholar 

  5. Sarri, G. et al. Ultrahigh brilliance multi-Mev γ-ray beams from nonlinear relativistic Thomson scattering. Phys. Rev. Lett. 113, 224801 (2014).

    Article  ADS  Google Scholar 

  6. Khrennikov, K. et al. Tunable all-optical quasimonochromatic Thomson X-ray source in the nonlinear regime. Phys. Rev. Lett. 114, 195003 (2015).

    Article  ADS  Google Scholar 

  7. Tsai, H. E. et al. Compact tunable Compton X-ray source from laser-plasma accelerator and plasma mirror. Phys. Plasmas 22, 023106 (2015).

    Article  ADS  Google Scholar 

  8. Yu, C. et al. Ultrahigh brilliance quasi-monochromatic MeV γ-rays based on self- synchronized all-optical Compton scattering. Sci. Rep. 6, 29518 (2016).

    Article  ADS  Google Scholar 

  9. Cole, J. M. et al. Experimental evidence of radiation reaction in the collision of a high-intensity laser pulse with a laser-wakefield accelerated electron beam. Phys. Rev. X 8, 011020 (2018).

    Google Scholar 

  10. Zhu, C. et al. Inverse Compton scattering X-ray source from laser electron accelerator in pure nitrogen with 15-TW laser pulses. Plasma Phys. Control. Fusion 61, 024001 (2019).

    Article  ADS  Google Scholar 

  11. Poder, K. et al. Experimental signatures of the quantum nature of radiation reaction in the field of an ultraintense laser. Phys. Rev. X 8, 031004 (2018).

    Google Scholar 

  12. Kneip, S. et al. Observation of synchrotron radiation from electrons accelerated in a petawatt-laser-generated plasma cavity. Phys. Rev. Lett. 100, 105006 (2008).

    Article  ADS  Google Scholar 

  13. Cipiccia, S. et al. Gamma-rays from harmonically resonant betatron oscillations in a plasma wake. Nat. Phys. 7, 867–871 (2011).

    Article  Google Scholar 

  14. Wang, X. et al. Quasi-monoenergetic laser-plasma acceleration of electrons to 2 GeV. Nat. Commun. 4, 1988 (2013).

    Article  ADS  Google Scholar 

  15. Cole, J. M. et al. Laser-wakefield accelerators as hard X-ray sources for 3D medical imaging of human bone. Sci. Rep. 5, 13244 (2015).

    Article  ADS  Google Scholar 

  16. Corde, S. et al. Femtosecond X-rays from laser-plasma accelerators. Rev. Mod. Phys. 85, 1–48 (2013).

    Article  ADS  Google Scholar 

  17. Huang, T. W. et al. Highly efficient laser-driven Compton gamma-ray source. New J. Phys. 21, 013008 (2019).

    Article  ADS  Google Scholar 

  18. Sylla, F. et al. Anticorrelation between ion acceleration and nonlinear coherent structures from laser-underdense plasma interaction. Phys. Rev. Lett. 108, 115003 (2012).

    Article  ADS  Google Scholar 

  19. Chen, S. N. et al. Density and temperature characterization of long-scale length, near-critical density controlled plasma produced from ultra-low density plastic foam. Sci. Rep. 6, 21495 (2016).

    Article  ADS  Google Scholar 

  20. Wang, P. et al. Fabrication of large-area uniform carbon nanotube foams as near-critical-density targets for laser-plasma experiments. High Power Laser Sci. Eng. 9, e29 (2021).

    Article  Google Scholar 

  21. Choi, I. W. et al. Highly efficient double plasma mirror producing ultrahigh-contrast multi-petawatt laser pulses. Opt. Lett. 45, 6342–6345 (2020).

    Article  ADS  Google Scholar 

  22. Bin, J. et al. Enhanced laser-driven ion acceleration by superponderomotive electrons generated from near-critical-density plasma. Phys. Rev. Lett. 120, 074801 (2018).

    Article  ADS  Google Scholar 

  23. Di Piazza, A. et al. Extremely high-intensity laser interactions with fundamental quantum systems. Rev. Mod. Phys. 84, 1177 (2012).

    Article  ADS  Google Scholar 

  24. Ostermayr, T. M. et al. Laser-driven X-ray and proton micro-source and application to simultaneous single-shot bi-modal radiographic imaging. Nat. Commun. 11, 6174 (2020).

    Article  ADS  Google Scholar 

  25. Cipiccia, S. et al. A tuneable ultra-compact high-power, ultra-short pulsed, bright gamma-ray source based on bremsstrahlung radiation from laser-plasma accelerated electrons. J. Appl. Phys. 111, 063302 (2012).

    Article  ADS  Google Scholar 

  26. Günther, M. et al. Forward-looking insights in laser-generated ultra-intense γ-ray and neutron sources for nuclear application and science. Nat. Commun. 13, 170 (2022).

    Article  ADS  Google Scholar 

  27. Benedetti, A. et al. Giant collimated gamma-ray flashes. Nat. Photon. 12, 319–323 (2018).

    Article  ADS  Google Scholar 

  28. Sampath, A. et al. Extremely dense gamma-ray pulses in electron beam-multifoil collisions. Phys. Rev. Lett. 126, 64801 (2021).

    Article  ADS  Google Scholar 

  29. Mourou, G. et al. The future is fibre accelerators. Nat. Photon. 7, 258–261 (2013).

    Article  ADS  Google Scholar 

  30. Fu, C., Zhang, G. & Ma, Y. New opportunities for nuclear and atomic physics on the femto- to nanometer scale with ultra-high-intensity lasers. Matter Radiat. Extrem. 7, 024201 (2022).

    Article  Google Scholar 

  31. Rio, M. S. D. & Dejus, R. J. XOP v2.4: recent developments of the X-ray optics software toolkit. Proc. SPIE 8141, 814115 (2011).

    Article  Google Scholar 

  32. Bohlen, T. T. et al. The FLUKA code: developments and challenges for high energy and medical applications. Nucl. Data Sheets 120, 211–214 (2014).

    Article  ADS  Google Scholar 

  33. Bonnet, T. et al. Response functions of imaging plates to photons, electrons and 4He particles. Rev. Sci. Instrum. 84, 103510 (2013).

    Article  ADS  Google Scholar 

  34. Arber, T. D. et al. Contemporary particle-in-cell approach to laser-plasma modelling. Plasma Phys. Control. Fusion 57, 113001 (2015).

    Article  ADS  Google Scholar 

Download references

Acknowledgements

The work was supported by the Institute for Basic Science, Korea under project code IBS-R012-D1, and the National Grand Instrument Project, China (2019YFF01014402). W.M. acknowledges support from the National Science Fund for Distinguished Young Scholars (12225501). W.M. and X.Y. thank the NSFC innovation group project (11921006) for financial support. X.Y. acknowledges support from the National Natural Science Foundation of China (11025523 and J1103206). The PIC simulations were carried out in Shanghai Super Computation Center and the High-performance Computing Platform of Peking University. We thank H. Deng for fruitful discussions.

Author information

Authors and Affiliations

Authors

Contributions

W.M., X.Y. and C.H.N. conducted the work. The experiments were performed by Y.S., P.W., S.G.L., Y.J.R., H.W.L., J.W.Y., J.H.S., S.K.L., Z.P., D.K., Z.M., J.L., S.X. and I.W.C. Y.S. carried out all simulations. Some details of the physics were clarified by Z.D., W.Z. and T.T. The manuscript was written by Y.S. and revised by W.M. All authors reviewed the manuscript.

Corresponding authors

Correspondence to Chang Hee Nam or Wenjun Ma.

Ethics declarations

Competing interests

The authors declare no competing interests.

Peer review

Peer review information

Nature Photonics thanks Tobias Ostermayr, Ingo Uschmann and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.

Additional information

Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Supplementary information

Supplementary Information

Supplementary Figs. 1–25, Tables 1–7 and Sections I–V.

Rights and permissions

Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Shou, Y., Wang, P., Lee, S.G. et al. Brilliant femtosecond-laser-driven hard X-ray flashes from carbon nanotube plasma. Nat. Photon. 17, 137–142 (2023). https://doi.org/10.1038/s41566-022-01114-8

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1038/s41566-022-01114-8

This article is cited by

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing