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Subradiant directional memory in cooperative scattering

A Publisher Correction to this article was published on 27 January 2022

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Abstract

The interaction between electromagnetic fields and randomly structured matter is at the core of many natural phenomena. In the steady state, its microscopic description involves the superposition of the incoming radiation and the field due to the presence of the material system. Owing to reciprocity, this secondary emission manifests a striking coherent feature leading to an enhancement of backward intensity. This portrayal is complicated when the incident field is suddenly shut off since the outcome depends on both the spatial and temporal properties of radiation. Here we demonstrate that a directional memory of the incoming field persists long after the incident radiation ceases to be present within a spatially bounded medium. Our results reveal that a coherent back-emission emerges as a result of subradiant quasi-modes of an electromagnetic field located primarily in the vicinity of the medium’s interface. The paradigm is general and complements the rich phenomenology of light interaction with strongly scattered matter. The temporal and spatial properties of this long-lived, reciprocity-maintaining radiation depend on the type of illumination, which opens up new opportunities for memory applications.

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Fig. 1: Long-lived directional memory in secondary emission.
Fig. 2: Initial conditions of coupled oscillators.
Fig. 3: Angular distributions of far-field intensities azimuthally averaged and recorded at three different delays: 0, 12.5γ−1, and 25γ−1.
Fig. 4: Time-resolved angular intensity distribution for a cylindrical medium consisting of 125 randomly distributed scatterers with \(\bar d\) = 0.3λ.

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All the data used within this paper are available from the corresponding author upon reasonable request.

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References

  1. Kuga, Y. & Ishimaru, A. Retroreflectance from a dense distribution of spherical particles. J. Opt. Soc. Am. A 1, 831–835 (1984).

    Article  ADS  Google Scholar 

  2. Van Albada, M. P. & Lagendijk, A. Observation of weak localization of light in a random medium. Phys. Rev. Lett. 55, 2692–2695 (1985).

    Article  ADS  Google Scholar 

  3. Wolf, P. E. & Maret, G. Weak localization and coherent backscattering of photons in disordered media. Phys. Rev. Lett. 55, 2696–2699 (1985).

    Article  ADS  Google Scholar 

  4. De Vries, P., Van Coevorden, D. V. & Lagendijk, A. Point scatterers for classical waves. Rev. Mod. Phys. 70, 447–466 (1998).

    Article  ADS  Google Scholar 

  5. Ellis, J. & Dogariu, A. Optical polarimetry of random fields. Phys. Rev. Lett. 95, 203905 (2005).

    Article  ADS  Google Scholar 

  6. Feynman, R. P., Leighton, R. B., & Sands, M. The Feynman Lectures on Physics Vol. I (Basic Books, 2011).

  7. Jackson, J. D. Classical Electrodynamics (Wiley, 1999).

  8. Thirunamachandran, T. Intermolecular interactions in the presence of an intense radiation field. Mol. Phys. 40, 393–399 (1980).

    Article  ADS  Google Scholar 

  9. O’dell, D., Giovanazzi, S., Kurizki, G. & Akulin, V. M. Bose–Einstein condensates with 1/r interatomic attraction: electromagnetically induced “gravity”. Phys. Rev. Lett. 84, 5687–5690 (2000).

    Article  ADS  Google Scholar 

  10. Luis-Hita, J. et al. Light induced inverse-square law interactions between nanoparticles:“mock gravity” at the nanoscale. Phys. Rev. Lett. 123, 143201 (2019).

    Article  ADS  Google Scholar 

  11. Shevchenko, A., Roussey, M., Friberg, A. T. & Setälä, T. Polarization time of unpolarized light. Optica 4, 64–70 (2017).

    Article  ADS  Google Scholar 

  12. Cipris, A., Bachelard, R., Kaiser, R. & Guerin, W. Van der Waals dephasing for Dicke subradiance in cold atomic clouds. Phys. Rev. A 103, 033714 (2021).

    Article  ADS  Google Scholar 

  13. Ishimaru, A. Wave Propagation and Scattering in Random Media (Academic, 1978).

  14. Lehmberg, R. H. Radiation from an N-atom system. I. General formalism. Phys. Rev. A 2, 883–888 (1970).

    Article  ADS  Google Scholar 

  15. Agarwal, G. S. Quantum Statistical Theories of Spontaneous Emission and Their Relation to Other Approaches (Springer, 1974).

  16. Svidzinsky, A. A., Chang, J. T. & Scully, M. O. Cooperative spontaneous emission of N atoms: many-body eigenstates, the effect of virtual Lamb shift processes, and analogy with radiation of N classical oscillators. Phys. Rev. A 81, 053821 (2010).

    Article  ADS  Google Scholar 

  17. Skipetrov, S. E. & Goetschy, A. Eigenvalue distributions of large Euclidean random matrices for waves in random media. J. Phys. A Math. Theor. 44, 065102 (2011).

    Article  ADS  MathSciNet  Google Scholar 

  18. Goetschy, A. & Skipetrov, S. E. Non-Hermitian Euclidean random matrix theory. Phys. Rev. E 84, 011150 (2011).

    Article  ADS  Google Scholar 

  19. Fox, A. G. & Li, T. Resonant modes in a maser interferometer. Bell Syst. Tech. J. 40, 453–488 (1961).

    Article  Google Scholar 

  20. Mishchenko, M. I. et al. Electromagnetic scattering by a morphologically complex object: fundamental concepts and common misconceptions. J. Quant. Spectrosc. Radiat. Transf. 112, 671–692 (2011).

    Article  ADS  Google Scholar 

  21. Wiersma, D. S., van Albada, M. P., van Tiggelen, B. A. & Lagendijk, A. Experimental evidence for recurrent multiple scattering events of light in disordered media. Phys. Rev. Lett. 74, 4193–4196 (1995).

    Article  ADS  Google Scholar 

  22. Akkermans, E., Wolf, P. E., Maynard, R. & Maret, G. Theoretical study of the coherent backscattering of light by disordered media. J. Phys. (Paris) 49, 77–98 (1988).

    Article  ADS  Google Scholar 

  23. Prasad, S. & Glauber, R. J. Coherent radiation by a spherical medium of resonant atoms. Phys. Rev. A 82, 063805 (2010).

    Article  ADS  Google Scholar 

  24. Schilder, N. J. et al. Polaritonic modes in a dense cloud of cold atoms. Phys. Rev. A 93, 063835 (2016).

    Article  ADS  Google Scholar 

  25. Kwong, C. C. et al. Cooperative emission of a coherent superflash of light. Phys. Rev. Lett. 113, 223601 (2014).

    Article  ADS  Google Scholar 

  26. Jennewein, S. et al. Coherent scattering of near-resonant light by a dense, microscopic cloud of cold two-level atoms: experiment versus theory. Phys. Rev. A 97, 053816 (2018).

    Article  ADS  Google Scholar 

  27. Corey, R., Kissner, M. & Saulnier, P. Coherent backscattering of light. Am. J. Phys. 63, 560–564 (1995).

    Article  ADS  Google Scholar 

  28. Weiss, P., Cipris, A., Araújo, M. O., Kaiser, R. & Guerin, W. Robustness of Dicke subradiance against thermal decoherence. Phys. Rev. A 100, 033833 (2019).

    Article  ADS  Google Scholar 

  29. Tourin, A., Derode, A., Roux, P., Van Tiggelen, B. A. & Fink, M. Time-dependent coherent backscattering of acoustic waves. Phys. Rev. Lett. 79, 3637–3639 (1997).

    Article  ADS  Google Scholar 

  30. Akkermans, E., & Montambaux, G. Mesoscopic Physics of Electrons and Photons (Cambridge Univ. Press, 2007).

  31. Fearn, H., James, D. F. & Milonni, P. W. Microscopic approach to reflection, transmission, and the Ewald–Oseen extinction theorem. Am. J. Phys. 64, 986–995 (1996).

    Article  ADS  Google Scholar 

  32. Rainò, G. et al. Superfluorescence from lead halide perovskite quantum dot superlattices. Nature 563, 671–675 (2018).

    Article  ADS  Google Scholar 

  33. Durand, M., Popoff, S. M., Carminati, R. & Goetschy, A. Optimizing light storage in scattering media with the dwell-time operator. Phys. Rev. Lett. 123, 243901 (2019).

    Article  ADS  Google Scholar 

  34. Yu, S., Qiu, C. W., Chong, Y., Torquato, S. & Park, N. Engineered disorder in photonics. Nat. Rev. Mater. 6, 226–243 (2021).

    Article  ADS  Google Scholar 

Download references

Acknowledgements

This work was partially supported by the Defense Advanced Research Projects Agency (DARPA) and the Office of Naval Research (N00014-20-1-2789).

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Authors

Contributions

Both authors developed the idea and prepared the manuscript. Z.S. conducted the numerical calculations and A.D. supervised the project.

Corresponding author

Correspondence to A. Dogariu.

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The authors declare no competing interests.

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Nature Photonics thanks Jean-Jacques Greffet and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.

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Supplementary information

Supplementary Information

Supplementary Figs. 1–5 and discussions.

Supplementary Video 1

The concept of coupled scatterers illuminated by Dirac δ pulse.

Supplementary Video 2

The concept of coupled scatterers illuminated by Heaviside H pulse.

Supplementary Video 3

The intensity dynamics for spherical random media (mean distance: 2.4λ, media radius: 7.5λ) illuminated by δ pulse.

Supplementary Video 4

The intensity dynamics for spherical random media (mean distance: 1.2λ, media radius: 3.8λ) illuminated by δ pulse.

Supplementary Video 5

The intensity dynamics for spherical random media (mean distance: 0.3λ, media radius: 0.9λ) illuminated by δ pulse.

Supplementary Video 6

The intensity dynamics for spherical random media (mean distance: 2.4λ, media radius: 7.5λ) illuminated by H pulse.

Supplementary Video 7

The intensity dynamics for spherical random media (mean distance: 1.2λ, media radius: 3.8λ) illuminated by H pulse.

Supplementary Video 8

The intensity dynamics for spherical random media (mean distance: 0.3λ, media radius: 0.9λ) illuminated by H pulse.

Supplementary Video 9

The intensity dynamics for spherical random media (mean distance: 0.6λ, media radius: 3.8λ) illuminated by δ pulse.

Supplementary Video 10

The intensity dynamics for spherical random media (mean distance: 0.3λ, media radius: 3.8λ) illuminated by δ pulse.

Supplementary Video 11

The intensity dynamics for spherical random media (mean distance: 0.6λ, media radius: 3.8λ) illuminated by H pulse.

Supplementary Video 12

The intensity dynamics for spherical random media (mean distance: 0.3λ, media radius: 3.8λ) illuminated by H pulse.

Supplementary Video 13

The intensity dynamics for cylindrical random media (mean distance: 0.3λ) illuminated by δ pulse (incidence angle: 45 deg).

Supplementary Video 14

The intensity dynamics for cylindrical random media (mean distance: 0.3λ) illuminated by H pulse (incidence angle: 45 deg).

Supplementary Video 15

The energy storage for spherical random media (mean distance: 0.6λ, media radius: 3.8λ) illuminated by δ pulse.

Supplementary Video 16

The energy storage for spherical random media (mean distance: 0.3λ, media radius: 3.8λ) illuminated by δ pulse.

Supplementary Video 17

The energy storage for spherical random media (mean distance: 0.6λ, media radius: 3.8λ) illuminated by H pulse.

Supplementary Video 18

The energy storage for spherical random media (mean distance: 0.3λ, media radius: 3.8λ) illuminated by H pulse.

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Shen, Z., Dogariu, A. Subradiant directional memory in cooperative scattering. Nat. Photon. 16, 148–153 (2022). https://doi.org/10.1038/s41566-021-00926-4

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