Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • Letter
  • Published:

Single-shot measurement of few-cycle optical waveforms on a chip

Abstract

The measurement of transient optical fields has proven critical to understanding the dynamical mechanisms underlying ultrafast physical and chemical phenomena, and is key to realizing higher speeds in electronics and telecommunications. However, complete characterization of optical waveforms requires an ‘optical oscilloscope’ capable of resolving the electric-field oscillations with sub-femtosecond resolution and with single-shot operation. Here we show that strong-field nonlinear excitation of photocurrents in a silicon-based image sensor chip can provide the sub-cycle optical gate necessary to characterize carrier-envelope phase-stable optical waveforms in the mid-infrared. By mapping the temporal delay between an intense excitation and weak perturbing pulse onto a transverse spatial coordinate of the image sensor, we show that the technique allows single-shot measurement of few-cycle waveforms.

This is a preview of subscription content, access via your institution

Access options

Buy this article

Prices may be subject to local taxes which are calculated during checkout

Fig. 1: Experimental set-up and principle of single-shot measurement.
Fig. 2: Single-image characterization of a few-cycle pulse.
Fig. 3: Determination of the carrier-envelope phase.
Fig. 4: Complete characterization of laser waveforms.

Similar content being viewed by others

Data availability

The data that supports the plots within this paper and other findings of this study are available at https://stars.library.ucf.edu/cgi/preview.cgi?article=1001&context=datasets.

Code availability

The codes that produced the modelled data within this paper and other findings of this study are available at https://stars.library.ucf.edu/cgi/preview.cgi?article=1001&context=datasets.

References

  1. Chini, M., Zhao, K. & Chang, Z. The generation, characterization and applications of broadband isolated attosecond pulses. Nat. Photon. 8, 178–186 (2014).

    Article  ADS  Google Scholar 

  2. Alismail, A. et al. Near-infrared molecular fieldoscopy of water. Proc. SPIE 10882, 1088231 (2019).

    Google Scholar 

  3. Sederberg, S. et al. Attosecond optoelectronic field measurement in solids. Nat. Commun. 11, 430 (2020).

    Article  ADS  Google Scholar 

  4. Pupeza, I. et al. Field-resolved infrared spectroscopy of biological systems. Nature 577, 52–59 (2020).

    Article  ADS  Google Scholar 

  5. Fattahi, H., Fattahi, Z. & Ghorbani, A. Prospects of third-generation femtosecond laser technology in biological spectromicroscopy. J. Opt. 20, 054005 (2018).

    Article  ADS  Google Scholar 

  6. Paulus, G. G. et al. Measurement of the phase of few-cycle laser pulses. Phys. Rev. Lett. 91, 253004 (2003).

    Article  ADS  Google Scholar 

  7. Goulielmakis, E. et al. Direct measurement of light waves. Science 305, 1267–1269 (2004).

    Article  ADS  Google Scholar 

  8. Zimin, D. et al. Petahertz-scale nonlinear photoconductive sampling in air. Optica 8, 586–590 (2021).

    Article  ADS  Google Scholar 

  9. Wu, Q. & Zhang, X.-C. Free-space electro-optic sampling of terahertz beams. Appl. Phys. Lett. 67, 3523–3525 (1995).

    Article  ADS  Google Scholar 

  10. Keiber, S. et al. Electro-optic sampling of near-infrared waveforms. Nat. Photon. 10, 159–162 (2016).

    Article  ADS  Google Scholar 

  11. Park, S. B. et al. Direct sampling of a light wave in air. Optica 5, 402–408 (2018).

    Article  ADS  Google Scholar 

  12. Ratner, J., Steinmeyer, G., Wong, T. C., Bartels, R. & Trebino, R. Coherent artifact in modern pulse measurements. Opt. Lett. 37, 2874–2876 (2012).

    Article  ADS  Google Scholar 

  13. Wyatt, A. S. et al. Attosecond sampling of arbitrary optical waveforms. Optica 3, 303–310 (2016).

    Article  ADS  Google Scholar 

  14. Liu, Y. et al. All-optical sampling of few-cycle infrared pulses using tunneling in a solid. Photon. Res. 9, 929–936 (2021).

    Article  Google Scholar 

  15. Trebino, R. et al. Measuring ultrashort laser pulses in the time-frequency domain using frequency-resolved optical gating. Rev. Sci. Instrum. 68, 3277–3295 (1997).

    Article  ADS  Google Scholar 

  16. Iaconis, C. & Walmsley, I. A. Spectral phase interferometry for direct electric-field reconstruction of ultrashort optical pulses. Opt. Lett. 23, 792–794 (1998).

    Article  ADS  Google Scholar 

  17. Kane, D. J., Taylor, A. J., Trebino, R. & DeLong, K. W. Single-shot measurement of the intensity and phase of a femtosecond UV laser pulse with frequency-resolved optical gating. Opt. Lett. 19, 1061–1063 (1994).

    Article  ADS  Google Scholar 

  18. Briggman, K. A., Richter, L. J. & Stephenson, J. C. Imaging and autocorrelation of ultrafast infrared laser pulses in the 3–11-μm range with silicon CCD cameras and photodiodes. Opt. Lett. 26, 238–240 (2001).

    Article  ADS  Google Scholar 

  19. Hammond, T. et al. Near-field imaging for single-shot waveform measurements. J. Phys. B 51, 065603 (2018).

    Article  ADS  Google Scholar 

  20. Hemmer, M., Baudisch, M., Thai, A., Couairon, A. & Biegert, J. Self-compression to sub-3-cycle duration of mid-infrared optical pulses in dielectrics. Opt. Express 21, 28095–28102 (2013).

    Article  ADS  Google Scholar 

  21. Gholam-Mirzaei, S., Beetar, J. E., Chacón, A. & Chini, M. High-harmonic generation in ZnO driven by selfcompressed mid-infrared pulses. J. Opt. Soc. Am. B 35, A27–A31 (2018).

    Article  ADS  Google Scholar 

  22. Lu, F. et al. Generation of sub-two-cycle CEP-stable optical pulses at 3.5 µm from a KTA-based optical parametric amplifier with multiple-plate compression. Opt. Lett. 43, 2720–2723 (2018).

    Article  ADS  Google Scholar 

  23. Malitson, I. H. A redetermination of some optical properties of calcium fluoride. Appl. Opt. 2, 1103–1107 (1963).

    Article  ADS  Google Scholar 

  24. Brabec, T. & Krausz, F. Intense few-cycle laser fields: frontiers of nonlinear optics. Rev. Mod. Phys. 72, 545–591 (2000).

    Article  ADS  Google Scholar 

  25. Ghafur, O. et al. Impulsive orientation and alignment of quantum-state-selected NO molecules. Nat. Phys. 5, 289–293 (2009).

    Article  Google Scholar 

  26. Long, J. P., Varadaraajan, S., Matthews, J. & Schetzina, J. F. UV detectors and focal plane array imagers based on AlGaN p-i-n photodiodes. Opto Electron. Rev. 10, 251–260 (2002).

    Google Scholar 

  27. Thiré, N. et al. 4-W, 100-kHz, few-cycle mid-infrared source with sub-100-mrad carrier-envelope phase noise. Opt. Express 25, 1505–1514 (2017).

    Article  ADS  Google Scholar 

Download references

Acknowledgements

This material is based primarily on research supported by the Air Force Office of Scientific Research under award no. FA9550-20-1-0284. S.G.-M. was supported by the Army Research Office under award no. W911NF-19-1-0211. We thank Z. Chang for helpful discussions and for loaning the PbSe spectrometer used to measure the mid-infrared spectra.

Author information

Authors and Affiliations

Authors

Contributions

M.C. had the idea for the single-shot waveform measurement scheme and oversaw the research team. Y.L. led the experimental effort and performed most of the measurements and simulations. J.E.B. assisted with the measurements of the carrier-envelope phase dependence. J.N. and S.G.-M. assisted with the construction of the experimental set-up and with the data collection. All authors contributed to data analysis and the creation of the manuscript.

Corresponding author

Correspondence to Michael Chini.

Ethics declarations

Competing interests

The authors declare no competing interests.

Additional information

Peer review information Nature Photonics thanks Nicholas Karpowicz, Gerhard Paulus and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.

Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Supplementary information

Supplementary Information

Supplementary Notes 1–5, Figs. 1–14 and Table 1.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Liu, Y., Beetar, J.E., Nesper, J. et al. Single-shot measurement of few-cycle optical waveforms on a chip. Nat. Photon. 16, 109–112 (2022). https://doi.org/10.1038/s41566-021-00924-6

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1038/s41566-021-00924-6

This article is cited by

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing