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Fast thermal relaxation in cavity-coupled graphene bolometers with a Johnson noise read-out

Abstract

High sensitivity, fast response time and strong light absorption are the most important metrics for infrared sensing and imaging. The trade-off between these characteristics remains the primary challenge in bolometry. Graphene with its unique combination of a record small electronic heat capacity and a weak electron–phonon coupling has emerged as a sensitive bolometric medium that allows for high intrinsic bandwidths13. Moreover, the material’s light absorption can be enhanced to near unity by integration into photonic structures. Here, we introduce an integrated hot-electron bolometer based on Johnson noise readout of electrons in ultra-clean hexagonal-boron-nitride-encapsulated graphene, which is critically coupled to incident radiation through a photonic nanocavity with Q = 900. The device operates at telecom wavelengths and shows an enhanced bolometric response at charge neutrality. At 5 K, we obtain a noise equivalent power of about 10 pW Hz1/2, a record fast thermal relaxation time, <35 ps, and an improved light absorption. However the device can operate even above 300 K with reduced sensitivity. We work out the performance mechanisms and limits of the graphene bolometer and give important insights towards the potential development of practical applications.

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Fig. 1: Device schematics and operation principle.
Fig. 2: Role of the PCC in enhancement of the bolometric response.
Fig. 3: Bolometric response.
Fig. 4: Detector performance.

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References

  1. Fong, K. C. & Schwab, K. C. Ultrasensitive and wide-bandwidth thermal measurements of graphene at low temperatures. Phys. Rev. X 2, 031006 (2012).

    Google Scholar 

  2. McKitterick, C. B., Prober, D. E. & Karasik, B. S. Performance of graphene thermal photon detectors. J. Appl. Phys. 113, 044512 (2013).

    Article  Google Scholar 

  3. Yan, J. et al. Dual-gated bilayer graphene hot-electron bolometer. Nat. Nanotech. 7, 472–478 (2012).

    Article  Google Scholar 

  4. Balandin, A. A. Thermal properties of graphene and nanostructured carbon materials. Nat. Mater. 10, 569–581 (2011).

    Article  Google Scholar 

  5. Fong, K. C. et al. Measurement of the electronic thermal conductance channels and heat capacity of graphene at lowtemperature. Phys. Rev. X 3, 041008 (2013).

    Google Scholar 

  6. Crossno, J. et al. Observation of the Dirac fluid and the breakdown of the Wiedemann–Franz law in graphene. Science 351, 1058–1061 (2016).

    Article  Google Scholar 

  7. Mak, K. F. et al. Measurement of the optical conductivity of graphene. Phys. Rev. Lett. 101, 196405 (2008).

    Article  Google Scholar 

  8. Walsh, E. D. et al. Graphene-based Josephson-junction single-photon detector. Phys. Rev. Appl. 8, 024022 (2017).

    Article  Google Scholar 

  9. Du, X., Prober, D. E., Vora, H. & Mckitterick, C. B. Graphene-based bolometers. Graphene 2D Mater. 1, 1–22 (2014).

    Google Scholar 

  10. Vora, H., Kumaravadivel, P., Nielsen, B. & Du, X. Bolometric response in graphene based superconducting tunnel junctions. Appl. Phys. Lett. 100, 153507 (2012).

    Article  Google Scholar 

  11. Cai, X. et al. Sensitive room-temperature terahertz detection via the photothermoelectric effect in graphene. Nat. Nanotech. 9, 814–819 (2014).

    Article  Google Scholar 

  12. Han, Q. et al. Highly sensitive hot electron bolometer based on disordered graphene. Sci. Rep. 3, 3533 (2013).

    Article  Google Scholar 

  13. El Fatimy, A. et al. Epitaxial graphene quantum dots for high-performance terahertz bolometers. Nat. Nanotech. 11, 335–338 (2016).

    Article  Google Scholar 

  14. Nair, R. R. et al. Fine structure constant defines visual transparency of graphene. Science 320, 1308 (2008).

    Article  Google Scholar 

  15. Li, Z. Q. et al. Dirac charge dynamics in graphene by infrared spectroscopy. Nat. Phys. 4, 532–535 (2008).

    Article  Google Scholar 

  16. McKitterick, C. B., Prober, D. E. & Rooks, M. J. Electron-phonon cooling in large monolayer graphene devices. Phys. Rev. B Condens. Matter 93, 075410 (2016).

    Article  Google Scholar 

  17. Dean, C. R. et al. Boron nitride substrates for high-quality graphene electronics. Nat. Nanotech. 5, 722–726 (2010).

    Article  Google Scholar 

  18. Gan, X. et al. Strong enhancement of light–matter interaction in graphene coupled to a photonic crystal nanocavity. Nano Lett. 12, 5626–5631 (2012).

    Article  Google Scholar 

  19. Bao, Q. & Loh, K. P. Graphene photonics, plasmonics, and broadband optoelectronic devices. ACS Nano 6, 3677–3694 (2012).

    Article  Google Scholar 

  20. Gabor, N. M. et al. Hot carrier–assisted intrinsic photoresponse in graphene. Science 334, 648–652 (2011).

    Article  Google Scholar 

  21. Gao, Y. et al. High-speed electro-optic modulator integrated with graphene-boron nitride heterostructure and photonic crystal nanocavity. Nano Lett. 15, 2001–2005 (2015).

    Article  Google Scholar 

  22. Shiue, R.-J. et al. Enhanced photodetection in graphene-integrated photonic crystal cavity. Appl. Phys. Lett. 103, 241109 (2013).

    Article  Google Scholar 

  23. Takano, H., Song, B. S., Asano, T. & Noda, S. Highly efficient multi-channel drop filter in a two-dimensional hetero photonic crystal. Opt. Express 14, 3491–3496 (2006).

    Article  Google Scholar 

  24. Zheng, J., Barton, R. A. & Englund, D. Broadband coherent absorption in chirped-planar-dielectric cavities for 2D-material-based photovoltaics and photodetectors. ACS Photonics 1, 768–774 (2014).

    Article  Google Scholar 

  25. Piper, J. R. & Fan, S. Total absorption in a graphene monolayer in the optical regime by critical coupling with a photonic crystal guided resonance. ACS Photonics 1, 347–353 (2014).

    Article  Google Scholar 

  26. Marini, A., Cox, J. D. & de Abajo, F. J. G. Theory of graphene saturable absorption. Phys. Rev. B 95, 125408 (2017).

    Article  Google Scholar 

  27. Tielrooij, K. J. et al. Generation of photovoltage in graphene on a femtosecond timescale through efficient carrier heating. Nat. Nanotech. 10, 437–443 (2015).

    Article  Google Scholar 

  28. Graham, M. W., Shi, S.-F., Ralph, D. C., Park, J. & McEuen, P. L. Photocurrent measurements of supercollision cooling in graphene. Nat. Phys. 9, 103–108 (2012).

    Article  Google Scholar 

  29. Shiue, R.-J. et al. High-responsivity graphene–boron nitride photodetector and autocorrelator in a silicon photonic integrated circuit. Nano Lett. 15, 7288–7293 (2015).

    Article  Google Scholar 

  30. Tielrooij, K. J. et al. Out-of-plane heat transfer in van der Waals stacks: electron–hyperbolic phonon coupling. Nat. Nanotech. 13, 41–46 (2018).

    Article  Google Scholar 

  31. Sun, D. et al. Ultrafast hot-carrier-dominated photocurrent in graphene. Nat. Nanotech. 7, 114–118 (2012).

    Article  Google Scholar 

  32. Tielrooij, K.-J. et al. Out-of-plane heat transfer in van der Waals stacks through electron–hyperbolic phonon coupling. Nat. Nanotech. 13, 41–46 (2018).

    Article  Google Scholar 

  33. Dicke, R. H. The measurement of thermal radiation at microwave frequencies. Rev. Sci. Instrum. 17, 268–275 (1946).

    Article  Google Scholar 

Download references

Acknowledgements

We thank L. Levitov, D. Prober, P. Kim and F. Koppens for fruitful discussions. D.K.E. acknowledges support from the Ministry of Economy and Competitiveness of Spain through the Severo Ochoa programme for Centres of Excellence in R&D (SEV-2015-0522), Fundació Privada Cellex, Fundació Privada Mir-Puig, the Generalitat de Catalunya through the CERCA program and the La Caixa Foundation. D.E. acknowledges support from the Office of Naval Research under grant no. N00014-14-1-0349. Y.G., C.T. and J.H. acknowledge support from the US Office of Naval Research, grant N00014-13-1-0662. K.C.F. acknowledges support from Raytheon BBN Technologies. B.S. was supported as part of the MIT Center for Excitonics, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Basic Energy Sciences under award no. DE-SC0001088. J.Z. carried out research in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the US Department of Energy, Office of Basic Energy Sciences, under contract no. DE-SC0012704. This work is supported in part by the Semiconductor Research Corporation’s NRI Center for Institute for Nanoelectronics Discovery and Exploration (INDEX).

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D.K.E., K.C.F. and D.E. conceived and designed the experiments. D.K.E. and R.-J.S. performed the experiments. D.K.E. analysed the data. B.S. performed the theoretical modelling of the data. Y.G., C.T., C.P., H.C., E.D.W., J.Z. and G.G. contributed materials/analysis tools. J.H., K.C.F. and D.E. supported the experiments. D.K.E. wrote the paper.

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Correspondence to Dmitri K. Efetov.

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Efetov, D.K., Shiue, RJ., Gao, Y. et al. Fast thermal relaxation in cavity-coupled graphene bolometers with a Johnson noise read-out. Nature Nanotech 13, 797–801 (2018). https://doi.org/10.1038/s41565-018-0169-0

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