New classes of functional soft materials show promise to revolutionize robotics. Now materials scientists must focus on realizing the predicted performance of these materials and developing effective and robust interfaces to integrate them into highly functional robotic systems that have a positive impact on human life.
This is a preview of subscription content, access via your institution
Access options
Subscribe to Nature+
Get immediate online access to Nature and 55 other Nature journal
$29.99
monthly
Subscribe to Journal
Get full journal access for 1 year
$119.00
only $9.92 per issue
All prices are NET prices.
VAT will be added later in the checkout.
Tax calculation will be finalised during checkout.
Buy article
Get time limited or full article access on ReadCube.
$32.00
All prices are NET prices.



References
Haines, C. S. et al. Science 343, 868–872 (2014).
Hu, W., Lum, G. Z., Mastrangeli, M. & Sitti, M. Nature 554, 81–85 (2018).
Ilievski, F., Mazzeo, A. D., Shepherd, R. F., Chen, X. & Whitesides, G. M. Angew. Chem. Int. Ed. 50, 1890–1895 (2011).
Shintake, J., Rosset, S., Schubert, B., Floreano, D. & Shea, H. Adv. Mater. 28, 231–238 (2016).
Rothemund, P. et al. Sci. Robot. 3, eaar7986 (2018).
Wehner, M. et al. Nature 536, 451–455 (2016).
Vantomme, G. et al. Nat. Mater. https://doi.org/10.1038/s41563-021-00931-6 (2021).
Kim, Y., Parada, G. A., Liu, S. & Zhao, X. Sci. Robot. 4, eaax7329 (2019).
Hawkes, E. W., Majidi, C. & Tolley, M. T. Sci. Robot. 6, eabg6049 (2021).
Acome, E. et al. Science 359, 61–65 (2018).
Kim, Y., Yuk, H., Zhao, R., Chester, S. A. & Zhao, X. Nature 558, 274–279 (2018).
Ohm, C., Brehmer, M. & Zentel, R. Adv. Mater. 22, 3366–3387 (2010).
Kellaris, N., Gopaluni Venkata, V., Smith, G. M., Mitchell, S. K. & Keplinger, C. Sci. Robot. 3, eaar3276 (2018).
Rothemund, P., Kellaris, N., Mitchell, S. K., Acome, E. & Keplinger, C. Adv. Mater. 33, 2003375 (2021).
Kellaris, N., Venkata, V. G., Rothemund, P. & Keplinger, C. Extrem. Mech. Lett. 29, 100449 (2019).
Xu, T., Zhang, J., Salehizadeh, M., Onaizah, O. & Diller, E. Sci. Robot. 4, eaav4494 (2019).
Zhang, J. et al. Sci. Robot. 6, eabf0112 (2021).
Xu, P. A. et al. Sci. Robot. 4, eaaw6304 (2019).
Kramer, R. K., Majidi, C. & Wood, R. J. In 2011 IEEE International Conference on Robotics and Automation 1103–1107 https://doi.org/10.1109/ICRA.2011.5980082 (IEEE, 2011).
Lipomi, D. J. et al. Nat. Nanotechnol. 6, 788–792 (2011).
Sun, J.-Y., Keplinger, C., Whitesides, G. M. & Suo, Z. Adv. Mater. 26, 7608–7614 (2014).
Kaltenbrunner, M. et al. Nature 499, 458–463 (2013).
Kim, D.-H. et al. Science 333, 838–843 (2011).
Van Meerbeek, I. M., De Sa, C. M. & Shepherd, R. F. Sci. Robot. 3, eaau2489 (2018).
Bai, H. et al. Science 370, 848–852 (2020).
Aubin, C. A. et al. Nature 571, 51–57 (2019).
Drotman, D., Jadhav, S., Sharp, D., Chan, C. & Tolley, M. T. Sci. Robot. 6, eaay2627 (2021).
Aubin, C. et al. Nature (in the press).
Kim, Y., van den Berg, J. & Crosby, A. J. Nat. Mater. https://doi.org/10.1038/s41563-020-00909-w (2021).
Peng, Y. et al. Nat. Mater. https://doi.org/10.1038/s41563-021-00990-9 (2021).
Kang, B. B., Choi, H., Lee, H. & Cho, K.-J. Soft Robot. 6, 214–227 (2019).
Kim, J. et al. Science 365, 668–672 (2019).
Roche, E. T. et al. Sci. Transl. Med. 9, eaaf3925 (2017).
Park, S. et al. Nat. Commun. 12, 3435 (2021).
Yuk, H., Lu, B. & Zhao, X. Chem. Soc. Rev. 48, 1642–1667 (2019).
Yang, J., Bai, R., Chen, B. & Suo, Z. Adv. Funct. Mater. 30, 1901693 (2020).
Zhao, X. et al. Chem. Rev. 121, 4309–4372 (2021).
Yuk, H., Zhang, T., Lin, S., Parada, G. A. & Zhao, X. Nat. Mater. 15, 190–196 (2016).
Bartlett, N. W. et al. Science 349, 161–165 (2015).
Keplinger, C. et al. Science 341, 984–987 (2013).
Acknowledgements
P.R. and C.K. acknowledge funding by the Max Planck Society, Germany. Y.K. acknowledges funding through scholarships from ILJU Academy and Culture Foundation and MIT School of Engineering MathWorks Fellowship. X.Z. acknowledges funding from the National Institutes of Health (no. 1R01HL153857-01) and the National Science Foundation (no. EFRI-1935291).
Author information
Authors and Affiliations
Contributions
C.K. developed the concept of the article. P.R. and C.K. led and coordinated the writing of the article. All authors contributed to the content and writing of the article.
Corresponding author
Ethics declarations
Competing interests
P.R. and C.K. are listed as inventors of patents that cover fundamentals and basic designs of HASEL actuators as well as methods of fabrication. Y.K. and X.Z. are listed as inventors of patents that cover fundamental principles and fabrication techniques for 3D-printed magnetic soft actuators and magnetically steerable soft continuum robots. X.Z. is a co-founder of SanaHeal Inc., a start-up company commercializing bioadhesives. R.F.S. is listed as an inventor for patents regarding stretchable lightguide-based optical sensing platforms, and is a co-founder of Organic Robotics Corporation, which licenses these patents. C.K. is a co-founder of Artimus Robotics, a start-up company commercializing HASEL actuators.
Additional information
Peer review information Nature Materials thanks the anonymous reviewers for their contribution to the peer review of this work.
Rights and permissions
About this article
Cite this article
Rothemund, P., Kim, Y., Heisser, R.H. et al. Shaping the future of robotics through materials innovation. Nat. Mater. 20, 1582–1587 (2021). https://doi.org/10.1038/s41563-021-01158-1
Published:
Issue Date:
DOI: https://doi.org/10.1038/s41563-021-01158-1