Review Article | Published:

Opportunities and challenges for tandem solar cells using metal halide perovskite semiconductors

Nature Energyvolume 3pages828838 (2018) | Download Citation

Abstract

Metal halide perovskite semiconductors possess excellent optoelectronic properties, allowing them to reach high solar cell performances. They have tunable bandgaps and can be rapidly and cheaply deposited from low-cost precursors, making them ideal candidate materials for tandem solar cells, either by using perovskites as the wide-bandgap top cell paired with low-bandgap silicon or copper indium diselenide bottom cells or by using both wide- and small-bandgap perovskite semiconductors to make all-perovskite tandem solar cells. This Review highlights the unique potential of perovskite tandem solar cells to reach solar-to-electricity conversion efficiencies far above those of single-junction solar cells at low costs. We discuss the recent developments in perovskite-based tandem fabrication, and detail directions for future research to take this technology beyond the proof-of-concept stage.

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Acknowledgements

We thank Department of Energy (DOE) SunShot and Office of Naval Research (ONR) for funding. T.L. is supported by a Marie Curie fellowship under Horizon 2020, and K.A.B. is supported by a National Science Foundation (NSF) fellowship.

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    • Tomas Leijtens

    Present address: Materials Science Center, National Renewable Energy Laboratory, Golden, CO, USA

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  1. Materials Science and Engineering, Stanford University, Stanford, CA, USA

    • Tomas Leijtens
    • , Kevin A. Bush
    • , Rohit Prasanna
    •  & Michael D. McGehee

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Correspondence to Tomas Leijtens or Michael D. McGehee.

Supplementary information

  1. Supplementary Tables 1–2

    Supplementary Table 1 provides the bandgap, open-circuit voltage, power conversion efficiency and reference for the data points in Fig. 1c. Supplementary Table 2 provides the bandgap, open-circuit voltage, power conversion efficiency and reference for each data point in Fig. 2b

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https://doi.org/10.1038/s41560-018-0190-4