Abstract
Supertoroidal light pulses, as spacetime nonseparable electromagnetic waves, exhibit unique topological properties including skyrmionic configurations, fractallike singularities, and energy backflow in free space, which however do not survive upon propagation. Here, we introduce the nondiffracting supertoroidal pulses (NDSTPs) with propagationrobust skyrmionic and vortex field configurations that persists over arbitrary propagation distances. Intriguingly, the field structure of NDSTPs has a similarity with the von Kármán vortex street, a pattern of swirling vortices in fluid and gas dynamics with staggered singularities that can stably propagate forward. NDSTPs will be of interest as directed channels for information and energy transfer applications.
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Introduction
The topological properties of light have been a subject of fascination and intense research interest over the last half century^{1,2,3} with implications for lightmatter interactions^{4,5,6}, nonlinear physics^{7,8,9}, spinorbit coupling^{10,11,12}, microscopy and imaging^{13,14,15}, metrology^{16}, and information transfer^{17,18,19,20,21,22}. Light pulses can be simultaneously structured in the space and time domains^{23,24,25}. Threedimensional topological structures have also been studied recently, such as the toroidal phase vortices in scalar light pulses^{26,27,28} and the photonic skyrmions and hopfions with particlelike topologies in vector beams^{29,30,31}. As a special type of topologically structured light with both ultrafast temporal and vectorial electromagnetic configurations, the toroidal light pulses are of particular interest^{32}, as they can engage toroidal excitations in matter^{33,34} and exhibit spacetime nonseparability and isodiffraction^{35,36,37}. A generalization of toroidal pulses, the supertoroidal pulses (STPs) exhibit striking topology including fractallike singularities, vortex rings, energy backflows, and optical skyrmionic patterns^{38,39}. To date, all known electromagnetic analogs of skyrmions are shortlived and do not persist upon propagation.
In this Letter, we introduce the nondiffracting supertoroidal pulses (NDSTPs), an extended family of STPs that propagate without diffraction. NDSTPs exhibit the topological properties of STPs, such as energy backflow, fractal organization of singularities, and skyrmionlike field configurations. In contrast to previously considered forms of skyrmionic light, typically observed in the steady state^{40,41,42}, NDSTPs exhibit spatiotemporal topological features that persist upon propagation. Intriguingly, the structure of an NDSTP resembles that of Kármán vortex street (KVS), propagating staggered vortex arrays observed in fluid and gas dynamics^{43}, previously observed in continuouswave structured light fields^{44,45,46,47}.
Results
Nondiffracting supertoroidal pulses
(ND)STPs originate from the “electromagnetic directedenergy pulse trains” (EDEPTs) theory introduced by Ziolkowski to obtain focused fewcycle electromagnetic pulses that are localized finiteenergy and spacetime nonseparable solutions of Maxwell’s equations^{48}. As such, NDSTPs are also finite energy spacetime nonseparable pulses. The first step is finding a scalar generating function f(r, t) that satisfies Helmholtz’s scalar wave equation:
where r = (r, θ, z) represents the position vector (in a cylindrical coordinate system), t is time, \(c=1/\sqrt{\varepsilon \mu }\) is the speed of light, and the ε and μ are the permittivity and permeability of medium. Here, we consider propagation in freespace and thus permittivity and permeability are set to their vacuum values. The exact solution of f(r, t) can be given by the modified power spectrum method proposed by Ziolkowski^{48,49}:
where f_{0} is a normalizing constant, where s = r^{2}/(q_{1} + iτ) − iσ, τ = z − ct, σ = z + ct, q_{1}, q_{2}, q_{3} are real positive parameters with units of length, and the real dimensionless parameter α must satisfy α≥1. The parameter α controls the energy confinement at focus and spatial divergence of the pulse. In particular, the pulse carries infinite energy when α < 1, the pulse has localized finite energy when α ≥ 1, and with increasing α the pulse becomes more divergent upon propagation, therefore the value of parameter α is usually fixed at unity to ensure finite energy of the pulse^{48,50}. In order to retrieve the toroidal electromagnetic fields, we construct the Hertz potential as \({{{{{{{\bf{\Pi }}}}}}}}={{{{{{{\boldsymbol{\nabla }}}}}}}}\times \hat{{{{{{{{\bf{z}}}}}}}}}f({{{{{{{\bf{r}}}}}}}},t)\), then the fields of transverse electric (TE) mode, i.e. the electric field is azimuthal (E_{θ}) and the magnetic field is nontransverse (including H_{r} and H_{z} components), can be solved by^{50} (see Supplementary Note 1 for more detailed derivations):
For the previous solution of supertoroidal pulses (q_{3} = ∞), q_{1} is the effective wavelength as a constant proportional to the central wavelength λ of the pulse (q_{1} ≈ 0.24 λ), q_{2} is related to the Rayleigh length (q_{2} = z_{0}/2) describing the spatial divergence along longitudinal direction^{39}. While, when q_{3} takes finite values, it quantifies the spatial divergence along the transverse direction of the structured pulse at focus, which refers to the distance from the pulse center along the transverse direction where the amplitude profile becomes bifurcate. At the same time, the longitudinal divergence of the pulse has a trend to be weakened becomes weaker and it is, no longer described by q_{2}, while the pulse becomes nondiffracting.
A representative elementary toroidal light pulse is shown in Fig. 1a. The transverse magnetic (TM) mode can be obtained by exchanging electric and magnetic fields of the TE mode. In prior works, the conditions q_{1} ≪ q_{2}, α = 1, and q_{3} → ∞ were assumed to generate various focused structured pulses^{50,51,52,53,54}, where q_{1} and q_{2} determine the wavelength and the longitudinal divergence or Rayleigh length of the pulses, respectively, as marked in Fig. 1a. The condition q_{2} ≫ q_{1} allows to avoid pathologies related to the presence of backward propagating components^{55,56}. The case of α ≥ 1 and q_{3} → ∞ was recently studied leading to the introduction of supertoroidal pulses^{39}. However, the solutions with finite values of q_{3} have never been studied before. In this work, we explore STPs with finite q_{3} (see Supplementary Note 1 for derivations). A characteristic example of such a pulse with q_{3} = q_{1} and α = 1 is plotted in Fig. 1b. Here, q_{3} defines the degree of transverse divergence: with decreasing value of q_{3} the pulse envelope is gradually squeezed into a dumbbelllike shape and eventually becomes nondiffracting for q_{3} = q_{1} and α = 1, approaching the case of nondiffraction ∣E(r, θ, z, t)∣ = ∣E(r, θ, z + Δz, t + Δz/v)∣ (Δz is a given propagation distance and v is group velocity)^{57}, see Supplementary Note 2. Note that, exact nondiffracting waves like ideal Bessel beams or plane waves only exist in theory and cannot be realized experimentally as practical light pulses would carry infinite energy. Here, we use the term “nondiffracting” to describe finite energy waves that propagate without diffraction over very large (but finite) distances.
The evolution of the pulse from diffracting to nondiffracting is illustrated in Fig. 2. An intermediate case of a weaklydiffracting supertoroidal pulse in terms of q_{1}, q_{2}, and q_{3}, is presented Fig. 2a. To illustrate the dependence of the (non)diffraction of the pulse on q_{3}, we calculate the zdependent full width at half maximum (FWHM) radius of the transverse intensity pattern of the STPs with q_{2} = 100q_{1} and q_{3} varying from infinity to q_{1}, for propagation distances from focus to z = 10^{3}q_{1}, see Fig. 2b. In the extreme case of q_{3} → ∞ (fundamental toroidal light pulse), the FWHM of the pulse follows a hyperbolic trajectory similar to a focused Gaussian beam. With decreasing q_{3}, the divergence becomes weaker and the pulse approaches a nondiffracting state for q_{3} ≤ 5q_{1}. Figure 2c–f shows the spatiotemporal evolution upon propagation for toroidal pulses with different q_{3} values. Here, decreasing q_{3} results in a faster spatiotemporal evolution of the cycle structure of the pulse (see Supplementary Movie 1), due to its increasingly complex shape. When the q_{3} value is decreased further to q_{1}, the pulse becomes Xshaped (Fig. 1b), which reveals a conical structure. We note that q_{1} is independent of q_{3} and thus we would not expect a change in the former when the latter varies. The counterintuitive decrease in beam waist with a decrease in divergence angle can be attributed to the presence of “long thick wings” at the peripheral area of the pulse. Upon propagation, the cycle structure keeps evolving on the conical surface akin to a breather (see Supplementary Movie 1). Note that similar Xtype nondiffracting pulses have been considered previously both theoretically and experimentally and are typically termed BesselX pulses^{58,59,60}. However, previous works focused on scalar longpulses within the slowlyvarying amplitude envelope approximation. Here, our NDSTPs are fewcycle, spacetime nonseparable with nontrivial electromagnetic toroidal topology lacking in the BesselX pulses. Table 1 summarizes the parameter requirements for various cases of fundamental toroidal pulse, STP, NDSTP, and intermediate states.
Singularities and topological properties
The emergence of NDSTPs allows us to explore intriguing topological optical effects. In our recent work, we showed that supertoroidal pulses exhibit a complex topology (controlled by the parameter α), including selfsimilar fractallike patterns, matryoshkalike singularity arrays, skyrmions, and areas of energy backflow^{39}. Here, we show that such topological structures are also present in NDSTPs. However, whereas in the former case, the selfsimilar topological structures were only instantaneously observed at focus (within a region of length q_{2}), in the NDSTP, they can be observed over arbitrarily long distances (see example in Fig. 3b). For instance, we have shown in our previous work that STPs exhibit a complex topology that evolves rapidly upon pulse propagation with elements of selfsimilarity consisting of concentric matryoshkalike spherical shells over which the electric field vanishes (see Fig. 3a). Similar propagationrobust fractallike topological structures exist in the NDSTP (see Fig. 3b) and persist upon pulse propagation (see also Supplementary Movie 2).
The complex topology of the NDSTPs manifests also in the magnetic field distribution. Figure 4a shows the magnetic field distribution of a NDSTP with q_{2}/q_{1} = 100 and q_{3}/q_{1} = 1 at t = 0. The magnetic field includes both radial and longitudinal components resulting in vector singularities of vortex and saddle types. The saddletype singularities are distributed along the propagation axis, while the vortices trace an offaxis trajectory, see Fig. 4a1. Such a singularity distribution induces multiple electromagnetic skyrmions at transverse planes of the pulse, see Fig. 4a2. Particularly, the optical skyrmion texture holds deepsubwavelength features in its field vector reversal regions, for instance shown in the plot of absolute value of normalized H_{z} field as the insert of Fig. 4a2, where the first reversal region occurs within size of q_{1}/2 and the second of q_{2}/10 along the radial direction (evaluated by full width at half maximum). In contrast to the previous optical skyrmions in free space that do not propagate^{41,42} or only exist around focus and collapse rapidly upon propagation^{39}, here in the NDSTP, the skyrmions persist upon propagation with their topological texture exhibiting a periodic behaviour alternating between four different skyrmion types (combination of opposite two polarities and two helical angles), see Supplementary Movie 3 and Supplementary Note 3. The evolution of skyrmion or toroidal structures is coupled with the evolution of optical cycles due to the phase shift along the zaxis. There are only two cases with skyrmion numbers of ±1 that can be observed in the transverse plane, and the total skyrmion number is zero due to the symmetry of the pulse structure.
Figure 4b shows the Poynting vector field distribution of the NDSTP, which possesses layered energy forwardflow and backflow structures (Fig. 4b1). Interestingly, energy transport is mediated by the vortex arrays of the magnetic field. Vortices on the front half of the pulse act as energy sources, whereas the vortices in the rear half behave as sinks. In between sources and sinks, we observe areas of extended backflow. In areas of high intensity, energy flows primarily forward, ensuring the propagation of the pulse.
Optical analogy of Kármán Vortex Streets (KVS)
Moreover, we observe that the vortex arrays exhibited by the NDSTPs form a striking trail of twovortex clusters (with opposite circulations, namely a vortex dipole) propagating in a periodic staggered manner, evocative of the KVS structure. In fluid dynamics, a KVS is a classic pattern of swirling vortices caused by a nonlinear process of vortex shedding, which refers to the unsteady separation of the flow of fluid around blunt bodies. Vortexstreetlike optical fields were reported previously in stationary optical fields exhibiting phase vortex patterns^{44,45,46,47}. In contrast, here we observe KVSlike structures in propagating electromagnetic pulses in the linear regime. Due to the nondiffracting nature of NDSTPs, such structures persist upon propagation. In fluid dynamics, a KVS is a pattern of repeating swirling vortices constructed in the flow velocity field, whilst in our optical analogy, the KVS pattern is constructed by the electric or magnetic field of NDSTPs. Moreover, whereas KVS in fluid dynamics is a nonlinear phenomenon, here we show that similar effects can be observed in a linear system. The analogy between KVS in fluid flows and NDSTPs can be drawn further by considering for instance the motion of electrons along the vortex streets of a TM NDSTP or the propagation of supertoroidal pulses in nonlinear media. We note that KVS in fluid dynamics are typically 2D, while their optical analogs in NDSTPs comprise 3D sets of vortex rings, owing to the pulse cylindrical symmetry, see Fig. 5.
Discussion
NDSTPs are nonpathological propagating solutions to Maxwell’s equations, as demonstrated by the spacetime spectral analysis of Fig. 6a, b. Indeed, over 99% of the pulse energy is carried by forward propagating waves (Fig. 6a2, b2). In addition, according to the standard criterion of nondiffraction for spacetime wave packets^{23,24}, the STP spectrum has a broad distribution in the k_{z}ω plane that indicates diffractive propagation. On the other hand, the NDSTP spectrum is confined in a conical section by a plane perpendicular to k_{z}ω plane, which implies a close to uniform constant group velocity v_{g} = ∂ω/(∂k_{z}) = c (the slope of the plane) along the zaxis and thus diffraction is almost completely absent. We note that while exact nondiffracting behavior corresponds to an infinitely thin line, NDSTPs approximate such behaviour closely, see details in Supplementary Note 4.
The generation of NDSTPs will involve addressing two main challenges: (1) The ω − k spectrum is distributed along a thin line of a conic section on the light cone, in order to fulfill the nondiffraction criterion; (2) The ω − k spectrum should include a null region at the center (k_{r} = 0), induced by the cylindrical polarization and vector singularity of the pulse. The former challenge can be addressed by realizing that the NDSTP pulse has a simple spectral structure in ω − k space as indicated by Fig. 6. Indeed, recently, photonic crystal slabs (PCS) consisting of 2D hole arrays were used to control the ω − k spectrum of emitted light in order to generate spacetime bullet pulses^{61}. Cylindrically polarized light fields have been generated by PCS of specific symmetry groups^{62}. Hence, we argue that controlling the geometry and symmetry of PCS will allow to generate NDSTPs. Alternatively, the recent method of generating picosecondlevel 3D nondiffracting wavepackets using transformation optics can be considered^{63}. Such an approach would need to be extended to cover the broad bandwidth of NDSTPs and allow control of vector polarization.
Of particular importance here is the relation between the size of the generating metasurface (aperture) and the distance over which the generated pulses propagate without diffraction. Our numerical study shows that an aperture of 400λ is sufficient for nondiffracting propagation (within 1% of the pulse FWHM) over a distance of 10^{5}λ (see Supplementary Note 4). Moreover, in contrast to the wellknown Bessel beams, NDSTPs are finite energy solutions to Maxwell’s equations. Thus, we argue that the NDSTPs are less sensitive to the metasurface size and thus their practical implementations remain closer to their ideal form.
In conclusion, we demonstrate NDSTPs with robust topological field structures including fractallike singularities, skyrmions, vortex rings, and energy backflow. In contrast to prior studies, the topological features of NDSTPs can stably propagate over an arbitrarily long distance. Our results provide a playground for the study of the propagation dynamics of electromagnetic skyrmions, as well as their interactions with matter, in particular in complex media with nonlinearity, anisotropy, or chirality. Due to its propagationrobust topology, the NDSTP acts as a spectacular display of staggered electromagnetic vortex dipole arrays with stable propagation, evocative of the classic KVS. The optical KVSs in NDSTPs unveil intriguing analogies between fluid transport and the flow of energy in structured light. The robust topological structure of NDSTPs that remains invariant upon propagation could be used for longdistance information transfer encoded in the topological features of the pulses with implications for telecommunications, remote sensing, and LIDAR. The toroidal field configuration of NDSTPs could be of interest in the spectroscopy of toroidal excitations in matter^{33,64,65}. Finally, the deeply subwavelength singularities of NDSTPs can be employed for applications in metrology, where such topological features have been shown to lead to orders of magnitude improvement in precision and resolution^{15}.
Data availability
The data from this paper can be obtained from the University of Southampton ePrints research repository at https://doi.org/10.5258/SOTON/D3058.
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Acknowledgements
The authors acknowledge the supports of the Singapore Ministry of Education (MOE) (MOE2016T31006), the UKs Engineering and Physical Sciences Research Council (grant EP/M009122/1, Funder Id: 10.13039/501100000266), the European Research Council (Advanced grant FLEET786851, Funder Id: https://doi.org/10.13039/501100000781), and the Defense Advanced Research Projects Agency (DARPA) under the Nascent Light Matter Interactions program. Y.S. thanks the support of a start grant from Nanyang Technological University and Singapore MOE AcRF Tier 1 grant (RG157/23).
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Y.S. conceived the idea, performed the theory and simulations, and wrote the article. N.P. and N.I.Z. contributed to data analysis and interpretation and supervised the project. All authors contributed to the revisions of the paper.
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Shen, Y., Papasimakis, N. & Zheludev, N.I. Nondiffracting supertoroidal pulses and optical “Kármán vortex streets”. Nat Commun 15, 4863 (2024). https://doi.org/10.1038/s41467024489275
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DOI: https://doi.org/10.1038/s41467024489275
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