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Geometric characterization of anomalous Landau levels of isolated flat bands

Abstract

According to the Onsager’s semiclassical quantization rule, the Landau levels of a band are bounded by its upper and lower band edges at zero magnetic field. However, there are two notable systems where the Landau level spectra violate this expectation, including topological bands and flat bands with singular band crossings, whose wave functions possess some singularities. Here, we introduce a distinct class of flat band systems where anomalous Landau level spreading (LLS) appears outside the zero-field energy bounds, although the relevant wave function is nonsingular. The anomalous LLS of isolated flat bands are governed by the cross-gap Berry connection that measures the wave-function geometry of multi bands. We also find that symmetry puts strong constraints on the LLS of flat bands. Our work demonstrates that an isolated flat band is an ideal system for studying the fundamental role of wave-function geometry in describing magnetic responses of solids.

Introduction

The geometry of Bloch wave functions, manifested in the quantities such as Berry curvature and Berry phase, is a central notion in the modern description of condensed matter. Due to the significant role of wave-function geometry in describing the fundamental properties of solids, finding efficient methods of measuring it has been considered a quintessential problem in solid-state physics. In this respect, examining the Landau level spectrum has received particular attention, as one of the most efficient and convenient methods for detecting the geometric properties of Bloch states.

A conventional way of determining the Landau levels of Bloch states is to use the semiclassical approach based on Onsager’s semiclassical quantization rule given by

$${S}_{0}(\epsilon )=\frac{2\pi eB}{\hslash }\left(n+\frac{1}{2}-\frac{{\gamma }_{\epsilon ,B}}{2\pi }\right),$$
(1)

which is generally valid in the weak-field limits. Here S0(ϵ) is the area of a closed semiclassical orbit at the energy ϵ in momentum space, B is a magnetic field, e is the electric charge, is the reduced Planck constant, and n is a non-negative integer. The last term γϵ,B indicates the quantum correction from Berry phase, orbital magnetization, etc.1,2,3,4,5, reflecting the geometric properties of solids. A collection of discrete energies (ϵ) satisfying Eq. (1) forms the Landau levels which critically depend on the geometric quantity γϵ,B. For instance, in graphene with relativistic energy dispersion, Eq. (1) successfully predicts the \(\sqrt{nB}\) dependence of the Landau levels, where the existence of the zero-energy Landau level is a direct manifestation of the π-Berry phase of massless Dirac particles6, 7. Later, this semiclassical approach is generalized further to the cases with an arbitrary strength of magnetic field8 where the zero-field energy dispersion in Eq. (1) is replaced by the magnetic band structure with B linear quantum corrections.

The Onsager’s semiclassical scheme has provided a powerful method of understanding complicated Landau level spectra of solids intuitively. In usual dispersive bands where B linear quantum corrections are negligible in weak-field limit, Onsager’s semiclassical approach in Eq. (1) predicts that the Landau levels are developed in the energy interval bounded by the upper and lower band edges of the zero-field band structure. However, there are a few examples of violating this expectation. Especially, several systems exhibit anomalous Landau levels appearing in gapped regions away from the zero-field energy bounds where the semiclassical orbit, as well as S0(ϵ), cannot be defined, according to Eq. (1). One famous example is the Landau levels of a Chern band which appear in an adjacent energy gap at zero-field. Similar behavior was also recently predicted in fragile topological bands characterized by nonzero Euler numbers9,10,11. More recently, it was shown that anomalous Landau levels also appear in singular flat bands12, 13, where a flat band is crossing with another parabolic band at a momentum14. Interestingly, it is found that the Landau levels of a singular flat band appear in the energy region with a vanishing density of states at zero magnetic fields. Moreover, the total energy spreading of the flat band’s Landau levels, dubbed the Landau level spreading (LLS), is solely determined by a geometric quantity, called the maximum quantum distance which characterizes the singularity of the relevant Bloch wave function14.

In this work, we propose a distinct class of flat-band systems that exhibit anomalous Landau level structures. The flat band we consider is isolated from other bands by a gap, which we call an isolated flat band (IFB). An IFB is generally non-singular as well as topologically trivial15,16,17 as opposed to nearly flat topological bands or degenerate flat bands18, 19, so that it does not belong to any category of the systems exhibiting anomalous Landau levels discussed above. However, it is found that the Landau levels of IFBs are anomalous, that is, unbounded by the original band structure at zero magnetic fields and developed in the band gaps above and below the flat band.

In fact, the Onsager’s semiclassical quantization rule in Eq. (1) generally does not work in flat bands, unless the B linear quantum corrections are properly included. This is because there are infinitely many semiclassical orbits allowed so that S0(ϵ) cannot be uniquely determined. Interestingly, after taking into account the B linear quantum corrections, we find that an IFB generally exhibits anomalous LLS, and the upper and lower energy bounds for the LLS are determined by the cross-gap Berry connection defined as

$${A}_{i}^{nm}({{{{{{{\bf{k}}}}}}}})=i\left\langle {u}_{n}({{{{{{{\bf{k}}}}}}}})| {\partial }_{i}{u}_{m}({{{{{{{\bf{k}}}}}}}})\right\rangle \quad (n\,\ne\, m),$$
(2)

where un(k) is the periodic part of the Bloch wave function of the nth band20. This is a multi-band extension of the conventional Abelian Berry connection and describes inter-band couplings. Let us note that, unlike the Abelian Berry connection defined for a single band, the cross-gap Berry connection \({A}_{i}^{nm}({{{{{{{\bf{k}}}}}}}})\,\)(n ≠ m) is gauge-covariant. We will show that the LLS of an IFB is given by the product of the x and y components of the cross-gap Berry connection between the flat band and other bands weighted by their energy. The LLS of an IFB is strongly constrained by the symmetry of the system, which is demonstrated in various flat band models including the Lieb and the Tasaki models as well as the model describing twisted bilayer graphene (see the “Results” section and Supplementary Note 4). Our work demonstrates the fundamental role of wave-function geometry in describing the Landau levels of flat bands.

Results

Modified band dispersion and the LLS

The original Onsager’s semiclassical approach predicts IFBs inert under external magnetic field, and thus it cannot explain the LLS of IFBs. On the other hand, the modified semiclassical approach developed by M.-C. Chang and Q. Niu8 can resolve this problem. Contrary to the Onsager’s approach, where the band structure at zero magnetic field εn(k) is used to define the closed semiclassical orbits and the corresponding area S0(ϵ), the modified semiclassical approach employs the modified band structure given by

$${E}_{n,B}({{{{{{{\bf{k}}}}}}}})={\varepsilon }_{n}({{{{{{{\bf{k}}}}}}}})+{\mu }_{n}({{{{{{{\bf{k}}}}}}}})B,$$
(3)

where \({{{{{{{\bf{B}}}}}}}}=B\hat{{{{{{{{\bf{z}}}}}}}}}\) is the magnetic field, n is the band index, and μn(k) is the orbital magnetic moment of the nth magnetic band in the z-direction arising from the self-rotation of the corresponding wave packet8. The explicit form of μn(k) is

$${\mu }_{n}({{{{{{{\bf{k}}}}}}}})=\frac{e}{\hslash }\ {{{{{{{\rm{Im}}}}}}}}\langle {\partial }_{x}{u}_{n}({{{{{{{\bf{k}}}}}}}})|[{\varepsilon }_{n}({{{{{{{\bf{k}}}}}}}})-H({{{{{{{\bf{k}}}}}}}})]|{\partial }_{y}{u}_{n}({{{{{{{\bf{k}}}}}}}})\rangle ,$$
(4)

where H(k) is the Hamiltonian in momentum space and \({\partial }_{i}={\partial }_{{k}_{i}}\)(i = x, y). Hence, the second term on the right-hand side of Eq. (3) indicates the leading energy correction from the orbital magnetic moment coupled to the magnetic field. In usual dispersive bands, the B-linear quantum correction is negligibly small in weak magnetic field limit compared to the zero-field band-width. This is the reason why the original Onsager’s semiclassical scheme in Eq. (1) works well.

In the case of a flat band with zero bandwidth, on the other hand, the B-linear quantum correction always dominates the modified band structure En,B(k) in Eq. (3) even in a weak magnetic field limit. Moreover, the modified band dispersion of an IFB is generally dispersive so that the relevant semiclassical orbits can be defined unambiguously. As a result, one can obtain the Landau levels of the IFB in the adjacent gapped regions by applying the semiclassical quantization rule to En,B(k), which naturally explains the LLS of the IFB. Especially, around the band edges of En,B(k), one can define the effective mass m*, which is inversely proportional to B, from which the Onsager’s scheme predicts Landau levels with a spacing eB/m*B2. The resulting Landau spectrum is bounded by the upper and lower band edges of En,B(k). The total magnitude Δ of the LLS is determined by the difference between the maximum and the minimum values of En,B(k), namely, \({{\Delta }}=\max \ {E}_{n,B}({{{{{{{\bf{k}}}}}}}})-\min \ {E}_{n,B}({{{{{{{\bf{k}}}}}}}})\). This result is valid as long as the band gap Egap between the IFB and its neighboring band at zero magnetic field is large enough, i.e., \({E}_{{{{{{{{\rm{gap}}}}}}}}}\gg \max | {E}_{n,B}({{{{{{{\bf{k}}}}}}}})|\). The generic behavior of an IFB under magnetic field is schematically described in Fig. 1 where one can clearly observe that the Landau levels of the IFB spread into the gaps at zero-field above and below the IFB.

Fig. 1: Landau level spreading (LLS) of an isolated flat band (IFB).
figure 1

a The band structure of a two-dimensional system in the absence of a magnetic field. The second band with the energy ε2(k) = 0 corresponds to the IFB. The inter-band coupling \({\varepsilon }_{m}({{{{{{{\bf{k}}}}}}}}){\chi }_{xy}^{m2}({{{{{{{\bf{k}}}}}}}})\) of the IFB with the other dispersive band of the energy εm(k)(m = 1, 3, 4) is indicated by a dashed vertical arrow. b The modified band dispersion En,B(k)(n = 1, …, 4) in the presence of the magnetic field. The corresponding Landau levels are shown by red solid lines. The LLS of the IFB is represented by the green arrow.

Geometric interpretation of the LLS

Interestingly, we find that the LLS of IFBs is a manifestation of the non-trivial wave-function geometry of the flat band arising from inter-band couplings. One can show that the modified band dispersion of the IFB is given by

$${E}_{n,B}({{{{{{{\bf{k}}}}}}}})=-2\pi \frac{\phi }{{\phi }_{0}}\frac{1}{{A}_{0}}{{{{{{{\rm{Im}}}}}}}}\ \mathop{\sum}\limits_{m\ne n}{\varepsilon }_{m}({{{{{{{\bf{k}}}}}}}}){\chi }_{xy}^{nm}({{{{{{{\bf{k}}}}}}}}),$$
(5)

in which

$${\chi }_{ij}^{nm}({{{{{{{\bf{k}}}}}}}})=\left\langle {\partial }_{i}{u}_{n}({{{{{{{\bf{k}}}}}}}})| {u}_{m}({{{{{{{\bf{k}}}}}}}})\right\rangle \langle {u}_{m}({{{{{{{\bf{k}}}}}}}})| {\partial }_{j}{u}_{n}({{{{{{{\bf{k}}}}}}}})\rangle ={A}_{i}^{nm}{({{{{{{{\bf{k}}}}}}}})}^{* }{A}_{j}^{nm}({{{{{{{\bf{k}}}}}}}}).$$
(6)

where ϕ0 = h/e, ϕ = BA0 is the magnetic flux per unit cell, and A0 is the unit cell area assumed to be A0 = 1. Here, we assume that the nth band is the IFB at the zero-energy without loss of generality so that εm(k) in Eq. (5) should be interpreted as the energy of the mth band with respect to the flat band energy. We note that \({A}_{i}^{nm}({{{{{{{\bf{k}}}}}}}})=\left\langle {u}_{m}({{{{{{{\bf{k}}}}}}}})| {\partial }_{i}{u}_{n}({{{{{{{\bf{k}}}}}}}})\right\rangle\) indicates the cross-gap Berry connection between the nth and mth bands (n ≠ m) defined above, and \({\chi }_{ij}^{nm}({{{{{{{\bf{k}}}}}}}})\) is the corresponding fidelity tensor that describes the transition amplitude between the nth and mth bands as discussed below. See Supplementary Notes 1 for the detailed derivation of Eq. (5). Hence, Eq. (5) indicates that the modified band dispersion of the IFB is given by the summation of the transition amplitudes \({\chi }_{xy}^{nm}({{{{{{{\bf{k}}}}}}}})\) between the IFB and the mth band weighted by the energy εm(k) of the mth band as illustrated in Fig. 1. This means that the immobile carriers with infinite effective mass in an IFB can respond to external magnetic field through the inter-band coupling, characterized by the cross-gap Berry connection, to dispersive bands. The geometric character of the LLS is evident in our interpretation based on Eq. (5).

Let us discuss the geometric character of the fidelity tensor \({\chi }_{xy}^{nm}({{{{{{{\bf{k}}}}}}}})\) more explicitly. In general, the geometry of the quantum state un(k) can be derived from the Hilbert–Schmidt quantum distance21,22,23 defined as

$$s\left({u}_{n}({{{{{{{\bf{k}}}}}}}}),{u}_{n}({{{{{{{\bf{k}}}}}}}}^{\prime} )\right)=1-| \langle {u}_{n}({{{{{{{\bf{k}}}}}}}})| {u}_{n}({{{{{{{\bf{k}}}}}}}}^{\prime} )\rangle {| }^{2},$$
(7)

which measures the similarity between un(k) and \({u}_{n}({{{{{{{\bf{k}}}}}}}}^{\prime} )\). For \({{{{{{{\bf{k}}}}}}}}^{\prime} ={{{{{{{\bf{k}}}}}}}}+d{{{{{{{\bf{k}}}}}}}}\), we obtain

$$s\left({u}_{n}({{{{{{{\bf{k}}}}}}}}),{u}_{n}({{{{{{{\bf{k}}}}}}}}+d{{{{{{{\bf{k}}}}}}}})\right)={{\mathfrak{G}}}_{ij}^{n}({{{{{{{\bf{k}}}}}}}})d{k}_{i}d{k}_{j},$$
(8)

where \({{\mathfrak{G}}}_{ij}^{n}({{{{{{{\bf{k}}}}}}}})\) indicates the quantum geometric tensor24,25,26 whose explicit form is

$${{\mathfrak{G}}}_{ij}^{n}({{{{{{{\bf{k}}}}}}}})=\mathop{\sum}\limits_{m\ne n}\left\langle {\partial }_{i}{u}_{n}({{{{{{{\bf{k}}}}}}}})| {u}_{m}({{{{{{{\bf{k}}}}}}}})\right\rangle \langle {u}_{m}({{{{{{{\bf{k}}}}}}}})| {\partial }_{j}{u}_{n}({{{{{{{\bf{k}}}}}}}})\rangle =\mathop{\sum}\limits_{m\ne n}{\chi }_{ij}^{nm}({{{{{{{\bf{k}}}}}}}}),$$
(9)

which shows that the quantum geometric tensor \({{\mathfrak{G}}}_{ij}^{n}({{{{{{{\bf{k}}}}}}}})\) of the nth band is given by the summation of the fidelity tensor \({\chi }_{ij}^{nm}({{{{{{{\bf{k}}}}}}}})\) over all m ≠ n. We note that \({\chi }_{ij}^{nm}({{{{{{{\bf{k}}}}}}}})\) itself cannot define a distance as the triangle inequality is not satisfied. However, it is related to the transition probability or the fidelity \(F\left({u}_{n}({{{{{{{\bf{k}}}}}}}}),{u}_{m}({{{{{{{\bf{k}}}}}}}}^{\prime} )\right)\) between the nth and mth bands27 through the following relations:

$$F\left({u}_{n}({{{{{{{\bf{k}}}}}}}}),{u}_{m}({{{{{{{\bf{k}}}}}}}}^{\prime} )\right)=| \langle {u}_{n}({{{{{{{\bf{k}}}}}}}})| {u}_{m}({{{{{{{\bf{k}}}}}}}}^{\prime} )\rangle {| }^{2},$$
(10)
$$F\left({u}_{n}({{{{{{{\bf{k}}}}}}}}),{u}_{m}({{{{{{{\bf{k}}}}}}}}+d{{{{{{{\bf{k}}}}}}}})\right)={\chi }_{ij}^{nm}({{{{{{{\bf{k}}}}}}}})d{k}_{i}d{k}_{j}.$$
(11)

Thus, the geometric interpretation based on Eqs. (5) and (11) clearly show that the LLS originates from the inter-band coupling.

Symmetry constraints on the LLS

The LLS of an IFB is strongly constrained by symmetry. First, we consider a generic symmetry σ whose action on the Hamiltonian is given by

$${U}_{\sigma }({{{{{{{\bf{k}}}}}}}}){\overline{H({{{{{{{\bf{k}}}}}}}})}}^{s}{U}_{\sigma }{({{{{{{{\bf{k}}}}}}}})}^{{{{\dagger}}} }=pH({O}_{\sigma }{{{{{{{\bf{k}}}}}}}}),$$
(12)

where s {0, 1}, p {−1, 1}, and Uσ(k) and Oσ are unitary and orthogonal matrices representing σ, respectively. \({\overline{x}}^{s = 1}\) denotes the complex conjugation of x while \({\overline{x}}^{s = 0}=x\). Note that s = 0 and 1 are relevant to the unitary and anti-unitary symmetries, respectively, while p = −1 and +1 correspond to anti-symmetry and symmetry, respectively.

Among all possible symmetries of the form in Eq. (12), we find that the modified band dispersion En,B(k) vanishes when the system respects the chiral C or space–time-inversion IST symmetries in the zero magnetic flux (see the “Methods” section and Supplementary Notes 2 and 3 for the detailed derivation). C and IST are characterized by \(({O}_{\sigma },s,p)=({\mathbb{1}},0,-1)\) and \(({\mathbb{1}},1,1)\), respectively, where \({\mathbb{1}}\) is the identity matrix. In the following, we demonstrate that the LLS is proportional to B2 for a flat-band system with IST symmetry in the zero magnetic fields, while the LLS is forbidden in the presence of chiral symmetry. Interestingly, although IST symmetry would be broken as the magnetic field is turned on, the LLS is strongly constrained by IST symmetry.

We further find that \(\max \ {E}_{n,B}({{{{{{{\bf{k}}}}}}}})=-\min \ {E}_{n,B}({{{{{{{\bf{k}}}}}}}})\) when the system respects a symmetry satisfying \({(-1)}^{s}p\ {{{{{{{\rm{Det}}}}}}}}{O}_{\sigma }=-1\) and \({O}_{\sigma }\,\ne\, {\mathbb{1}}\), such as time-reversal T or reflection R symmetry, at the zero magnetic field (see the “Methods” section and Supplementary Note 2 for detailed derivations). This implies that the minimum and maximum values of the LLS have the same magnitude but with opposite signs. The relevant tight-binding models are shown in Supplementary Notes 4.

Generic flat-band systems

We first consider the spin–orbit-coupled (SOC) Lieb model28 as an example of generic flat-band systems. The lattice structure for this model is shown in Fig. 2a. The model consists of the nearest-neighbor hopping with the amplitude 1 and the spin–orbit coupling between the next nearest neighbor sites, which are denoted as green solid and dashed arrows, respectively, in Fig. 2a. The tight-binding Hamiltonian in momentum space is given by

$${H}_{{{{{{{{\rm{socL}}}}}}}}}({{{{{{{\bf{k}}}}}}}})=\left(\begin{array}{lll}0&2\cos \frac{{k}_{y}}{2}&-4i{\lambda }_{{{{{{{{\rm{soc}}}}}}}}}\sin \frac{{k}_{x}}{2}\sin \frac{{k}_{y}}{2}\\ 2\cos \frac{{k}_{y}}{2}&0&2\cos \frac{{k}_{x}}{2}\\ 4i{\lambda }_{{{{{{{{\rm{soc}}}}}}}}}\sin \frac{{k}_{x}}{2}\sin \frac{{k}_{y}}{2}&2\cos \frac{{k}_{x}}{2}&0\end{array}\right),$$
(13)

where λsoc denotes the strength of spin–orbit coupling. The flat band’s energy is zero, i.e., εsocL,fb(k) = 0, and the energies of the other two bands are

$${\varepsilon }_{{{{{{{{\rm{socL}}}}}}}},\pm }({{{{{{{\bf{k}}}}}}}})=\pm 2\sqrt{{\cos }^{2}\frac{{k}_{x}}{2}+{\cos }^{2}\frac{{k}_{y}}{2}+4{\lambda }_{soc}^{2}{\sin }^{2}\frac{{k}_{x}}{2}{\sin }^{2}\frac{{k}_{y}}{2}},$$
(14)

which are plotted in Fig. 2b for λsoc = 0.2. The band gap between the IFB and its neighboring bands is given by 4λsoc if λsoc < 1/2, and 2 if λsoc ≥ 1/2, thus the flat band is decoupled from other bands for non-zero λsoc.

Fig. 2: Landau level spreading of a generic system with an IFB.
figure 2

a Lattice structure for the spin–orbit-coupled (SOC) Lieb model composed of three sublattices, A, B and C. The double-headed green arrows denote the nearest neighbor hoppings, and the single-headed green arrows indicate the spin–orbit coupling between A and C sublattices. The next-nearest hoppings t between A and C is set to be zero (t = 0.0) in the SOC Lieb model. b The band structure of HsocL(k) with λsoc = 0.2. c Distribution of \({{{{{{{\rm{Im}}}}}}}}\ {\chi }_{{{{{{{{\rm{socL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},-}({{{{{{{\bf{k}}}}}}}})\). Note that \({{{{{{{\rm{Im}}}}}}}}\ {\chi }_{{{{{{{{\rm{socL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},-}({{{{{{{\bf{k}}}}}}}})=-{{{{{{{\rm{Im}}}}}}}}\ {\chi }_{{{{{{{{\rm{socL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},+}({{{{{{{\bf{k}}}}}}}})\). d The modified band dispersion \({E}_{{{{{{{{\rm{fb}}}}}}}},B}^{{{{{{{{\rm{socL}}}}}}}}}({{{{{{{\bf{k}}}}}}}})\) of the flat band in the presence of magnetic flux. e Landau level spectra of the flat band (black dots) as a function of λsoc for magnetic flux ϕ/ϕ0 = 1/500. f Landau level spectra of the flat band (black dots) as a function of magnetic flux ϕ/ϕ0 for λsoc = 0.2.

The analytic form of the fidelity tensor \({\chi }_{xy}^{nm}({{{{{{{\bf{k}}}}}}}})\) is given by

$${\chi }_{{{{{{{{\rm{socL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},+}({{{{{{{\bf{k}}}}}}}})={\left({\chi }_{{{{{{{{\rm{socL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},-}({{{{{{{\bf{k}}}}}}}})\right)}^{* }=\frac{f({k}_{x},{k}_{y})f({k}_{y},{k}_{x})}{{\left({\varepsilon }_{{{{{{{{\rm{socL}}}}}}}},+}({{{{{{{\bf{k}}}}}}}})\right)}^{4}(2+\cos {k}_{x}+\cos {k}_{y})},$$
(15)

where \(f({k}_{x},{k}_{y})=4{\lambda }_{{{{{{{{\rm{soc}}}}}}}}}\sin \frac{{k}_{x}}{2}\cos \frac{{k}_{y}}{2}({\cos }^{2}\frac{{k}_{x}}{2}+1)+i{\varepsilon }_{{{{{{{{\rm{socL}}}}}}}},+}({{{{{{{\bf{k}}}}}}}})\cos \frac{{k}_{x}}{2}\sin \frac{{k}_{y}}{2}\). Then, from Eq. (5), the modified band dispersion for the flat band is given by

$${E}_{{{{{{{{\rm{fb}}}}}}}},B}^{{{{{{{{\rm{socL}}}}}}}}}({{{{{{{\bf{k}}}}}}}})=-\frac{2\pi {\lambda }_{{{{{{{{\rm{soc}}}}}}}}}\left(3-\cos {k}_{x}-\cos {k}_{y}-\cos {k}_{x}\cos {k}_{y}\right)}{{\left({\varepsilon }_{{{{{{{{\rm{socL}}}}}}}},+}({{{{{{{\bf{k}}}}}}}})\right)}^{2}}\ \frac{\phi }{{\phi }_{0}}.$$
(16)

In Fig. 2c, d, \({{{{{{{\rm{Im}}}}}}}}\ {\chi }_{{{{{{{{\rm{socL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},-}({{{{{{{\bf{k}}}}}}}})\) and \({E}_{{{{{{{{\rm{fb}}}}}}}},B}^{{{{{{{{\rm{socL}}}}}}}}}({{{{{{{\bf{k}}}}}}}})\) are shown. We note that

$$\max {E}_{{{{{{{{\rm{fb}}}}}}}},B}^{{{{{{{{\rm{socL}}}}}}}}}({{{{{{{\bf{k}}}}}}}})={E}_{{{{{{{{\rm{fb}}}}}}}},B}^{{{{{{{{\rm{socL}}}}}}}}}(0,0)=0,$$
(17)
$$\min {E}_{{{{{{{{\rm{fb}}}}}}}},B}^{{{{{{{{\rm{socL}}}}}}}}}({{{{{{{\bf{k}}}}}}}})=\left\{\begin{array}{ll}{E}_{{{{{{{{\rm{fb}}}}}}}},B}^{{{{{{{{\rm{socL}}}}}}}}}(\pi ,\pi )=-\frac{\pi }{2{\lambda }_{{{{{{{{\rm{soc}}}}}}}}}}\frac{\phi }{{\phi }_{0}}&({\lambda }_{{{{{{{{\rm{soc}}}}}}}}}\le \frac{1}{2})\\ {E}_{{{{{{{{\rm{fb}}}}}}}},B}^{{{{{{{{\rm{socL}}}}}}}}}(0,\pi )=-2\pi {\lambda }_{{{{{{{{\rm{soc}}}}}}}}}\frac{\phi }{{\phi }_{0}}&({\lambda }_{{{{{{{{\rm{soc}}}}}}}}} > \frac{1}{2})\end{array}\right..$$
(18)

These minimum and maximum values of \({E}_{{{{{{{{\rm{fb}}}}}}}},B}^{{{{{{{{\rm{socL}}}}}}}}}({{{{{{{\bf{k}}}}}}}})\) correspond to the lower and upper bounds for the LLS of the IFB as illustrated by red lines in Fig. 2e, f. Interestingly, the fidelity tensors \({\chi }_{{{{{{{{\rm{socL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},+}({{{{{{{\bf{k}}}}}}}})\) and \({\chi }_{{{{{{{{\rm{socL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},-}({{{{{{{\bf{k}}}}}}}})\) are conjugate of each other. This originates from the anti-unitary symmetry CIST, a combination of chiral C and space–time-inversion IST symmetries, present in the system (see Supplementary Note 2 for the details.)

Chiral-symmetric system

We construct a chiral-symmetric Lieb (c-Lieb) model as a representative example for chiral-symmetric IFB systems. The c-Lieb is defined on the same Lieb lattice as the SOC-Lieb model, but with different hoppings. As shown in Fig. 3a, this model consists only of the nearest-neighbor hoppings, denoted by green arrows. The hopping parameter from a B-site to a C-site is t1 for the rightward hopping, and 1 for the leftward hopping. On the other hand, the hopping parameter from a B-site to an A-site is t2 for the upward hopping, and 1 for the downward hopping. The corresponding tight-binding Hamiltonian in momentum space is given by

$${H}_{{{{{{{{\rm{cL}}}}}}}}}({{{{{{{\bf{k}}}}}}}})=\left(\begin{array}{lll}0&{e}^{i\frac{{k}_{y}}{2}}+{t}_{2}{e}^{-i\frac{{k}_{y}}{2}}&0\\ {e}^{-i\frac{{k}_{y}}{2}}+{t}_{2}{e}^{i\frac{{k}_{y}}{2}}&0&{e}^{-i\frac{{k}_{x}}{2}}+{t}_{1}{e}^{i\frac{{k}_{x}}{2}}\\ 0&{e}^{i\frac{{k}_{x}}{2}}+{t}_{1}{e}^{-i\frac{{k}_{x}}{2}}&0\end{array}\right),$$
(19)

with energy eigenvalues εcL,fb(k) = 0 and \({\varepsilon }_{{{{{{{{\rm{cL}}}}}}}},\pm }({{{{{{{\bf{k}}}}}}}})=\pm \sqrt{2+{t}_{1}^{2}+{t}_{2}^{2}+2{t}_{1}\cos {k}_{x}+2{t}_{2}\cos {k}_{y}}\). The chiral symmetry operator C is given by C = Diag(1,−1,1) which gives a symmetry relation,

$$C{H}_{{{{{{{{\rm{cL}}}}}}}}}({{{{{{{\bf{k}}}}}}}}){C}^{-1}=-{H}_{{{{{{{{\rm{cL}}}}}}}}}({{{{{{{\bf{k}}}}}}}}).$$
(20)

Note that the wave function of the flat band is also a simultaneous eigenstate of the chiral symmetry having a definite chiral charge c = +1:

$$C|{u}_{{{{{{{{\rm{cL,fb}}}}}}}}}({{{{{{{\bf{k}}}}}}}})\rangle =c|{u}_{{{{{{{{\rm{cL,fb}}}}}}}}}({{{{{{{\bf{k}}}}}}}})\rangle .$$
(21)

Also, we obtain the fidelity tensor \({\chi }_{xy}^{{{{{{{{\rm{fb}}}}}}}},\pm }\), expressed by

$${\chi }_{{{{{{{{\rm{cL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},+}({{{{{{{\bf{k}}}}}}}}) ={\chi }_{{{{{{{{\rm{cL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},-}({{{{{{{\bf{k}}}}}}}})\\ =-\frac{(1+{t}_{1}{e}^{i{k}_{x}})(1-{t}_{1}{e}^{-i{k}_{x}})(1+{t}_{2}{e}^{-i{k}_{y}})(1-{t}_{2}{e}^{i{k}_{y}})}{8{\left({\varepsilon }_{{{{{{{{\rm{cL}}}}}}}},+}({{{{{{{\bf{k}}}}}}}})\right)}^{4}}.$$
(22)

The band structure and \({{{{{{{\rm{I}}}}}}}}m\ {\chi }_{{{{{{{{\rm{cL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},-}({{{{{{{\bf{k}}}}}}}})\) are shown in Fig. 3b, c. Equation (22) indicates that the modified band dispersion Efb,B(k) vanishes for all k because εcL,+(k) = −εcL,−(k), which means that there is no LLS in the weak magnetic field. Also, we calculate the Hofstadter spectrum29 for the c-Lieb model. Interestingly, we find that the LLS is absent even in the strong magnetic field, as shown in Fig. 3d. The existence of such zero-energy flat bands in the finite magnetic flux is guaranteed by chiral symmetry C. As explained in Supplementary Note 3, the minimal number of zero-energy flat bands is given by \(| {{{{{{{\rm{Tr}}}}}}}}[C]|\) at the zero magnetic flux. Moreover, when the system has the \(| {{{{{{{\rm{Tr}}}}}}}}[C]| ( > 0)\) number of zero-energy flat bands at the zero magnetic flux, the LLS of the flat band(s) is forbidden unless a gap closes at zero energy E = 0 as the magnetic flux increases (see Supplementary Note 3). In the c-Lieb model, such a gap closing at E = 0 does not occur at any magnetic flux. Hence, there is no LLS in all range of magnetic flux. On the other hand, when a gap closes at E = 0 as the magnetic flux increases, the LLS is forbidden only in a finite range of magnetic flux. As an example, in Supplementary Note 4, we show the Hofstadter spectrum of the ten-band model for twisted-bilayer graphene proposed in ref. 30.

Fig. 3: Landau level spreading of a flat-band system with chiral symmetry.
figure 3

a Lattice structure for the c-Lieb model. The green arrows denote the hoppings. Note that the direction dependent hopping parameters induce a finite gap between the flat band and other bands. b The band structure for HcL(k) with t1 = t2 = 2. c Distribution of \({{{{{{{\rm{Im}}}}}}}}\ {\chi }_{{{{{{{{\rm{cL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},-}({{{{{{{\bf{k}}}}}}}})\). Due to the chiral symmetry, \({{{{{{{\rm{Im}}}}}}}}\ {\chi }_{{{{{{{{\rm{cL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},-}({{{{{{{\bf{k}}}}}}}})={{{{{{{\rm{Im}}}}}}}}\ {\chi }_{{{{{{{{\rm{cL}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},+}({{{{{{{\bf{k}}}}}}}})\) holds. d The Hofstadter spectrum of the c-Lieb model HcL(k) with t1 = t2 = 2. For any value of magnetic flux, the Landau levels of the flat band are fixed to the zero energy.

Space–time-inversion-symmetric system

The LLS of an IFB is weakly dependent on the magnetic field when the system respects space–time-inversion IST symmetry at zero magnetic field. We consider spinless fermions on the checkerboard lattice shown in Fig. 4a, which is sometimes called the Tasaki or decorated square lattice31,32,33. This model respects both time-reversal T and inversion I symmetries. Hence, a combined symmetry, space–time-inversion symmetry IST = IT, exists. We note that the following discussion holds even if T and I are broken as long as IST is not broken. The tight-binding Hamiltonian consists of the hopping processes up to the third nearest-neighbor hopping. In momentum space, the Hamiltonian is written as

$${H}_{{I}_{{{{{{{{\rm{ST}}}}}}}}}}({{{{{{{\bf{k}}}}}}}})=\left(\begin{array}{ll}1&\cos \frac{{k}_{+}}{2}+2t\cos \frac{{k}_{-}}{2}\\ \cos \frac{{k}_{+}}{2}+2t\cos \frac{{k}_{-}}{2}&2t\cos {k}_{x}+2t\cos {k}_{y}+{\cos }^{2}\frac{{k}_{+}}{2}+4{t}^{2}{\cos }^{2}\frac{{k}_{-}}{2}\end{array}\right),$$
(23)
$$=\left(\begin{array}{l}1\\ \cos \frac{{k}_{+}}{2}+2t\cos \frac{{k}_{-}}{2}\end{array}\right)\left(1\cos \frac{{k}_{+}}{2}+2t\cos \frac{{k}_{-}}{2}\right),$$
(24)

where k± = kx ± ky. For t = 1.0, the band structure is shown in Fig. 4b. This system hosts a flat band with zero energy and a dispersive band with positive energy. The energy eigenvalues are given by \({\varepsilon }_{{I}_{{{{{{{{\rm{ST}}}}}}}}},\uparrow }({{{{{{{\bf{k}}}}}}}})=1+{(\cos \frac{{k}_{+}}{2}+2t\cos \frac{{k}_{-}}{2})}^{2}\) and \({\varepsilon }_{{I}_{{{{{{{{\rm{ST}}}}}}}}},{{{{{{{\rm{fb}}}}}}}}}({{{{{{{\bf{k}}}}}}}})=0\).

Fig. 4: Landau level spreading of a flat-band system with space–time-inversion symmetry.
figure 4

a The lattice structure for the IST-symmetric checkerboard model. The red and black lines denote the hopping processes between A and B sublattices. b The band structure of \({H}_{{I}_{{{{{{{{\rm{ST}}}}}}}}}}({{{{{{{\bf{k}}}}}}}})\) with t = 1.0. c The Hofstadter spectrum of the IST-symmetric checkerboard model with t = 1.0. d Variation of the lowest and highest Landau levels related to the flat band in the weak magnetic field (blue and black circles). \({E}_{{{{{{{{\rm{fb}}}}}}}},\min }(\phi /{\phi }_{0})\) and \({E}_{{{{{{{{\rm{fb}}}}}}}},\max }(\phi /{\phi }_{0})\) indicate the corresponding fitting functions (red and black solid lines) that exhibit quadratic magnetic field dependence dominantly.

In this system, IST is simply given by the complex conjugation, i.e., \({I}_{{{{{{{{\rm{ST}}}}}}}}}={{{{{{{\mathcal{K}}}}}}}}\) and

$${I}_{{{{{\rm{{ST}}}}}}}|{u}_{{I}_{{{{{{{{\rm{ST}}}}}}}}},{{{{{{{\rm{fb}}}}}}}}/\uparrow }({{{{{{{\bf{k}}}}}}}})\rangle =|{u}_{{I}_{{{{{{{{\rm{ST}}}}}}}}},{{{{{{{\rm{fb}}}}}}}}/\uparrow }({{{{{{{\bf{k}}}}}}}})\rangle .$$
(25)

Also, explicit calculations show \({{{{{{{\rm{Im}}}}}}}}\ {\chi }_{{I}_{{{{{{{{\rm{ST}}}}}}}}},xy}^{{{{{{{{\rm{fb}}}}}}}},\uparrow }({{{{{{{\bf{k}}}}}}}})=0\) and the vanishing modified band dispersion for the flat band En,B(k) = 0, which results from Eq. (25). In Supplementary Note 2, we have proved that space–time inversion IST imposes En,B(k) = 0 in general. We also note that En,B(k) = 0 is consistent with the fact that the orbital angular momentum, which is proportional to the orbital magnetic moment, is constrained to be zero in IST-symmetric systems. Although the LLS is negligible in the weak magnetic field, it becomes considerably large in the strong magnetic field as shown in the Hofstadter spectrum in Fig. 4c. As shown in Fig. 4c, the Landau levels of the flat band acquire or lose their energy as the magnetic flux increases from 0 to some finite value much less than 1. This implies that the higher-order corrections of the magnetic field must be considered. Although it is out of the scope of this work, we present a fitting of the highest and lowest Landau levels of the flat band with respect to the magnetic flux:

$${E}_{{{{{{{{\rm{fb}}}}}}}},\min }(\phi /{\phi }_{0})=1.35\times 1{0}^{-5}-5.51\times 1{0}^{-3}(\phi /{\phi }_{0})-2.53{(\phi /{\phi }_{0})}^{2},$$
(26)
$${E}_{{{{{{{{\rm{fb}}}}}}}},\max }(\phi /{\phi }_{0})=-4.56\times 1{0}^{-7}+1.82\times 1{0}^{-4}(\phi /{\phi }_{0})+0.50{(\phi /{\phi }_{0})}^{2},$$
(27)

which is plotted in Fig. 4d where one can observe the dominant quadratic dependence on the magnetic field.

Finally, we comment on the gap closing at (ϕ/ϕ0, E) = (1, 1.0) in the Hofstadter spectrum in Fig. 4c. At (ϕ/ϕ0, E) = (1, 1.0), the Landau levels related to the flat and dispersive bands show a closing of an indirect gap. We note that there is no closing of direct gaps in the Hofstadter Hamiltonian. Unlike the inevitable closing of the direct gap between topological bands in the finite magnetic flux reported before11, 34, it is not necessary to close a direct gap in our system.

Discussion

We have shown that the LLS of an IFB is determined by its wave-function geometry and the underlying symmetry of the system. The idea presented in this work goes beyond the conventional semiclassical idea in which the Landau level spectrum is dominantly determined by the band dispersion at zero magnetic fields. So far, we have focused on cases when the bandwidth of the IFB is strictly zero. However, in real materials, it is difficult to observe perfect flat bands due to the long-range hoppings and spin–orbit coupling35,36,37,38,39. To understand the influence of finite bandwidth of the IFB, we have studied another tight-binding model defined in the Lieb lattice including spin–orbit coupling. The hopping parameters, the band structure, and the LLS of this system are described in Figs. 2a,  5a–c, respectively. Under weak magnetic flux with tλsocϕ > 0, the LLS of the IFB cannot be observed because it is dominated by the energy scale of the bandwidth of the nearly flat band. However, the anomalous LLS arising from the wave-function geometry can be observed for the magnetic flux larger than a threshold value \({(\phi /{\phi }_{0})}_{{{{{{{{\rm{thres}}}}}}}}} \sim 8t{\lambda }_{{{{{{{{\rm{soc}}}}}}}}}/\pi\) (see Fig. 5c). On the other hand, the LLS is not disturbed by the bandwidth when tλsocϕ < 0, because the nearly flat band has only positive energy (see Fig. 5c). Such a Lieb lattice model with spin–orbit coupling hosting a nearly flat band was already realized in an exciton-polariton system40, and also is expected to be realized in electronic systems consisting of covalently bonded organic frameworks41.

Fig. 5: Influence of finite bandwidth and disorder on the Landau level spreading of IFBs.
figure 5

ac A nearly flat band in the spin-orbit coupled Lieb lattice where the dispersion of the FB arises from the next nearest neighbor hoppings between A and C sublattices with the amplitude t (see Fig. 2a). a The band structure of the nearly-flat-Lieb model with (t, λsoc) = (0, 0.2) and (0.02, 0.2), which are denoted by the black and red lines, respectively. The right side of the band structure describes the first Brillouin zone and the high-symmetry points. b The Landau levels in the weak magnetic field for t = 0.00 and λsoc = 0.2. The lowest (highest) Landau level has the energy \(-\frac{\pi }{2{\lambda }_{{{{{{{{\rm{soc}}}}}}}}}}\phi /{\phi }_{0}\) when ϕ > 0 (ϕ < 0). c Similar plot for t = 0.02 and λsoc = 0.2. When ϕ > 0, the LLS can be observed once the magnetic flux exceeds the threshold value \({(\phi /{\phi }_{0})}_{{{{{{{{\rm{thres}}}}}}}}} \sim \frac{8t{\lambda }_{{{{{{{{\rm{soc}}}}}}}}}}{\pi }\) because of the finite band width 4t. While, the threshold magnetic flux is zero when ϕ < 0 since the LLS develops only in the negative energy direction. df Density of states (DOS) of Landau levels in the presence of disorder. d DOS of Landau levels in very clean system with W = 0.001. The red (black) line corresponds to ϕ/ϕ0 = 1.00 × 10−2 (1.25 × 10−2). The lowest Landau level (LLL) peaks are denoted by black and red arrows. The energy range of the plot corresponds to the red dashed box in (b). e DOS of Landau levels for W = 0.02. f The intensity plot of the DOS (or the Landau fan diagram) for W = 0.02 and the iteration number \({N}_{{{{{{{{\rm{itr}}}}}}}}}=20\) as a function of ϕ/ϕ0. The plot ranges for the energy and magnetic flux correspond to the red dashed box in (b). The black dashed line indicates the LLL peak positions. Note that the maximum value of DOS in the plotted region is 2.306 × 10−2 (arb. unit).

Finally, we discuss the influence of disorder on the LLS of an IFB and the related Landau level fan diagram. The fan diagram is obtained by calculating the density of states (DOS) of Landau levels of the disordered SOC Lieb model including a random impurity potential whose maximum strength is denoted by W (see the “Methods” section for details). As shown in Fig. 5d, e, aside from the huge and wide DOS peaks from the dense Landau levels with higher Landau level indices, one can find small but sharp peaks corresponding to the LLLs of the IFB, from which the LLS of the IFB can be determined. While this LLL peak is buried in the DOS envelope of the higher Landau levels in the weak magnetic field, it splits away from this envelope as the magnetic field is large enough as shown in Fig. 5f. From the fan diagram, one can check the geometric principle described by Eq. (5) by extracting the slope of the LLL, which is represented by the dashed guideline in Fig. 5f. Here we considered the magnetic fluxes ϕ/ϕ0 below 1.25 × 10−2, which correspond to the experimentally accessible region. Note that when the size of a unit cell is equal to lnm, the relevant magnetic field is about B ~ 4000 × ϕ/ϕ0 × l−2(T) approximately. For instance, in the case of the Lieb lattice composed of the covalently bonded organic frameworks41, ϕ/ϕ0 = 1.25 × 10−2 corresponds to B ~ 50 T. We expect the DOS peak corresponding to the LLL to be detected by the resistance measurement from magnetotransport experiments or the dI/dV measurement from the scanning tunneling spectroscopy if the magnetic field is strong enough or the system is sufficiently clean so that the Landau level spacing becomes larger than the Landau level broadening. Especially, when the LLS develops asymmetrically, like in Fig. 5b, an overall energy shift of the DOS from the flat band’s energy appears more prominently, which provides a direct experimental signature of the LLS even in disordered systems.

Up to now, our discussion has been focused on conventional materials to realize flat bands. However, it is worth noting that there are various artificial systems such as photonic systems13, 42,43,44, optical lattices45,46,47,48,49,50, and systems with synthetic dimensions51,52,53,54,55, which could offer better opportunities to test our theoretical prediction. In these systems, band engineering is relatively easier, and controlled experiments with artificial magnetic fields can also be performed. Designing realistic experimental setups for observing LLS of flat bands in such artificial systems would be one important problem for future study.

Methods

Symmetry constraints on the LLS

In order to derive the symmetry constraints on En,B(k) and \({\chi }_{xy}^{nm}({{{{{{{\bf{k}}}}}}}})\), let us consider a symmetry operation σ acting on the Hamiltonian,

$${U}_{\sigma }({{{{{{{\bf{k}}}}}}}}){\overline{H({{{{{{{\bf{k}}}}}}}})}}^{s}{U}_{\sigma }{({{{{{{{\bf{k}}}}}}}})}^{{{{\dagger}}} }=pH({O}_{\sigma }{{{{{{{\bf{k}}}}}}}}),$$
(28)

where s {0, 1}, p {−1,1}, Uσ indicates a unitary matrix representing the symmetry σ, and \(\overline{x}={x}^{* }\) means the complex conjugation of x. From now on, we use a compact notation \({{\mathfrak{g}}}_{\sigma }=({O}_{\sigma },s,p)\) to describe the operation of the symmetry σ. For example, \({{\mathfrak{g}}}_{T}=(-{{\mathbb{1}}}_{d},1,1)\) is used for time-reversal symmetry T where d and \({{\mathbb{1}}}_{d}\) denote the dimensionality and the d × d identity matrix, respectively. The symmetry constraints on En,B(k) and \({\chi }_{ij}^{nm}({{{{{{{\bf{k}}}}}}}})\) derived from Eq. (28) are

$${E}_{n,B}({O}_{\sigma }{{{{{{{\bf{k}}}}}}}})={(-1)}^{s}p\ {{{{{{{\rm{Det}}}}}}}}{O}_{\sigma }\ {E}_{n,B}({{{{{{{\bf{k}}}}}}}}),$$
(29)
$${\chi }_{ij}^{n{m}_{\sigma }}({O}_{\sigma }{{{{{{{\bf{k}}}}}}}})={[{O}_{\sigma }]}_{i{i}^{\prime}}{[{O}_{\sigma }]}_{j{j}^{\prime}}{\overline{{\chi }_{{i}^{\prime}{j}^{\prime}}^{nm}({{{{{{{\bf{k}}}}}}}})}}^{s},$$
(30)

where the band indices m and mσ in Eq. (30) are chosen such that \({\varepsilon }_{m}({{{{{{{\bf{k}}}}}}}})=p\ {\varepsilon }_{{m}_{\sigma }}({O}_{\sigma }{{{{{{{\bf{k}}}}}}}})\). Detailed derivation of Eqs. (29) and (30) and comments on the degenerate bands can be found in Supplementary Note 2. From equation (29), we obtain two symmetries that give vanishing modified band dispersion, En,B(k) = 0: \({{\mathfrak{g}}}_{C}=({{\mathbb{1}}}_{d},0,-1)\) and \({{\mathfrak{g}}}_{{I}_{{{{{{{{\rm{ST}}}}}}}}}}=({{\mathbb{1}}}_{d},1,1)\) which correspond to chiral symmetry C and space–time-inversion symmetry IST, respectively. On the other hand, when \({(-1)}^{s}p\ {{{{{{{\rm{Det}}}}}}}}{O}_{\sigma }=-1\) and \({{{{{{{\rm{Det}}}}}}}}{O}_{\sigma }\ne {\mathbb{1}}\), the modified band dispersion satisfies En,B(Oσk) = −En,B(k), which implies \(\max \ {E}_{n,B}({{{{{{{\bf{k}}}}}}}})=-\min \ {E}_{n,B}({{{{{{{\bf{k}}}}}}}})\). Time-reversal T and reflection R symmetries belong to this case. Also, the contribution to the En,B(k) from each band via the inter-band coupling in Eq. (5) can be systematically understood by using equation (30) (see Supplementary Note 2 for details).

Calculation scheme for the Landau levels

We calculate the Hofstadter spectrum by numerically implementing the Peierls substitution to the tight-binding Hamiltonian29.

Calculation of Landau fan diagram including disorder

To obtain the Landau fan diagram including disorder effect, we study a finite-size SOC Lieb model HsocL(k) composed of 40 by 40 unit cells. Disorder is introduced by the Hamiltonian Hdis with components \({\left({H}_{{{{{{{{\rm{dis}}}}}}}}}\right)}_{ij}={w}_{i}{\delta }_{ij}\), where i, j = 1, …, 4800 denotes the unit cell index and wi [−W/2,W/2] follows a uniform probability distribution. By diagonalizing the disordered Hamiltonian \({N}_{{{{{{{{\rm{itr}}}}}}}}}=200\) times and averaging the results, the density of states (DOS) of Landau levels is obtained. Note that chiral edge states are found in the gap between flat and dispersive bands. It is because the two dispersive bands in the SOC Lieb model have the Chern number ±1, respectively depending on the sign of spin–orbit coupling, despite the topologically trivial middle flat band. However, the contribution of edge states to DOS is quantitatively negligible.

Data availability

The data that support the findings of this study are available from the corresponding authors upon reasonable request.

Code availability

The numerical codes used in this paper are available from the corresponding authors upon reasonable request.

References

  1. Onsager, L. Interpretation of the de Haas–van Alphen effect. Lond. Edinb. Dublin Philos. Mag. J. Sci. 43, 1006–1008 (1952).

    Article  Google Scholar 

  2. Roth, L. M. Semiclassical theory of magnetic energy levels and magnetic susceptibility of Bloch electrons. Phys. Rev. 145, 434 (1966).

    ADS  CAS  Article  Google Scholar 

  3. Mikitik, G. & Sharlai, Y. V. Manifestation of Berry’s phase in metal physics. Phys. Rev. Lett. 82, 2147 (1999).

    ADS  CAS  Article  Google Scholar 

  4. Gao, Y. & Niu, Q. Zero-field magnetic response functions in Landau levels. Proc. Natl Acad. Sci. USA 114, 7295–7300 (2017).

    ADS  CAS  PubMed  PubMed Central  Article  Google Scholar 

  5. Fuchs, J.-N., Piéchon, F. & Montambaux, G. Landau levels, response functions and magnetic oscillations from a generalized Onsager relation. SciPost Phys. 4, 024 (2018).

    ADS  Article  Google Scholar 

  6. Zhang, Y., Tan, Y.-W., Stormer, H. L. & Kim, P. Experimental observation of the quantum Hall effect and Berry’s phase in graphene. Nature 438, 201–204 (2005).

    ADS  CAS  PubMed  Article  Google Scholar 

  7. Novoselov, K. S. et al. Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene. Nat. Phys. 2, 177–180 (2006).

    Article  CAS  Google Scholar 

  8. Chang, M.-C. & Niu, Q. Berry phase, hyperorbits, and the Hofstadter spectrum: semiclassical dynamics in magnetic Bloch bands. Phys. Rev. B 53, 7010 (1996).

    ADS  CAS  Article  Google Scholar 

  9. Po, H. C., Watanabe, H. & Vishwanath, A. Fragile topology and Wannier obstructions. Phys. Rev. Lett. 121, 126402 (2018).

    ADS  CAS  PubMed  Article  Google Scholar 

  10. Ahn, J., Park, S. & Yang, B.-J. Failure of Nielsen–Ninomiya theorem and fragile topology in two-dimensional systems with space–time inversion symmetry: application to twisted bilayer graphene at magic angle. Phys. Rev. X 9, 021013 (2019).

    CAS  Google Scholar 

  11. Lian, B., Xie, F. & Bernevig, B. A. Landau level of fragile topology. Phys. Rev. B 102, 041402(R) (2020).

    ADS  Article  Google Scholar 

  12. Rhim, J.-W. & Yang, B.-J. Classification of flat bands according to the band-crossing singularity of Bloch wave functions. Phys. Rev. B 99, 045107 (2019).

    ADS  CAS  Article  Google Scholar 

  13. Ma, J. et al. Direct observation of flatband loop states arising from nontrivial real-space topology. Phys. Rev. Lett. 124, 183901 (2020).

    ADS  CAS  PubMed  Article  Google Scholar 

  14. Rhim, J.-W., Kim, K. & Yang, B.-J. Quantum distance and anomalous Landau levels of flat bands. Nature 584, 59–63 (2020).

    ADS  CAS  PubMed  Article  Google Scholar 

  15. Chen, L., Mazaheri, T., Seidel, A. & Tang, X. The impossibility of exactly flat non-trivial Chern bands in strictly local periodic tight binding models. J. Phys. A 47, 152001 (2014).

    ADS  MATH  Article  Google Scholar 

  16. Read, N. Compactly supported Wannier functions and algebraic K-theory. Phys. Rev. B 95, 115309 (2017).

    ADS  Article  Google Scholar 

  17. Alexandradinata, A. & Höller, J. No-go theorem for topological insulators and high-throughput identification of Chern insulators. Phys. Rev. B 98, 184305 (2018).

    ADS  Article  Google Scholar 

  18. Ma, D.-S. et al. Spin–orbit-induced topological flat bands in line and split graphs of bipartite lattices. Phys. Rev. Lett. 125, 266403 (2020).

    ADS  CAS  PubMed  Article  Google Scholar 

  19. Chiu, C., Ma, D.-S., Song, Z.-D., Bernevig, B. & Houck, A. Fragile topology in line-graph lattices with two, three, or four gapped flat bands. Phys. Rev. Res. 2, 043414 (2020).

    CAS  Article  Google Scholar 

  20. de Juan, F., Grushin, A. G., Morimoto, T. & Moore, J. E. Quantized circular photogalvanic effect in Weyl semimetals. Nat. Commun. 8, 15995 (2017).

    ADS  PubMed  PubMed Central  Article  CAS  Google Scholar 

  21. Bužek, V. & Hillery, M. Quantum copying: beyond the no-cloning theorem. Phys. Rev. A 54, 1844 (1996).

    ADS  MathSciNet  PubMed  Article  Google Scholar 

  22. Dodonov, V., Man’Ko, O., Man’Ko, V. & Wünsche, A. Hilbert-Schmidt distance and non-classicality of states in quantum optics. J. Mod. Opt. 47, 633–654 (2000).

    ADS  MathSciNet  MATH  Article  Google Scholar 

  23. Berry, M. V. The quantum phase, and five years after in Geometric Phases in Physics (ed. Shapere A. and Wilczek F.) 7–28 (World Scientific, 1989).

  24. Provost, J. & Vallee, G. Riemannian structure on manifolds of quantum states. Commun. Math. Phys. 76, 289–301 (1980).

    ADS  MathSciNet  MATH  Article  Google Scholar 

  25. Zanardi, P., Giorda, P. & Cozzini, M. Information-theoretic differential geometry of quantum phase transitions. Phys. Rev. Lett. 99, 100603 (2007).

    ADS  PubMed  MATH  Article  CAS  Google Scholar 

  26. Ma, Y.-Q., Chen, S., Fan, H. & Liu, W.-M. et al. Abelian and non-Abelian quantum geometric tensor. Phys. Rev. B 81, 245129 (2010).

    ADS  Article  CAS  Google Scholar 

  27. Jozsa, R. Fidelity for mixed quantum states. J. Mod. Opt. 41, 2315–2323 (1994).

    ADS  MathSciNet  MATH  Article  Google Scholar 

  28. Goldman, N., Urban, D. & Bercioux, D. Topological phases for fermionic cold atoms on the Lieb lattice. Phys. Rev. A 83, 063601 (2011).

    ADS  Article  CAS  Google Scholar 

  29. Hofstadter, D. R. Energy levels and wave functions of Bloch electrons in rational and irrational magnetic fields. Phys. Rev. B 14, 2239 (1976).

    ADS  CAS  Article  Google Scholar 

  30. Po, H. C., Zou, L., Senthil, T. & Vishwanath, A. Faithful tight-binding models and fragile topology of magic-angle bilayer graphene. Phys. Rev. B 99, 195455 (2019).

    ADS  CAS  Article  Google Scholar 

  31. Tasaki, H. Ferromagnetism in the Hubbard models with degenerate single-electron ground states. Phys. Rev. Lett. 69, 1608 (1992).

    ADS  MathSciNet  CAS  PubMed  MATH  Article  Google Scholar 

  32. Aoki, H., Ando, M. & Matsumura, H. Hofstadter butterflies for flat bands. Phys. Rev. B 54, R17296 (1996).

    ADS  CAS  Article  Google Scholar 

  33. Misumi, T. & Aoki, H. New class of flat-band models on tetragonal and hexagonal lattices: gapped versus crossing flat bands. Phys. Rev. B 96, 155137 (2017).

    ADS  Article  Google Scholar 

  34. Herzog-Arbeitman, J., Song, Z.-D., Regnault, N. & Bernevig, B. A. Hofstadter topology: noncrystalline topological materials at high flux. Phys. Rev. Lett. 125, 236804 (2020).

    ADS  CAS  PubMed  Article  Google Scholar 

  35. Taie, S. et al. Coherent driving and freezing of bosonic matter wave in an optical Lieb lattice. Sci. Adv. 1, e1500854 (2015).

    ADS  PubMed  PubMed Central  Article  CAS  Google Scholar 

  36. Kajiwara, S., Urade, Y., Nakata, Y., Nakanishi, T. & Kitano, M. Observation of a nonradiative flat band for spoof surface plasmons in a metallic Lieb lattice. Phys. Rev. B 93, 075126 (2016).

    ADS  Article  CAS  Google Scholar 

  37. Slot, M. R. et al. Experimental realization and characterization of an electronic Lieb lattice. Nat. Phys. 13, 672–676 (2017).

    CAS  PubMed  PubMed Central  Article  Google Scholar 

  38. Drost, R., Ojanen, T., Harju, A. & Liljeroth, P. Topological states in engineered atomic lattices. Nat. Phys. 13, 668–671 (2017).

    CAS  Article  Google Scholar 

  39. Leykam, D., Andreanov, A. & Flach, S. Artificial flat band systems: from lattice models to experiments. Adv. Phys.: X 3, 1473052 (2018).

    Google Scholar 

  40. Whittaker, C. et al. Exciton polaritons in a two-dimensional Lieb lattice with spin–orbit coupling. Phys. Rev. Lett. 120, 097401 (2018).

    ADS  CAS  PubMed  Article  Google Scholar 

  41. Cui, B. et al. Realization of Lieb lattice in covalent-organic frameworks with tunable topology and magnetism. Nat. Commun. 11, 66 (2020).

    ADS  CAS  PubMed  PubMed Central  Article  Google Scholar 

  42. Vicencio, R. A. et al. Observation of localized states in Lieb photonic lattices. Phys. Rev. Lett. 114, 245503 (2015).

    ADS  PubMed  Article  CAS  Google Scholar 

  43. Baboux, F. et al. Bosonic condensation and disorder-induced localization in a flat band. Phys. Rev. Lett. 116, 066402 (2016).

    ADS  CAS  PubMed  Article  Google Scholar 

  44. Ozawa, T. et al. Topological photonics. Rev. Mod. Phys. 91, 015006 (2019).

    ADS  MathSciNet  CAS  Article  Google Scholar 

  45. Bloch, I. Ultracold quantum gases in optical lattices. Nat. Phys. 1, 23–30 (2005).

    CAS  Article  Google Scholar 

  46. Aidelsburger, M. et al. Experimental realization of strong effective magnetic fields in an optical lattice. Phys. Rev. Lett. 107, 255301 (2011).

    ADS  CAS  PubMed  Article  Google Scholar 

  47. Wu, C., Bergman, D., Balents, L. & Sarma, S. D. Flat bands and wigner crystallization in the honeycomb optical lattice. Phys. Rev. Lett. 99, 070401 (2007).

    ADS  PubMed  Article  CAS  Google Scholar 

  48. Apaja, V., Hyrkäs, M. & Manninen, M. Flat bands, Dirac cones, and atom dynamics in an optical lattice. Phys. Rev. A 82, 041402 (2010).

    ADS  Article  CAS  Google Scholar 

  49. Song, B. et al. Observation of nodal-line semimetal with ultracold fermions in an optical lattice. Nat. Phys. 15, 911–916 (2019).

    CAS  Article  Google Scholar 

  50. Tian, B., Endres, M. & Pekker, D. Landau levels in strained optical lattices. Phys. Rev. Lett. 115, 236803 (2015).

    ADS  PubMed  Article  CAS  Google Scholar 

  51. Ozawa, T. & Price, H. M. Topological quantum matter in synthetic dimensions. Nat. Rev. Phys. 1, 349–357 (2019).

    Article  Google Scholar 

  52. Celi, A. et al. Synthetic gauge fields in synthetic dimensions. Phys. Rev. Lett. 112, 043001 (2014).

    ADS  CAS  PubMed  Article  Google Scholar 

  53. Ozawa, T. & Carusotto, I. Synthetic dimensions with magnetic fields and local interactions in photonic lattices. Phys. Rev. Lett. 118, 013601 (2017).

    ADS  PubMed  Article  Google Scholar 

  54. Ozawa, T. Artificial magnetic field for synthetic quantum matter without dynamical modulation. Phys. Rev. A 103, 033318 (2021).

    ADS  CAS  Article  Google Scholar 

  55. Dutt, A. et al. Experimental band structure spectroscopy along a synthetic dimension. Nat. Commun. 10, 3122 (2019).

    ADS  PubMed  PubMed Central  Article  CAS  Google Scholar 

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Acknowledgements

Y.H. was supported by IBS-R009-D1 and Samsung Science and Technology Foundation under Project Number SSTF-BA2002-06. J.-W.R. was supported by IBS-R009-D1, and the National Research Foundation of Korea (NRF) Grant funded by the Korea government (MSIT) (Grant No. 2021R1A2C1010572). B.-J.Y. was supported by the Institute for Basic Science in Korea (Grant No. IBS-R009-D1), Samsung Science and Technology Foundation under Project Number SSTF-BA2002-06, the National Research Foundation of Korea (NRF) Grant funded by the Korea government (MSIT) (No.2021R1A2C4002773, and No. NRF-2021R1A5A1032996), and the U.S. Army Research Office and Asian Office of Aerospace Research & Development (AOARD) under Grant No. W911NF-18-1-0137.

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Y.H. and J.-W.R. performed theoretical and numerical analyses. B.-J.Y. supervised the project. All authors analysed the data. The manuscript was written by all authors.

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Correspondence to Jun-Won Rhim or Bohm-Jung Yang.

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Hwang, Y., Rhim, JW. & Yang, BJ. Geometric characterization of anomalous Landau levels of isolated flat bands. Nat Commun 12, 6433 (2021). https://doi.org/10.1038/s41467-021-26765-z

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