Abstract
The finger-like branching pattern that occurs when a less viscous fluid displaces a more viscous one confined between two parallel plates has been widely studied as a classical example of a mathematically tractable hydrodynamic instability1,2,3. Fingering in such Hele–Shaw geometries has been generated not only with newtonian fluids4,5,6 but also with various non-newtonian fluids7,8,9 including fine granular material displaced by gas, liquid or larger grains10,11,12,13,14,15. Here, we study a granular Hele–Shaw system to explore the zero-surface-tension property of granular ‘fluids’16. We demonstrate that the grain–gas interface exhibits fractal structure and sharp cusps, which are associated with the hitherto-unrealizable singular hydrodynamics predicted in the zero-surface-tension limit of normal fluid fingering2,17,18,19,20,21,22,23. Above the yield stress, the scaling for the finger width is distinct from that for ordinary fluids, reflecting unique granular properties such as friction-induced dissipation as opposed to viscous damping24,25,26,27. Despite such differences, the dimension of the global fractal structure and the shape of the singular cusps on the interface agree with the theories based on simple laplacian growth of conventional fluid fingering in the zero-surface-tension limit2,17,18,19,20,21,22,23.
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Our granular material consists of spherical glass beads with diameters for separate experiments of: d=54±10 μm, 107±19 μm and 359±61 μm. The material is loaded into a traditional radial Hele–Shaw cell consisting of two 1.9-cm-thick circular glass plates of diameter L. In most experiments, L=50.8 cm, but smaller plates with L=25.3 cm and 17.5 cm are also used. The gap between the plates, b, is uniform and in different experiments was varied between 0.25 mm and 1.14 mm. The two plates are maintained at a fixed gap with spacers and clamps around the perimeter. The granular material driven by the displacing gas can flow freely out of the cell boundary. The system was vibrated so that the material between the plates was uniformly dense with a packing fraction near that of random close-packing. To drive off any humidity, which can cause cohesion between particles, the beads are baked under vacuum before use. We estimated the cohesive force between beads from the angle of the repose of the material28. The ratio between the cohesive force and the weight of beads is 6.9% for 54 μm beads and 3.5% for 107 μm beads. By calculating the surplus surface energy resulting from this cohesive force, we find that the effective surface tension of the granular material is about 10−6 mJ m−2 for both 54 μm and 107 μm beads, which is seven orders of magnitude smaller than that of normal fluids such as water (72.8 mJ m−2) or ethyl alcohol (22.3 mJ m−2).
Pressurized nitrogen, with pressure ΔP higher than ambient pressure, is blown through a 2 mm hole in the centre of the bottom plate. The patterns formed are recorded by a high-speed camera (Phantom V7.1) at 2,000 frames per second or by a high-resolution still camera. To study the dynamics of granular fingering near the yield stress of the granular material, corresponding to a threshold pressure ΔPth, we also conducted our experiment under small constant flow rate conditions using a syringe pushed by a speed-controlled motor. With a flow rate of 22.9±0.1 ml s−1 at the smallest gap thickness used, b=0.25 mm, this covered 0.04% of the entire plate area per second. The patterns grow by stick–slip motion. When the gas pressure is above ΔPth, patterns grow leading to a drop in pressure so that finger growth halts. Then the gas pressure builds up until the fingers resume their expansion. This method forces the pattern to grow under conditions such that the pressure is always close to ΔPth.
Figure 1a,b shows viscous fingering patterns in the granular Hele–Shaw experiments. The shape and dynamics of the pattern depend on the driving pressure, ΔP. When below the yield stress, patterns do not form. Above the yield stress, there are two stages of growth that can be seen by measuring the size of the fastest moving finger. In the early stage, the finger grows at a slow, approximately constant, speed as seen in Fig. 1c. In this regime, shown in Fig. 1a, we can see a pattern similar to those in fluids. In the late stage, shown in Fig. 1b, possibly influenced by the boundary, the growth is accelerated and the patterns grow wildly. In this regime, we see the merging of fingers and the pinch-off of fingers from the main structure. Such phenomena are rare in fluid fingering. Figure 1c shows that the two stages are connected by a sharp kink at low ΔP that becomes smoother as the pressure increases. We focus here on the patterns in the early stage.
Figure 2a–c shows the patterns of fingers at different ΔP. The patterns are sharper and more ramified at low pressure and become smoother and more circular at high pressure. This is opposite to what happens in newtonian fluids where the width of a finger, W, depends on the capillary number Ca as
where σ is the surface tension acting across an interface, η is the viscosity of the more viscous fluid (ignoring the viscosity of the less viscous fluid as it is usually much smaller) and V is the local interface velocity2,5. The competition between viscous forces, which narrows fingers to a singular point, and surface tension, which blunts sharp structures in the interface, determines the characteristic length scale of the pattern. Hence, decreasing the driving pressure, which slows down pattern growth, results in blunter patterns in fluid fingering6.
As in newtonian fluid fingering, granular fingering grows through tip-splitting instead of side-branching2. However, rather than exhibiting an obvious characteristic length scale as found in fluids, the granular fingers widen during growth. To quantify the growth, we define the characteristic width of our pattern, W, as the width of fingers just before splitting, as shown in the lower inset of Fig. 2d. We measure W versus the local interface velocity, V, at the tip of fingers for systems with different gap thickness, b, and plate diameter, L, and with different granular material density ρ and size d. The results of these studies are shown in the upper inset of Fig. 2d. As shown, higher velocities produce wider fingers. The main panel of Fig. 2d shows that we can collapse all data onto a single curve with a scaling W∼(V L d)1/2ρ1/4. Compared with the scaling of classical fluid fingering, equation (1), the width of granular fingers grows as V1/2 rather than decreasing as V−1/2 and it is independent of the gap thickness b. Furthermore, the parameters of the granular particles themselves, the size and density of the beads, enter the scaling.
To quantify global features of patterns at different ΔP, we calculate their fractal dimension by measuring the number of boxes, N, needed to cover the entire pattern, as a function of the size of the box, l. The analysed patterns are taken from the end of the early stage. We find that the dimension of patterns, D, defined as the power of N∼lD, is limited between that of a circle, D=2, and that of a diffusion-limit-aggregation (DLA) pattern29, D=1.70±0.02.
In the zero-surface-tension limit, viscous fingering patterns are predicted to have the same fractal dimension as DLA (refs 2, 7, 18, 19). As we decrease the driving pressure towards the threshold pressure, ΔPth, we find that D approaches the exponent characteristic of DLA. This suggests that granular fingering may only show the zero-surface-tension-fluid behaviour or the anticipated singularity near the threshold pressure, ΔPth. To investigate this regime in detail, we conducted a constant flow rate experiment as described above. The fractal dimension of the resulting pattern (D=1.68±0.02) indeed overlaps with that of DLA as seen in Fig. 3a.
We can also focus on a small region along the interface and observe cusp formation as seen in the upper inset of Fig. 3b. These cusp tips can be sharp down to the grain level. Cusp formation occurs just before each finger starts to grow. These cusps are sharp and different from any structures found in newtonian fluids where the finger tips are always round owing to surface tension4,5,6. Theory based on the laplacian growth of conventional fluid fingering in the zero-surface-tension limit suggests2,17,21,22,23 that the shape of the profile at the singularity should scale as y=A(x−x0)3/2, where A is a free parameter and x=x0 is the position of the singularity. We can collapse the experimental profiles at the time when they are sharpest, onto a single master curve: y=A(x−x0)β with β=1.43±0.20 as shown in Fig. 3b. Although the β=3/2 scaling was not derived with dense granular fluids in mind, it is consistent with our granular results at the instant of cusp formation. The lower inset of Fig. 3b shows the time evolution of an individual cusp. However, owing to the stick–slip motion of the interface and to the rapid movement of the finger tips, we cannot resolve the time scaling of the tip velocity.
Because of the absence of surface tension and the irrelevance of thermal energy in granular material, the interfacial patterns formed in our system do not relax when we turn off the driving pressure. Without mechanical perturbation, patterns such as those shown in Fig. 2 retain their sharp structure. Hence, our system provides an opportunity to study the steady-state structure of the patterns. This is in contrast to other systems where surface tension and thermal diffusion always smooth out the interface30.
Theoretically, it has been known that fluid fingering in the zero-surface-tension limit would lead to singular cusp structure locally and DLA fractal geometry globally2,17,18,19,20,21,22,23. Nevertheless, the connection between the local singular dynamics and global fractal shape remains far from clear. Despite its unique properties such as compressibility, permeability to gas and interparticle friction, granular flow nevertheless provides the first experimental evidence for the coexistence of these two singular features and shows how the local cusps evolve into a global fractal. Surprisingly, theories based on the hydrodynamics of normal fluids give a good description of the singularity formation observed here in the two-phase dense granular flow. However, we note that the particle diameter, d, enters the scaling of granular fingers as an important parameter. Without surface tension to provide a scale to regularize the singularity, the grain diameter may provide that scale.
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Acknowledgements
We thank E. Bettelheim, E. Corwin, S. Y. Lee, J. Royer, P. Wiegmann and L. N. Zou for fruitful discussions. This work was supported by the MRSEC program of the NSF under No. DMR-0213745 and by the W. M. Keck Foundation.
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Cheng, X., Xu, L., Patterson, A. et al. Towards the zero-surface-tension limit in granular fingering instability. Nature Phys 4, 234–237 (2008). https://doi.org/10.1038/nphys834
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DOI: https://doi.org/10.1038/nphys834
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