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Phonon scattering inhibits simultaneous near-unity efficiency and indistinguishability in semiconductor single-photon sources

Abstract

Semiconductor quantum dots (QDs) have recently emerged as a leading platform to generate highly indistinguishable photons efficiently, and this work addresses the timely question of how good these solid-state sources can ultimately be. We establish the crucial role of lattice relaxation in these systems in giving rise to trade-offs between indistinguishability and efficiency. We analyse the two source architectures most commonly employed: a QD embedded in a waveguide and a QD coupled to an optical cavity. For waveguides, we demonstrate that the broadband Purcell effect results in a simple inverse relationship, in which indistinguishability and efficiency cannot be simultaneously increased. For cavities, the frequency selectivity of the Purcell enhancement results in a more subtle trade-off, in which indistinguishability and efficiency can be increased simultaneously, although not arbitrarily, which limits a source with near-unity indistinguishability (>99%) to an efficiency of approximately 96% for realistic parameters.

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Figure 1: Lattice relaxation in QDs and the phonon SB.
Figure 2: Single-photon source architectures and emission spectra.
Figure 3: Indistinguishability and efficiency of the three source set-ups shown in Fig. 2.

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Acknowledgements

The authors thank N. Gregersen for useful discussions. J.I.-S. and J.M. acknowledge support from the Danish Research Council (DFF-4181-00416) and Villum Fonden (NATEC Centre, grant 8692). A.N. is supported by the University of Manchester and the Engineering and Physical Sciences Research Council, grant number EP/N008154/1. This project has received funding from the European Union's Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie grant agreement no. 703193.

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Correspondence to Jake Iles-Smith.

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Iles-Smith, J., McCutcheon, D., Nazir, A. et al. Phonon scattering inhibits simultaneous near-unity efficiency and indistinguishability in semiconductor single-photon sources. Nature Photon 11, 521–526 (2017). https://doi.org/10.1038/nphoton.2017.101

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