Abstract
Monolayer transition-metal dichalcogenides (TMDs) have the potential to become efficient optical-gain materials for low-energy-consumption nanolasers with the smallest gain media because of strong excitonic emission. However, until now TMD-based lasing has been realized only at low temperatures. Here we demonstrate for the first time a room-temperature laser operation in the infrared region from a monolayer of molybdenum ditelluride on a silicon photonic-crystal cavity. The observation is enabled by the unique combination of a TMD monolayer with an emission wavelength transparent to silicon, and a high-Q cavity of the silicon nanobeam. The laser is pumped by a continuous-wave excitation, with a threshold density of 6.6 W cm–2. Its linewidth is as narrow as 0.202 nm with a corresponding Q of 5,603, the largest value reported for a TMD laser. This demonstration establishes TMDs as practical materials for integrated TMD–silicon nanolasers suitable for silicon-based nanophotonic applications in silicon-transparent wavelengths.
This is a preview of subscription content, access via your institution
Relevant articles
Open Access articles citing this article.
-
Prolonging valley polarization lifetime through gate-controlled exciton-to-trion conversion in monolayer molybdenum ditelluride
Nature Communications Open Access 14 July 2022
-
Continuous-wave upconversion lasing with a sub-10 W cm−2 threshold enabled by atomic disorder in the host matrix
Nature Communications Open Access 21 July 2021
-
Ten years of spasers and plasmonic nanolasers
Light: Science & Applications Open Access 25 May 2020
Access options
Access Nature and 54 other Nature Portfolio journals
Get Nature+, our best-value online-access subscription
$29.99 / 30 days
cancel any time
Subscribe to this journal
Receive 12 print issues and online access
$259.00 per year
only $21.58 per issue
Rent or buy this article
Get just this article for as long as you need it
$39.95
Prices may be subject to local taxes which are calculated during checkout




References
Wu, S. et al. Monolayer semiconductor nanocavity lasers with ultralow thresholds. Nature 520, 69–72 (2015).
Ye, Y. et al. Monolayer excitonic laser. Nat. Photon. 9, 733–737 (2015).
Withers, F. et al. Light-emitting diodes by band-structure engineering in van der Waals heterostructures. Nat. Mater. 14, 301–306 (2015).
Ross, J. S. et al. Electrically tunable excitonic light-emitting diodes based on monolayer WSe2 p–n junctions. Nat. Nanotech. 9, 268–272 (2014).
Mak, K. F., Lee, C., Hone, J., Shan, J. & Heinz, T. F. Atomically thin MoS2: a new direct-gap semiconductor. Phys. Rev. Lett. 105, 136805 (2010).
Splendiani, A. et al. Emerging photoluminescence in monolayer MoS2 . Nano Lett. 10, 1271–1275 (2010).
Chernikov, A. et al. Exciton binding energy and nonhydrogenic Rydberg series in monolayer WS2 . Phys. Rev. Lett. 113, 076802 (2014).
Ugeda, M. M. et al. Giant bandgap renormalization and excitonic effects in a monolayer transition metal dichalcogenide semiconductor. Nat. Mater. 13, 1091–1095 (2014).
Yang, J. et al. Robust excitons and trions in monolayer MoTe2 . ACS Nano 9, 6603–6609 (2015).
He, K. et al. Tightly bound excitons in monolayer WSe2 . Phys. Rev. Lett. 113, 026803 (2014).
Noginov, M. A. et al. Demonstration of a spaser-based nanolaser. Nature 460, 1110–1112 (2009).
Hill, M. T. et al. Lasing in metallic-coated nanocavities. Nat. Photon. 1, 589–594 (2007).
Oulton, R. F. et al. Plasmon lasers at deep subwavelength scale. Nature 461, 629–632 (2009).
Ding, K. et al. Room-temperature continuous wave lasing in deep-subwavelength metallic cavities under electrical injection. Phys. Rev. B 85, 041301 (2012).
Ding, K. et al. Record performance of electrical injection sub-wavelength metallic-cavity semiconductor lasers at room temperature. Opt. Express 21, 4728–4733 (2013).
Nezhad, M. P. et al. Room-temperature subwavelength metallo-dielectric lasers. Nat. Photon. 4, 395–399 (2010).
Huang, M. H. et al. Room-temperature ultraviolet nanowire nanolasers. Science 292, 1897–1899 (2001).
Lu, Y.-J. et al. Plasmonic nanolaser using epitaxially grown silver film. Science 337, 450–453 (2012).
Ning, C. Z. Semiconductor nanolasers. Phys. Status Solidi B 247, 774–788 (2010).
Jeong, K.-Y. et al. Electrically driven nanobeam laser. Nat. Commun. 4, 2822 (2013).
Ding, K., Diaz, J. O., Bimberg, D. & Ning, C. Z. Modulation bandwidth and energy efficiency of metallic cavity semiconductor nanolasers with inclusion of noise effects. Laser Photon. Rev. 9, 488–497 (2015).
Salehzadeh, O., Djavid, M., Tran, N. H., Shih, I. & Mi, Z. Optically pumped two-dimensional MoS2 lasers operating at room-temperature. Nano Lett. 15, 5302–5306 (2015).
Reed, J. C., Zhu, A. Y., Zhu, H., Yi, F. & Cubukcu, E. Wavelength tunable microdisk cavity light source with a chemically enhanced MoS2 emitter. Nano Lett. 15, 1967–1971 (2015).
Deotare, P. B., McCutcheon, M. W., Frank, I. W., Khan, M. & Lončar, M. High quality factor photonic crystal nanobeam cavities. Appl. Phys. Lett. 94, 121106 (2009).
Ramasubramaniam, A. Large excitonic effects in monolayers of molybdenum and tungsten dichalcogenides. Phys. Rev. B 86, 115409 (2012).
Ruppert, C., Aslan, O. B. & Heinz, T. F. Optical properties and band gap of single- and few-layer MoTe2 crystals. Nano Lett. 14, 6231–6236 (2014).
Green, M. A. & Keevers, M. J. Optical properties of intrinsic silicon at 300 K. Prog. Photovolt. Res. Appl. 3, 189–192 (1995).
Hull, R. Properties of Crystalline Silicon (IET, 1999).
John, S. Strong localization of photons in certain disordered dielectric superlattices. Phys. Rev. Lett. 58, 2486–2489 (1987).
Yablonovitch, E. Inhibited spontaneous emission in solid-state physics and electronics. Phys. Rev. Lett. 58, 2059–2062 (1987).
Foresi, J. S. et al. Photonic-bandgap microcavities in optical waveguides. Nature 390, 143–145 (1997).
Notomi, M., Kuramochi, E. & Taniyama, H. Ultrahigh-Q nanocavity with 1D photonic gap. Opt. Express 16, 11095–11102 (2008).
M. d Zain, A. R., Johnson, N. P., Sorel, M. & De La Rue, R. M. Design and fabrication of high quality-factor 1-D photonic crystal/photonic wire extended microcavities. IEEE Photon. Technol. Lett. 22, 610–612 (2010).
Koirala, S., Mouri, S., Miyauchi, Y. & Matsuda, K. Homogeneous linewidth broadening and exciton dephasing mechanism in MoTe2 . Phys. Rev. B 93, 075411 (2016).
Ning, C. Z. What is laser threshold? IEEE J. Sel. Top. Quantum Electron. 19, 1503604 (2013).
Soref, R. & Bennett, B. Electrooptical effects in silicon. IEEE J. Quantum Electron. 23, 123–129 (1987).
Christmann, G., Butté, R., Feltin, E., Carlin, J.-F. & Grandjean, N. Room temperature polariton lasing in a GaN∕AlGaN multiple quantum well microcavity. Appl. Phys. Lett. 93, 051102 (2008).
Acknowledgements
This research is supported by the 985 University Project of China and Tsinghua University Initiative Scientific Research Program (No. 20141081296). The authors thank Y. Huang for the usage of their fabrication equipment.
Author information
Authors and Affiliations
Contributions
C.Z.N. initiated the research on the silicon-based monolayer MoTe2 lasers, and supervised the overall project. Y.L. developed the simulations and design of the devices. Y.L., J.Z., D.H. and J.F. exfoliated monolayer MoTe2 from the bulk material. Y.L., J.Z. and D.H. fabricated the devices. Y.L., J.Z., H.S. and F.F. performed the optical measurements and data analysis. J.Z. and Z.W. carried out the laser equation fitting. Y.L. and C.Z.N. analysed data and wrote the manuscript. All the authors participated in the discussions.
Corresponding author
Ethics declarations
Competing interests
The authors declare no competing financial interests.
Supplementary information
Supplementary information
Supplementary information (PDF 1204 kb)
Rights and permissions
About this article
Cite this article
Li, Y., Zhang, J., Huang, D. et al. Room-temperature continuous-wave lasing from monolayer molybdenum ditelluride integrated with a silicon nanobeam cavity. Nature Nanotech 12, 987–992 (2017). https://doi.org/10.1038/nnano.2017.128
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1038/nnano.2017.128
This article is cited by
-
Photonic van der Waals integration from 2D materials to 3D nanomembranes
Nature Reviews Materials (2023)
-
Prolonging valley polarization lifetime through gate-controlled exciton-to-trion conversion in monolayer molybdenum ditelluride
Nature Communications (2022)
-
Room-temperature continuous-wave indirect-bandgap transition lasing in an ultra-thin WS2 disk
Nature Photonics (2022)
-
Continuous-wave upconversion lasing with a sub-10 W cm−2 threshold enabled by atomic disorder in the host matrix
Nature Communications (2021)
-
Strong exciton-photon interaction and lasing of two-dimensional transition metal dichalcogenide semiconductors
Nano Research (2021)