Letter

Emergent dynamic chirality in a thermally driven artificial spin ratchet

Received:
Accepted:
Published online:

Abstract

Modern nanofabrication techniques have opened the possibility to create novel functional materials, whose properties transcend those of their constituent elements. In particular, tuning the magnetostatic interactions in geometrically frustrated arrangements of nanoelements called artificial spin ice1,2 can lead to specific collective behaviour3, including emergent magnetic monopoles4,5, charge screening6,7 and transport8,9, as well as magnonic response10,11,12. Here, we demonstrate a spin-ice-based active material in which energy is converted into unidirectional dynamics. Using X-ray photoemission electron microscopy we show that the collective rotation of the average magnetization proceeds in a unique sense during thermal relaxation. Our simulations demonstrate that this emergent chiral behaviour is driven by the topology of the magnetostatic field at the edges of the nanomagnet array, resulting in an asymmetric energy landscape. In addition, a bias field can be used to modify the sense of rotation of the average magnetization. This opens the possibility of implementing a magnetic Brownian ratchet13,14, which may find applications in novel nanoscale devices, such as magnetic nanomotors, actuators, sensors or memory cells.

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Acknowledgements

The authors thank O. Sendetskyi, H. Arava, V. Guzenko, E. Deckardt and J. Bosgra for technical assistance. S.G. wishes to thank N. Leo and A. S. Arrott for helpful discussions as well as S. Arnold for advice on the graphics in the manuscript. R.L.S. thanks F. Nascimento for discussions. S.G. was funded by the European Union’s Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie grant agreement no. 708674. The work of G.H. was supported by the EPSRC (grants EP/M015173/1 and EP/L019876/1), the Vienna Science and Technology Fund under WWTF Project MA14-44 and the Royal Society under Grant No. UF080837. The work of R.L.S. was supported by the EPSRC (grants EP/ L002922/1 and EP/M024423/1). This work was supported by JSPS Core-to-Core Program, A. Advanced Research Networks. A.F. was supported by the Swiss National Science Foundation. Part of this work was performed at the Surface/Interface: Microscopy (SIM) beamline of the Swiss Light Source, Paul Scherrer Institut, Villigen, Switzerland. This research used resources of the Advanced Light Source, which is a DOE Office of Science User Facility under contract no. DE-AC02-05CH11231. Use of the Center for Nanoscale Materials, an Office of Science user facility, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357.

Author information

Affiliations

  1. SUPA, School of Physics and Astronomy, University of Glasgow, Glasgow G12 8QQ, UK

    • Sebastian Gliga
    •  & Robert L. Stamps
  2. Laboratory for Mesoscopic Systems, Department of Materials, ETH Zurich, 8093 Zurich, Switzerland

    • Sebastian Gliga
    • , Claire Donnelly
    • , Jonathan Büchi
    • , Jizhai Cui
    • , Alan Farhan
    • , Eugenie Kirk
    • , Nicholas S. Bingham
    •  & Laura J. Heyderman
  3. Paul Scherrer Institut, 5232 Villigen PSI, Switzerland

    • Sebastian Gliga
    • , Claire Donnelly
    • , Armin Kleibert
    • , Jizhai Cui
    • , Alan Farhan
    • , Eugenie Kirk
    • , Nicholas S. Bingham
    •  & Laura J. Heyderman
  4. College of Engineering, Mathematics and Physical Sciences, University of Exeter, Exeter EX4 4QF, UK

    • Gino Hrkac
  5. Advanced Light Source, Lawrence Berkeley National Laboratory (LBNL), 1 Cyclotron Road, Berkeley, California 94720, USA

    • Alan Farhan
    •  & Andreas Scholl
  6. Department of Materials Science and Engineering, University of California, Davis, Davis, California 95616, USA

    • Rajesh V. Chopdekar
  7. Department of Physics, University of Tokyo, Tokyo 113-0033, Japan

    • Yusuke Masaki
  8. National Research Council Research Associate at the US Naval Research Laboratory, 4555 Overlook Avenue, SW Washington DC 20375, USA

    • Nicholas S. Bingham

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Contributions

R.L.S. and S.G. conceived the spin ice geometry and the experiment. S.G., A.F., C.D. and J.C. prepared the samples. S.G., C.D., J.C., J.B., A.K., A.F., R.V.C., E.K., A.S. and N.S.B. performed the experiments and analysed the experimental data. G.H., S.G. and J.B. performed and evaluated the micromagnetic simulations. S.G., G.H., R.L.S., J.B., C.D., A.K., Y.M. and L.J.H. interpreted the results. S.G. wrote the manuscript with input from all coauthors. All authors discussed the results and commented on the manuscript.

Competing interests

The authors declare no competing financial interests.

Corresponding author

Correspondence to Sebastian Gliga.

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