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Direct creation of three-dimensional photonic crystals by a top-down approach

Abstract

Three-dimensional (3D) photonic crystals1,2,3,4,5,6,7,8,9,10,11 can block photons in any direction and are expected to make possible their ultimate control. However, creating 3D crystals without any unintentional defects over large areas at optical wavelengths has been challenging. For example, opal-based crystals7,8,9,10 inevitably contain unintentional defects, it is difficult to increase the sizes of micro-manipulated crystals6 over 6 μm and producing stacked 3D crystals with thin 2D layers2,3,4,5,6 requires complicated and time-consuming processes. So far, these difficulties have hindered 3D photonic-crystal research. Here, we demonstrate a novel top–down approach to creating 3D crystals that overcomes these difficulties and significantly simplifies the process. We have developed a double-angled deep-etching method, which enables the direct creation of 3D woodpile crystals in single-crystalline silicon. A strong photonic bandgap effect with >20 dB attenuation in all directions has been achieved. Furthermore, bonding a light emitter onto or between 3D crystals created in this way has been shown to enhance or suppress spontaneous emission.

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Figure 1: Top–down method of fabrication and fabrication tolerance.
Figure 2: Calculated space-charge and potential distribution inside the ion sheath during the RIE process and the resultant ion trajectory (or etching direction).
Figure 3: Fabricated 3D photonic crystals and optical properties.
Figure 4: Spontaneous emission control by fabricated 3D photonic crystals.

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References

  1. Yablonovitch, E. Inhibited spontaneous emission in solid-state physics and electronics. Phys. Rev. Lett. 58, 2059–2062 (1987).

    Article  CAS  Google Scholar 

  2. Noda, S., Tomoda, K., Yamamoto, N. & Chutinan, A. Full three-dimensional photonic bandgap crystals at near-infrared wavelengths. Science 289, 604–606 (2000).

    Article  CAS  Google Scholar 

  3. Ogawa, S., Imada, M., Yoshimoto, S., Okano, M. & Noda, S. Control of light emission by 3D photonic crystals. Science 305, 227–229 (2004).

    Article  CAS  Google Scholar 

  4. Fleming, J. G. & Lin, S. Y. Three-dimensional photonic crystal with a stop band from 1.35 to 1.95 μm. Opt. Lett. 24, 49–51 (1999).

    Article  CAS  Google Scholar 

  5. Qi, M. et al. A three-dimensional optical photonic crystal with designed point defects. Nature 429, 538–542 (2004).

    Article  CAS  Google Scholar 

  6. Aoki, K. et al. Coupling of quantum-dot light emission with a three-dimensional photonic-crystal nanocavity. Nature Photon. 2, 688–692 (2008).

    Article  CAS  Google Scholar 

  7. Blanco, A. et al. Large-scale synthesis of a silicon photonic crystal with a complete three-dimensional bandgap near 1.5 micrometres. Nature 405, 437–440 (2000).

    Article  CAS  Google Scholar 

  8. Vlasov, Y. A., Bo, X. Z., Sturm, J. C. & Norris, D. J. On-chip natural assembly of silicon photonic bandgap crystals. Nature 414, 289–293 (2001).

    Article  CAS  Google Scholar 

  9. Lodahl, P. et al. Controlling the dynamics of spontaneous emission from quantum dots by photonic crystals. Nature 430, 654–657 (2004).

    Article  CAS  Google Scholar 

  10. Rinne, S. A., García-Santamaría, F. & Braun, P. V. Embedded cavities and waveguides in three-dimensional silicon photonic crystals. Nature Photon. 2, 52–56 (2008).

    Article  CAS  Google Scholar 

  11. Ramanan, V., Nelson, E., Brzezinski, A., Braun, P. V. & Wiltzius, P. Three dimensional silicon-air photonic crystals with controlled defects using interference lithography. Appl. Phys. Lett. 92, 173304 (2008).

    Article  Google Scholar 

  12. Cheng, C. C., Arbet-Engels, V., Scherer, A. & Yablonovitch, E. Nanofabricated three dimensional photonic crystals operating at optical wavelengths. Phys. Scr. T68, 17–20 (1996).

    CAS  Google Scholar 

  13. Chelnokov, A. et al. Fabrication of 2-D and 3-D silicon photonic crystals by deep etching. IEEE J. Sel. Top. Quant. 8, 919–927 (2002).

    Article  CAS  Google Scholar 

  14. Schilling, J. et al. Three-dimensional macroporous silicon photonic crystal with large photonic band gap. Appl. Phys. Lett. 86, 011101 (2005).

    Article  Google Scholar 

  15. Takahashi, S., Okano, M., Imada, M. & Noda, S. Three-dimensional photonic crystals based on double-angled etching and wafer-fusion techniques. Appl. Phys. Lett. 89, 123106 (2006).

    Article  Google Scholar 

  16. Tjerkstra, R. W., Segerink, F. B., Kelly, J. J. & Vos, W. L. Fabrication of three-dimensional nanostructures by focused ion beam milling. J. Vac. Sci. Technol. B 26, 973–977 (2008).

    Article  CAS  Google Scholar 

  17. Toader, O., Berciu, M. & John, S. Photonic band gaps based on tetragonal lattices of slanted pores. Phys. Rev. Lett. 90, 233901 (2003).

    Article  Google Scholar 

  18. Chutinan, A. & Noda, S. Effects of structural fluctuations on the photonic bandgap during fabrication of a photonic crystal. J. Opt. Soc. Am. B 16, 240–244 (1999).

    Article  CAS  Google Scholar 

  19. Ishizaki, K., Okano, M. & Noda, S. Numerical investigation of emission in finite-sized three-dimensional photonic crystals with structural fluctuations. J. Opt. Soc. Am. B 26, 1157–1161 (2009).

    Article  CAS  Google Scholar 

  20. Fang, A. W. et al. Electrically pumped hybrid AlGaInAs–silicon evanescent laser. Opt. Express 14, 9203–9210 (2006).

    Article  CAS  Google Scholar 

Download references

Acknowledgements

This work was supported in part by ‘Global Centre of Excellence for Education and Research on Photonics and Electronics Science and Engineering’, which is one of the education and research programs of the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan.

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Authors and Affiliations

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Contributions

S.N. proposed the concept of the double-angled etching based on an ion-sheath control plate and supervised the whole project. S.T. developed the method of the self-consistent ion-trajectory analysis to find the most appropriate structures of the ion-sheath control plate. S.T. along with M.I. developed experimental conditions to realize the double-angled etching. M.O. and S.T. calculated the band structure, transmission and reflection spectra of the 3D crystals based on the double-angled etching. K.S. along with T.N and K.I. developed the bonding and thinning process of the very thin quantum well onto and between the 3D photonic crystals. S.T., K.S., T.N. and Y.O carried out optical measurements. S.N., S.T. and K.S. worked together to write the manuscript.

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Correspondence to Susumu Noda.

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Takahashi, S., Suzuki, K., Okano, M. et al. Direct creation of three-dimensional photonic crystals by a top-down approach. Nature Mater 8, 721–725 (2009). https://doi.org/10.1038/nmat2507

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