Abstract
When Einstein showed that light amplification needed a collection of atoms in ‘population inversion’ (that is, where more than half the atoms are in an excited state, ready to emit light rather than absorb it) he was using thermodynamic arguments1. Later on, quantum theory predicted2,3 that matter–wave interference effects inside the atoms could, in principle, allow gain without inversion (GWI). The coherent conditions needed to observe this strange effect have been generated in atomic vapours4, but here we show that semiconductor nanostructures can be tailored to have ‘artificial atom’ electron states which, for the first time in a solid, also show GWI. In atomic experiments, the coherent conditions, typically generated either by coupling two electron levels to a third with a strong light beam2,3 or by tunnel coupling both levels to the same continuum (Fano effect5), are also responsible for the observation of ‘electromagnetically induced transparency’ (EIT)6. In turn, this has allowed observations of markedly slowed7 and even frozen8 light propagation. Our ‘artificial atom’ GWI effects are rooted in the same phenomena and, from an analysis of the absorption changes, we infer that the light slows to ∼c/40 over the spectral range where the optical gain appears.
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References
Einstein, A. The quantum theory of radiation. Phys. Z. 18, 121–128 (1917).
Scully, M. O. & Zubairy, M. S. Quantum Optics (Cambridge Univ. Press, Cambridge, 1997).
Mandel, L. & Wolf, E. Optical Coherence and Quantum Optics (Cambridge Univ. Press, Cambridge, 1995).
Mompart, J. & Corbalan, R. Lasing without inversion. J. Opt. B 2, R7–R24 (2000).
Harris, S. E. Lasers without inversion: Interference of lifetime broadened resonances. Phys. Rev. Lett. 62, 1033–1036 (1989).
Boller, K.-J., Imamoǧlu, A. & Harris, S. E. Observation of electromagnetically induced transparency. Phys. Rev. Lett. 66, 2954–2956 (1991).
Hau, L. W., Harris, S. E., Dutton, Z. & Behroozi, C. H. Light speed reduction to 17 metres per second in an ultracold atomic gas. Nature 397, 594–598 (1999).
Bajcsy, M., Zibrov, A. S. & Lukin, M. D. Stationary pulses of light in an atomic medium. Nature 426, 638–641 (2003).
Berman, P. R. & Salomaa, R. Comparison between dressed-atom and bare-atom pictures in laser spectroscopy. Phys. Rev. A 25, 2667–2692 (1982).
Wu, F. Y., Ezekiel, E., Ducloy, M. & Mollow, B. R. Observation of amplification in a strongly driven two-level atomic system at optical frequencies. Phys. Rev. Lett. 38, 1077–1080 (1977).
Luo, C. W. et al. Phase resolved non-linear response of a two dimensional electron gas under femtosecond intersubband excitation. Phys. Rev. Lett. 92, 047402 (2004).
Dynes, J. F., Frogley, M. D., Beck, M., Faist, J. & Phillips, C. C. AC stark splitting and quantum interference with intersubband transitions in quantum wells. Phys. Rev. Lett. 94, 157403 (2005).
Turukhin, A. V. et al. Observation of ultraslow and stored light pulses in a solid. Phys. Rev. Lett. 88, 023602 (2002).
Bigelow, M. S., Lepeshkin, N. N. & Boyd, R. W. Superluminal and slow light propagation in a room-temperature solid. Science 301, 200–202 (2003).
Bigelow, M. S., Lepeshkin, N. N. & Boyd, R. W. Observation of ultraslow light propagation in ruby crystals at room temperature. Phys. Rev. Lett. 90, 113903 (2003).
Schültzgen, A. et al. Direct observation of excitonic Rabi oscillations in semiconductors. Phys. Rev. Lett. 82, 2346–2349 (1999).
Shimano, R. & Kuwata-Gonokami, M. Observation of Autler-Townes splitting of biexcitons in CuCl. Phys. Rev. Lett. 72, 530–533 (1994).
Faist, J., Capasso, F., Sirtori, C., West, K. W. & Pfeiffer, L. N. Controlling the sign of quantum interference by tunnelling from quantum wells. Nature 390, 589–591 (1997).
Serapiglia, G. B., Paspalakis, E., Sirtori, C., Vodopyanov, K. L. & Phillips, C. C. Observation of laser-induced quantum coherence in a semiconductor quantum well. Phys. Rev. Lett. 84, 1019–1022 (2000).
Acknowledgements
We are grateful to the UK Engineering and Physical Sciences Research Council for funding this project.
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Frogley, M., Dynes, J., Beck, M. et al. Gain without inversion in semiconductor nanostructures. Nature Mater 5, 175–178 (2006). https://doi.org/10.1038/nmat1586
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DOI: https://doi.org/10.1038/nmat1586
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