Letter | Published:

Granular materials flow like complex fluids

Nature volume 551, pages 360363 (16 November 2017) | Download Citation

Abstract

Granular materials such as sand, powders and foams are ubiquitous in daily life and in industrial and geotechnical applications1,2,3,4. These disordered systems form stable structures when unperturbed, but in the presence of external influences such as tapping or shear they ‘relax’, becoming fluid in nature. It is often assumed that the relaxation dynamics of granular systems is similar to that of thermal glass-forming systems3,5. However, so far it has not been possible to determine experimentally the dynamic properties of three-dimensional granular systems at the particle level. This lack of experimental data, combined with the fact that the motion of granular particles involves friction (whereas the motion of particles in thermal glass-forming systems does not), means that an accurate description of the relaxation dynamics of granular materials is lacking. Here we use X-ray tomography to determine the microscale relaxation dynamics of hard granular ellipsoids subject to an oscillatory shear. We find that the distribution of the displacements of the ellipsoids is well described by a Gumbel law6 (which is similar to a Gaussian distribution for small displacements but has a heavier tail for larger displacements), with a shape parameter that is independent of the amplitude of the shear strain and of the time. Despite this universality, the mean squared displacement of an individual ellipsoid follows a power law as a function of time, with an exponent that does depend on the strain amplitude and time. We argue that these results are related to microscale relaxation mechanisms that involve friction and memory effects (whereby the motion of an ellipsoid at a given point in time depends on its previous motion). Our observations demonstrate that, at the particle level, the dynamic behaviour of granular systems is qualitatively different from that of thermal glass-forming systems, and is instead more similar to that of complex fluids. We conclude that granular materials can relax even when the driving strain is weak.

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Acknowledgements

Some of the preliminary experiments were carried out at BL13W1 beamline of Shanghai Synchrotron Radiation Facility. The work is supported by the National Natural Science Foundation of China (numbers 11175121, 11675110 and U1432111), Specialized Research Fund for the Doctoral Program of Higher Education of China (grant number 20110073120073) and ANR-15-CE30-0003-02. W.K. is member of the Institut Universitaire de France.

Author information

Affiliations

  1. School of Physics and Astronomy, Shanghai Jiao Tong University, 800 Dong Chuan Road, Shanghai 200240, China

    • Binquan Kou
    • , Yixin Cao
    • , Jindong Li
    • , Chengjie Xia
    • , Zhifeng Li
    • , Jie Zhang
    •  & Yujie Wang
  2. Department of Radiology, Ruijin Hospital, Shanghai Jiao Tong University School of Medicine, Shanghai 200025, China

    • Haipeng Dong
    •  & Ang Zhang
  3. Institute of Natural Sciences, Shanghai Jiao Tong University, Shanghai 200240, China

    • Jie Zhang
  4. Laboratoire Charles Coulomb, University of Montpellier and CNRS, UMR 5221, 34095 Montpellier, France

    • Walter Kob
  5. Materials Genome Initiative Center, Shanghai Jiao Tong University, 800 Dong Chuan Road, Shanghai 200240, China

    • Yujie Wang
  6. Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, 210093, China

    • Yujie Wang

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Contributions

Y.W. and W.K. designed the research. B.K., Y.C., J.L., C.X., Z.L., H.D., A.Z., J.Z. and Y.W. performed the experiment. B.K., W.K. and Y.W. analysed the data and wrote the paper.

Competing interests

The authors declare no competing financial interests.

Corresponding authors

Correspondence to Walter Kob or Yujie Wang.

Reviewer Information Nature thanks R. Behringer and the other anonymous reviewer(s) for their contribution to the peer review of this work.

Publisher's note: Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Extended data

Supplementary information

Videos

  1. 1.

    The dynamics of the particles during the cycling experiment (γ=0.26): Top view.

    The video shows a view of the system from the top. It shows a horizontal cut through the middle of the sample and only the particles in the lower half of the central region of the box are displayed. The value of γ is 0.26 and the video covers the 615 cycles of the measurement with the CT scanner. Note that on the time scale considered, most of the particles move less than their long axis (see Fig. 1b of the main text)

  2. 2.

    The dynamics of the particles during the cycling experiment (γ=0.26): Side view.

    The video shows a side view of the same system of Supplementary Video 1. We made a vertical cut through the middle of the sample and show only the particles in the sector with large x. Note that the system shows no evident signature for convective motion.

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DOI

https://doi.org/10.1038/nature24062

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