Abstract
The generation, distribution and control of entanglement across quantum networks is one of the main goals of quantum information science1,2. In previous studies, hyperfine ground states of single atoms or atomic ensembles have been entangled with spontaneously emitted light3,4,5,6. The probabilistic character of the spontaneous emission process leads to long entanglement generation times, limiting realized network implementations to just two nodes7,8,9,10. The success probability for atom–photon entanglement protocols can be increased by confining a single atom in a high-finesse optical cavity11,12. Alternatively, quantum networks with superior scaling properties could be achieved using entanglement between light fields and atoms in quantum superpositions of the ground and highly excited (Rydberg) electronic states2,13,14. Here we report the generation of such entanglement. The dephasing of the optical atomic coherence is inhibited by state-insensitive confinement of both the ground and Rydberg states of an ultracold atomic gas in an optical lattice15. Our results pave the way for functional, many-node quantum networks capable of deterministic quantum logic operations between long-lived atomic memories.
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References
Duan, L.-M., Lukin, M. D., Cirac, J. I. & Zoller, P. Long-distance quantum communication with atomic ensembles and linear optics. Nature 414, 413–418 (2001)
Saffman, M., Walker, T. G. & Mølmer, K. Quantum information with Rydberg atoms. Rev. Mod. Phys. 82, 2313–2363 (2010)
Monroe, C. & Kim, J. Scaling the ion trap quantum processor. Science 339, 1164–1169 (2013)
Matsukevich, D. N. & Kuzmich, A. Quantum state transfer between matter and light. Science 306, 663–666 (2004)
Volz, J. et al. Observation of entanglement of a single photon with a trapped atom. Phys. Rev. Lett. 96, 030404 (2006)
Simon, J., Tanji, H., Ghosh, S. & Vuletic, V. Single-photon bus connecting spin-wave quantum memories. Nature Phys. 3, 765–769 (2007)
Chanelière, T. et al. Storage and retrieval of single photons transmitted between remote quantum memories. Nature 438, 833–836 (2005)
Eisaman, M. et al. Electromagnetically induced transparency with tunable single-photon pulses. Nature 438, 837–841 (2005)
Matsukevich, D. N. et al. Entanglement of remote atomic qubits. Phys. Rev. Lett. 96, 030405 (2006)
Hofmann, J. et al. Heralded entanglement between widely separated atoms. Science 337, 72–75 (2012)
Ritter, S. et al. An elementary quantum network of single atoms in optical cavities. Nature 484, 195–200 (2012)
Stute, A. et al. Tunable ion-photon entanglement in an optical cavity. Nature 485, 482–485 (2012)
Lukin, M. D. et al. Dipole blockade and quantum information processing in mesoscopic atomic ensembles. Phys. Rev. Lett. 87, 037901 (2001)
Saffman, M. & Walker, T. G. Creating single-atom and single-photon sources from entangled atomic ensembles. Phys. Rev. A 66, 065403 (2002)
Saffman, M. & Walker, T. G. Analysis of a quantum logic device based on dipole-dipole interactions of optically trapped Rydberg atoms. Phys. Rev. A 72, 022347 (2005)
Acín, A., Cirac, J. I. & Lewenstein, M. Entanglement percolation in quantum networks. Nature Phys. 3, 256–259 (2007)
Gallagher, T. F. Rydberg Atoms (Cambridge Univ. Press, 1994)
Urban, E. et al. Observation of Rydberg blockade between two atoms. Nature Phys. 5, 110–114 (2009)
Gaëtan, A. et al. Observation of collective excitation of two individual atoms in the Rydberg blockade regime. Nature Phys. 5, 115–118 (2009)
Zhao, B., Mueller, M., Hammerer, K. & Zoller, P. Efficient quantum repeater based on deterministic Rydberg gates. Phys. Rev. A 81, 052329 (2010)
Brion, E., Carlier, F., Akulin, V. M. & Mølmer, K. Quantum repeater with Rydberg-blocked atomic ensembles in fiber-coupled cavities. Phys. Rev. A 85, 042324 (2012)
Mohapatra, A. K., Jackson, T. R. & Adams, C. S. Coherent optical detection of highly excited Rydberg states using electromagnetically induced transparency. Phys. Rev. Lett. 98, 113003 (2007)
Dudin, Y. O. & Kuzmich, A. Strongly interacting Rydberg excitations of a cold atomic gas. Science 336, 887–889 (2012)
Dudin, Y. O., Li, L., Bariani, F. & Kuzmich, A. Observation of coherent many-body Rabi oscillations. Nature Phys. 8, 790–794 (2012)
Dudin, Y. O., Bariani, F. & Kuzmich, A. Emergence of spatial spin-wave correlations in a cold atomic gas. Phys. Rev. Lett. 109, 133602 (2012)
Schauß, P. et al. Observation of spatially ordered structures in a two-dimensional Rydberg gas. Nature 491, 87–91 (2012)
Peyronel, T. et al. Quantum nonlinear optics with single photons enabled by strongly interacting atoms. Nature 488, 57–60 (2012)
Maxwell, D. T. et al. Storage and control of optical photons using Rydberg polaritons. Phys. Rev. Lett. 110, 103001 (2013)
Anderson, S. E., Younge, K. C. & Raithel, G. Trapping Rydberg atoms in an optical lattice. Phys. Rev. Lett. 107, 263001 (2011)
Tan, S. M., Walls, D. F. & Collett, M. J. Nonlocality of a single photon. Phys. Rev. Lett. 66, 252–255 (1991)
Dudin, Y. O., Li, L. & Kuzmich, A. Light storage on the minute scale. Phys. Rev. A 87, 031801(R) (2013)
Acknowledgements
This work was supported by the Atomic Physics Program and the Quantum Memories MURI of the Air Force Office of Scientific Research and the National Science Foundation.
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Li, L., Dudin, Y. & Kuzmich, A. Entanglement between light and an optical atomic excitation. Nature 498, 466–469 (2013). https://doi.org/10.1038/nature12227
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DOI: https://doi.org/10.1038/nature12227
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