Abstract
Entanglement has a central role in fundamental tests of quantum mechanics1 as well as in the burgeoning field of quantum information processing. Particularly in the context of quantum networks and communication, a main challenge is the efficient generation of entanglement between stationary (spin) and propagating (photon) quantum bits2. Here we report the observation of quantum entanglement between a semiconductor quantum dot spin and the colour of a propagating optical photon. The demonstration of entanglement relies on the use of fast, single-photon detection, which allows us to project the photon into a superposition of red and blue frequency components. Our results extend the previous demonstrations of single-spin/single-photon entanglement in trapped ions3, neutral atoms4,5 and nitrogen–vacancy centres6 to the domain of artificial atoms in semiconductor nanostructures that allow for on-chip integration of electronic and photonic elements7,8. As a result of its fast optical transitions and favourable selection rules, the scheme we implement could in principle generate nearly deterministic entangled spin–photon pairs at a rate determined ultimately by the high spontaneous emission rate. Our observation constitutes a first step towards implementation of a quantum network with nodes9 consisting of semiconductor spin quantum bits10,11,12.
This is a preview of subscription content, access via your institution
Relevant articles
Open Access articles citing this article.
-
Magnetic tuning of tunnel coupling between InAsP double quantum dots in InP nanowires
Scientific Reports Open Access 24 March 2022
-
Optical charge injection and coherent control of a quantum-dot spin-qubit emitting at telecom wavelengths
Nature Communications Open Access 08 February 2022
-
Optically driving the radiative Auger transition
Nature Communications Open Access 12 November 2021
Access options
Subscribe to this journal
Receive 51 print issues and online access
$199.00 per year
only $3.90 per issue
Rent or buy this article
Get just this article for as long as you need it
$39.95
Prices may be subject to local taxes which are calculated during checkout



References
Aspect, A., Grangier, P. & Roger, G. Experimental realization of Einstein-Podolsky-Rosen-Bohm gedanken experiment: a new violation of Bell’s inequalities. Phys. Rev. Lett. 49, 91–94 (1982)
DiVincenzo, D. P. The physical implementation of quantum computation. Fortschr. Phys. 48, 771–783 (2000)
Blinov, B., Moehring, D. & Duan, L. Observation of entanglement between a single trapped atom and a single photon. Nature 428, 153–157 (2004)
Volz, J. et al. Observation of entanglement of a single photon with a trapped atom. Phys. Rev. Lett. 96, 030404 (2006)
Wilk, T., Webster, S. C., Kuhn, A. & Rempe, G. Single-atom single-photon quantum interface. Science 317, 488–490 (2007)
Togan, E. et al. Quantum entanglement between an optical photon and a solid-state spin qubit. Nature 466, 730–734 (2010)
Hennessy, K. et al. Quantum nature of a strongly coupled single quantum dot-cavity system. Nature 445, 896–899 (2007)
Faraon, A. et al. Coupling of nitrogen-vacancy centers to photonic crystal cavities in monocrystalline diamond. Phys. Rev. Lett 109, 033604 (2012)
Yuan, Z.-S. et al. Experimental demonstration of a BDCZ quantum repeater node. Nature 454, 1098–1101 (2008)
Loss, D. & DiVincenzo, D. P. Quantum computation with quantum dots. Phys. Rev. A 57, 120–126 (1998)
Imamoğlu, A. et al. Quantum information processing using quantum dot spins and cavity QED. Phys. Rev. Lett. 83, 4204–4207 (1999)
Hanson, R. et al. Spins in few-electron quantum dots. Rev. Mod. Phys. 79, 1217–1265 (2007)
Press, D., Ladd, T. D., Zhang, B. & Yamamoto, Y. Complete quantum control of a single quantum dot spin using ultrafast optical pulses. Nature 456, 218–221 (2008)
Greilich, A. et al. Ultrafast optical rotations of electron spins in quantum dots. Nature Phys. 5, 262–266 (2009)
Poem, E. et al. Accessing the dark exciton with light. Nature Phys. 6, 993–997 (2010)
Kim, D. et al. Ultrafast optical control of entanglement between two quantum-dot spins. Nature Phys. 7, 223–229 (2011)
Shulman, M. D. et al. Demonstration of entanglement of electrostatically coupled singlet-triplet qubits. Science 336, 202–205 (2012)
Cirac, J., Ekert, A. & Huelga, S. Distributed quantum computation over noisy channels. Phys. Rev. A 59, 4249–4254 (1999)
Xu, X. et al. Fast spin state initialization in a singly charged InAs-GaAs quantum dot by optical cooling. Phys. Rev. Lett. 99, 097401 (2007)
Muller, A. et al. Resonance fluorescence from a coherently driven semiconductor quantum dot in a cavity. Phys. Rev. Lett. 99, 187402 (2007)
Vamivakas, A. N., Zhao, Y., Lu, C.-Y. & Atature, M. Spin-resolved quantum-dot resonance fluorescence. Nature Phys. 5, 198–202 (2009); corrigendum. 5, 925 (2009)
Yılmaz, S. T., Fallahi, P. & Imamoglu, A. Quantum-dot-spin single-photon interface. Phys. Rev. Lett. 105, 033601 (2010)
Gol’tsman, G. N. et al. Picosecond superconducting single-photon detector. Appl. Phys. Lett. 79, 705–707 (2001)
Press, D. et al. Ultrafast optical spin echo in a single quantum dot. Nature Photon. 4, 367–370 (2010)
Claudon, J. et al. A highly efficient single-photon source based on a quantum dot in a photonic nanowire. Nature Photon. 4, 174–177 (2010)
Dousse, A. et al. Ultrabright source of entangled photon pairs. Nature 466, 217–220 (2010)
Xu, X. et al. Optically controlled locking of the nuclear field via coherent dark-state spectroscopy. Nature 459, 1105–1109 (2009)
Flagg, E. B. et al. Interference of single photons from two separate semiconductor quantum dots. Phys. Rev. Lett. 104, 137401 (2010)
Patel, R. et al. Two-photon interference of the emission from electrically tunable remote quantum dots. Nature Photon. 4, 632–635 (2010)
Moehring, D. L. et al. Entanglement of single-atom quantum bits at a distance. Nature 449, 68–71 (2007)
Acknowledgements
We acknowledge discussions with W. Chin, M. Kroner, A. Srivastava, J. Elzerman, A. Reinhard, T. Volz, P. Maletinsky and D. Gershoni. This work is supported by NCCR Quantum Science and Technology, a research instrument of the Swiss National Science Foundation; the Swiss NSF (grant no. 200021-140818); an ERC Advanced Investigator Grant (A.I.); and a Marie Curie International Incoming Fellowship within FP7 (W.B.G.).
Author information
Authors and Affiliations
Contributions
All authors contributed extensively to this work.
Corresponding authors
Ethics declarations
Competing interests
The authors declare no competing financial interests.
Supplementary information
Supplementary Information
This file contains Supplementary Text and Data, additional references and Supplementary Figures 1-2. (PDF 622 kb)
Rights and permissions
About this article
Cite this article
Gao, W., Fallahi, P., Togan, E. et al. Observation of entanglement between a quantum dot spin and a single photon. Nature 491, 426–430 (2012). https://doi.org/10.1038/nature11573
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1038/nature11573
This article is cited by
-
Quantum photonics with layered 2D materials
Nature Reviews Physics (2022)
-
Optical charge injection and coherent control of a quantum-dot spin-qubit emitting at telecom wavelengths
Nature Communications (2022)
-
Magnetic tuning of tunnel coupling between InAsP double quantum dots in InP nanowires
Scientific Reports (2022)
-
Quantum-dot-based deterministic photon–emitter interfaces for scalable photonic quantum technology
Nature Nanotechnology (2021)
-
Spin-induced linear polarization of photoluminescence in antiferromagnetic van der Waals crystals
Nature Materials (2021)
Comments
By submitting a comment you agree to abide by our Terms and Community Guidelines. If you find something abusive or that does not comply with our terms or guidelines please flag it as inappropriate.