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Nanostructure-enhanced atomic line emission

Abstract

Arising from S. Kim et al. Nature 453, 757–760 (2008)10.1038/nature07012; Kim et al. reply

Plasmonic nanostructures offer unique possibilities for enhancing linear and nonlinear optical processes1,2,3,4,5,6. Recently, Kim et al.7 reported nanostructure-enhanced high harmonic generation (HHG). Here, using nearly identical conditions, we demonstrate extreme-ultraviolet (EUV) emission from gas-exposed nanostructures, but come to entirely different conclusions: instead of HHG, we observe line emission of neutral and ionized gas atoms. We also discuss fundamental physical aspects limiting nanostructure-based HHG.

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Figure 1: Experimental set-up and results.

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References

  1. Fischer, H. & Martin, O. J. F. Engineering the optical response of plasmonic nanoantennas. Opt. Express 16, 9144–9154 (2008)

    Article  ADS  Google Scholar 

  2. Genov, D. A., Sarychev, A. K., Shalaev, V. M. & Wei, A. Resonant field enhancements from metal nanoparticle arrays. Nano Lett. 4, 153–158 (2004)

    Article  ADS  CAS  Google Scholar 

  3. Merlein, J. et al. Nanomechanical control of an optical antenna. Nature Photon. 2, 230–233 (2008)

    Article  CAS  Google Scholar 

  4. Fromm, D. P., Sundaramurthy, A., Schuck, P. J., Kino, G. & Moerner, W. E. Gap-dependent optical coupling of single “bowtie” nanoantennas resonant in the visible. Nano Lett. 4, 957–961 (2004)

    Article  ADS  CAS  Google Scholar 

  5. Li, K., Stockman, M. I. & Bergman, D. J. Self-similar chain of metal nanospheres as an efficient nanolens. Phys. Rev. Lett. 91, 227402 (2003)

    Article  ADS  Google Scholar 

  6. Hanke, T. et al. Efficient nonlinear light emission of single gold optical antennas driven by few-cycle near-infrared pulses. Phys. Rev. Lett. 103, 257404 (2009)

    Article  ADS  CAS  Google Scholar 

  7. Kim, S. et al. High-harmonic generation by resonant plasmon field enhancement. Nature 453, 757–760 (2008)

    Article  ADS  CAS  Google Scholar 

  8. Minnhagen, L. Accurately measured and calculated ground-term combinations of Ar II. J. Opt. Soc. Am. 61, 1257–1262 (1971)

    Article  ADS  CAS  Google Scholar 

  9. Minnhagen, L. Spectrum and the energy levels of neutral argon, Ar I. J. Opt. Soc. Am. 63, 1185–1198 (1973)

    Article  ADS  CAS  Google Scholar 

  10. Sansonetti, J. E. & Martin, W. C. Handbook of basic atomic spectroscopic data. J. Phys. Chem. Ref. Data 34, 1582–1591; 2109–2117 (2005)

    Article  Google Scholar 

  11. Li, X. F., L'Huillier, A., Ferray, M., Lompré, L. A. & Mainfray, G. Multiple-harmonic generation in rare gases at high laser intensity. Phys. Rev. A 39, 5751–5761 (1989)

    Article  ADS  CAS  Google Scholar 

  12. Park, I.-Y. et al. Plasmonic generation of ultrashort extreme-ultraviolet light pulses. Nature Photon. 5, 677–681 (2011)

    Article  ADS  CAS  Google Scholar 

  13. Kim, S., Park, I.-Y., Choi, J. & Kim, S.-W. in Progress in Ultrafast Intense Laser Science Vol. 6 (eds Yamanouchi, K., Gerber, G. & Bandrauk, A. D. ) 129–144 (Springer, 2010)

    Book  Google Scholar 

  14. Boyce, J. The spectra of xenon in the extreme ultraviolet. Phys. Rev. 49, 730–732 (1936)

    Article  ADS  CAS  Google Scholar 

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All authors were closely involved in this study and contributed to the ideas, realization of the experiments, data analysis and interpretation, and writing of the paper.

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Correspondence to C. Ropers.

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Sivis, M., Duwe, M., Abel, B. et al. Nanostructure-enhanced atomic line emission. Nature 485, E1–E2 (2012). https://doi.org/10.1038/nature10978

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