Abstract
Heat generation by electric current, which is ubiquitous in electronic devices and circuits, raises energy consumption and will become increasingly problematic in future generations of high-density electronics. The control and re-use of heat are therefore important topics for existing and emerging technologies, including spintronics. Recently it was reported that heat flow within a ferromagnet can produce a flow of spin angular momentum—a spin current—and an associated voltage1. This spin Seebeck effect has been observed in metallic1,2, insulating3 and semiconductor ferromagnets4 with temperature gradients across them. Here we describe and report the demonstration of Seebeck spin tunnelling—a distinctly different thermal spin flow, of purely interfacial nature—generated in a tunnel contact between electrodes of different temperatures when at least one of the electrodes is a ferromagnet. The Seebeck spin current is governed by the energy derivative of the tunnel spin polarization. By exploiting this in ferromagnet–oxide–silicon tunnel junctions, we observe thermal transfer of spins from the ferromagnet to the silicon without a net tunnel charge current. The induced spin accumulation scales linearly with heating power and changes sign when the temperature differential is reversed. This thermal spin current can be used by itself, or in combination with electrical spin injection, to increase device efficiency. The results highlight the engineering of heat transport in spintronic devices and facilitate the functional use of heat.
This is a preview of subscription content, access via your institution
Relevant articles
Open Access articles citing this article.
-
A double quantum dot spin valve
Communications Physics Open Access 06 August 2020
-
Low field magneto-tunable photocurrent in CoFe2O4 nanostructure films for enhanced photoelectrochemical properties
Scientific Reports Open Access 25 April 2018
-
Large magneto-Seebeck effect in magnetic tunnel junctions with half-metallic Heusler electrodes
Nature Communications Open Access 20 November 2017
Access options
Subscribe to this journal
Receive 51 print issues and online access
$199.00 per year
only $3.90 per issue
Rent or buy this article
Get just this article for as long as you need it
$39.95
Prices may be subject to local taxes which are calculated during checkout




References
Uchida, K. et al. Observation of the spin Seebeck effect. Nature 455, 778–781 (2008)
Slachter, A., Bakker, F. L., Adam, J.-P. & van Wees, B. J. Thermally driven spin injection from a ferromagnet into a non-magnetic metal. Nature Phys. 6, 879–882 (2010)
Uchida, K. et al. Spin Seebeck insulator. Nature Mater. 9, 894–897 (2010)
Jaworski, C. M. et al. Observation of the spin-Seebeck effect in a ferromagnetic semiconductor. Nature Mater. 9, 898–903 (2010)
Zˇutic´, I., Fabian, J. & Das Sarma, S. Spintronics: fundamentals and applications. Rev. Mod. Phys. 76, 323–410 (2004)
Chappert, C., Fert, A. & Nguyen van Dau, F. The emergence of spin electronics in data storage. Nature Mater. 6, 813–823 (2007)
Johnson, M. & Silsbee, R. H. Thermodynamic analysis of interfacial transport and of the thermomagnetoelectric system. Phys. Rev. B 35, 4959–4972 (1987)
Fukushima, A. et al. Peltier effect in sub-micron-size metallic junctions. Jpn. J. Appl. Phys. 44, L12–L14 (2005)
Gravier, L., Serrano-Guisan, S., Reuse, F. & Ansermet, J.-Ph. Spin-dependent Peltier effect of perpendicular currents in multilayered nanowires. Phys. Rev. B 73, 052410 (2006)
Hatami, M., Bauer, G. E. W., Zhang, Q. & Kelly, P. J. Thermoelectric effects in magnetic nanostructures. Phys. Rev. B 79, 174426 (2009)
Slonckzewski, J. C. Initiation of spin-transfer torque by thermal transport from magnons. Phys. Rev. B 82, 054403 (2010)
Bauer, G. E. W., MacDonald, A. H. & Maekawa, S. Spin caloritronics. Solid State Commun. 150, 459–460 (2010)
Xiao, J., Bauer, G. E. W., Uchida, K., Saitoh, E. & Maekawa, S. Theory of magnon-driven spin Seebeck effect. Phys. Rev. B 81, 214418 (2010)
Sinova, J. Spin Seebeck effect: thinks globally but acts locally. Nature Mater. 9, 880–881 (2010)
Adachi, H. et al. Gigantic enhancement of spin Seebeck effect by phonon drag. Appl. Phys. Lett. 97, 252506 (2010)
Dash, S. P., Sharma, S., Patel, R. S., de Jong, M. P. & Jansen, R. Electrical creation of spin polarization in silicon at room temperature. Nature 462, 491–494 (2009)
Min, B. C., Motohashi, K., Lodder, J. C. & Jansen, R. Tunable spin-tunnel contacts to silicon using low-work-function ferromagnets. Nature Mater. 5, 817–822 (2006)
Nolas, G. S., Sharp, J. & Goldsmid, H. J. Thermoelectrics: Basic Principles and New Materials Developments Ch. 1 (Springer, 2001)
Valenzuela, S. O., Monsma, D. J., Marcus, C. M., Narayanamurti, V. & Tinkham, M. Spin polarized tunneling at finite bias. Phys. Rev. Lett. 94, 196601 (2005)
Park, B. G., Banerjee, T., Lodder, J. C. & Jansen, R. Tunnel spin polarization versus energy for clean and doped Al2O3 barriers. Phys. Rev. Lett. 99, 217206 (2007)
Wang, Z.-C., Su, G. & Gao, S. Spin-dependent thermal and electrical transport in a spin-valve system. Phys. Rev. B 63, 224419 (2001)
McCann, E. & Fal'ko, V. I. Giant magnetothermopower of magnon-assisted transport in ferromagnetic tunnel junctions. Phys. Rev. B 66, 134424 (2002)
McCann, E. & Fal’ko, V. I. A tunnel junction between a ferromagnet and a normal metal: magnon-assisted contribution to thermopower and conductance. J. Magn. Magn. Mater. 268, 123–131 (2004)
Jansen, R. et al. Electrical spin injection into moderately doped silicon enabled by tailored interfaces. Phys. Rev. B 82, 241305 (2010)
Dash, S. P. et al. Spin precession and decoherence near an interface with a ferromagnet. Preprint at 〈http://arxiv.org/abs/1101.1691〉 (2011)
Acknowledgements
We are grateful to S. P. Dash for help with the device fabrication and discussions, T. Yorozu for the finite-element calculations and A. Yamamoto for making the finite-element program available to us. This work was financially supported by the program “Controlling spin dynamics in magnetic nanostructures” of the Netherlands Foundation for Fundamental Research on Matter (FOM).
Author information
Authors and Affiliations
Contributions
J.-C.L.B. and R.J. designed the experiments. J.-C.L.B. and S.S. fabricated the devices. J.-C.L.B., S.S., H.S. and R.J. contributed to the measurements. R.J. developed the model calculation. All authors contributed to the planning, discussion and analysis of the research, and to the writing of the manuscript.
Corresponding author
Ethics declarations
Competing interests
The authors declare no competing financial interests.
Supplementary information
Supplementary Information
This file contains Supplementary Text and Data 1-7, Supplementary Figures 1-8 with legends, Supplementary Table 1 and additional references. (PDF 611 kb)
Rights and permissions
About this article
Cite this article
Le Breton, JC., Sharma, S., Saito, H. et al. Thermal spin current from a ferromagnet to silicon by Seebeck spin tunnelling. Nature 475, 82–85 (2011). https://doi.org/10.1038/nature10224
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1038/nature10224
This article is cited by
-
A double quantum dot spin valve
Communications Physics (2020)
-
Low field magneto-tunable photocurrent in CoFe2O4 nanostructure films for enhanced photoelectrochemical properties
Scientific Reports (2018)
-
Effects of the Spin Heat Accumulation on the Heat Generation in a Quantum Dot Coupled to Leads
Journal of Low Temperature Physics (2018)
-
Observation of transverse spin Nernst magnetoresistance induced by thermal spin current in ferromagnet/non-magnet bilayers
Nature Communications (2017)
-
Large magneto-Seebeck effect in magnetic tunnel junctions with half-metallic Heusler electrodes
Nature Communications (2017)
Comments
By submitting a comment you agree to abide by our Terms and Community Guidelines. If you find something abusive or that does not comply with our terms or guidelines please flag it as inappropriate.