Abstract
The energy-level structure of a quantum system, which has a fundamental role in its behaviour, can be observed as discrete lines and features in absorption and emission spectra. Conventionally, spectra are measured using frequency spectroscopy, whereby the frequency of a harmonic electromagnetic driving field is tuned into resonance with a particular separation between energy levels. Although this technique has been successfully employed in a variety of physical systems, including natural and artificial atoms and molecules, its application is not universally straightforward and becomes extremely challenging for frequencies in the range of tens to hundreds of gigahertz. Here we introduce a complementary approach, amplitude spectroscopy, whereby a harmonic driving field sweeps an artificial atom through the avoided crossings between energy levels at a fixed frequency. Spectroscopic information is obtained from the amplitude dependence of the system’s response, thereby overcoming many of the limitations of a broadband-frequency-based approach. The resulting ‘spectroscopy diamonds’, the regions in parameter space where transitions between specific pairs of levels can occur, exhibit interference patterns and population inversion that serve to distinguish the atom’s spectrum. Amplitude spectroscopy provides a means of manipulating and characterizing systems over an extremely broad bandwidth, using only a single driving frequency that may be orders of magnitude smaller than the energy scales being probed.
This is a preview of subscription content, access via your institution
Relevant articles
Open Access articles citing this article.
-
Solid-state qubits integrated with superconducting through-silicon vias
npj Quantum Information Open Access 03 July 2020
-
Probing the strongly driven spin-boson model in a superconducting quantum circuit
Nature Communications Open Access 11 April 2018
-
The flux qubit revisited to enhance coherence and reproducibility
Nature Communications Open Access 03 November 2016
Access options
Subscribe to this journal
Receive 51 print issues and online access
$199.00 per year
only $3.90 per issue
Rent or buy this article
Get just this article for as long as you need it
$39.95
Prices may be subject to local taxes which are calculated during checkout




References
Schawlow, A. L. Spectroscopy in a new light. Rev. Mod. Phys. 54, 697–707 (1982)
Thompson, R. C. High resolution laser spectroscopy of atomic systems. Rep. Prog. Phys. 48, 531–578 (1985)
Friedman, J. R., Patel, V., Chen, W., Tolpygo, S. K. & Lukens, J. E. Quantum superposition of distinct macroscopic states. Nature 406, 43–46 (2000)
van der Wal, C. H. et al. Quantum superposition of macroscopic persistent-current states. Science 290, 773–777 (2000)
Berkley, A. J. et al. Entangled macroscopic quantum states in two superconducting qubits. Science 300, 1548–1550 (2003)
Izmalkov, A. et al. Evidence for entangled states of two coupled flux quibits. Phys. Rev. Lett. 93, 037003 (2004)
van der Wiel, W. G. et al. Electron transport through double quantum dots. Rev. Mod. Phys. 75, 1–22 (2003)
Clarke, J., Cleland, A. N., Devoret, M. H., Esteve, D. & Martinis, J. H. Quantum mechanics of a macroscopic variable: the phase difference of a Josephson junction. Science 239, 992–997 (1988)
Hanson, R., Kouwenhoven, L. P., Petta, J. R., Tarucha, S. & Vandersypen, L. M. K. Spins in few-electron quantum dots. Rev. Mod. Phys. 79, 1217–1265 (2007)
Nakamura, Y., Pashkin, Y. A. & Tsai, J. S. Coherent control of macroscopic quantum states in a single-Cooper-pair box. Nature 398, 786–788 (1999)
Vion, D. et al. Manipulating the quantum state of an electrical circuit. Science 296, 886–889 (2002)
Yu, Y., Han, S., Chu, X., Chu, S.-I. & Wang, Z. Coherent temporal oscillations of macroscopic quantum states in a Josephson junction. Science 296, 889–892 (2002)
Martinis, J. M., Nam, S. & Aumentado, J. Rabi oscillations in a large Josephson-junction qubit. Phys. Rev. Lett. 89, 117901 (2002)
Chiorescu, I., Nakamura, Y., Harmans, C. J. P. M. & Mooij, J. E. Coherent quantum dynamics of a superconducting flux qubit. Science 299, 1869–1871 (2003)
Collin, R. E. Foundations for Microwave Engineering (Wiley-IEEE, 2001)
Friedman, J. R. et al. Macroscopic measurement of resonant magnetization tunnelling in high-spin molecules. Phys. Rev. Lett. 76, 3830–3833 (1996)
Thomas, L. et al. Macroscopic quantum tunnelling of magnetization in a single crystal of nanomagnets. Nature 383, 145–147 (1996)
Wernsdorfer, W. & Sessoli, R. Quantum phase interference and parity effects in magnetic molecular clusters. Science 284, 133–135 (1999)
Cohen-Tannoudji, C., Dupont-Roc, J. & Grynberg, G. Atom-Photon Interactions: Basic Processes and Applications Ch. 6 (Wiley, 1992)
Nakamura, H. Nonadiabatic Transition Ch. 1 2 (World Scientific, 2001)
Stückelberg, E. C. G. Theory of inelastic collisions between atoms. Helv. Phys. Acta 5, 369–422 (1932)
Nakamura, Y., Pashkin, Y. A. & Tsai, J. S. Rabi oscillations in a large Josephson-junction charge two-level system. Phys. Rev. Lett. 87, 246601 (2001)
Claudon, J., Balestro, F., Hekking, J. W. J. & Buisson, O. Coherent oscillations in a superconducting multilevel quantum system. Phys. Rev. Lett. 93, 187003 (2004)
Plourde, B. L. T. et al. Flux qubits and readout device with two independent flux lines. Phys. Rev. B 72, 060506(R) (2005)
Saito, S. et al. Parametric control of a superconducting flux qubit. Phys. Rev. Lett. 96, 107001 (2006)
Izmalkov, A. et al. Observation of macroscopic Landau-Zener transitions in a superconducting device. Eur. Phys. Rev. Lett. 65, 844–849 (2004)
Oliver, W. D. et al. Mach-Zehnder interferometry in a strongly driven superconducting qubit. Science 310, 1653–1657 (2003)
Sillanpää, M., Lehtinen, T., Paila, A., Makhlin & Hakonen, P. Continuous-time monitoring of Landau-Zener interference in a Cooper-pair box. Phys. Rev. Lett. 96, 187002 (2006)
Berns, D. M. et al. Coherent quasiclassical dynamics of a persistent current qubit. Phys. Rev. Lett. 97, 150502 (2006)
Wilson, C. M. et al. Coherence times of dressed states of a superconducting qubit under extreme driving. Phys. Rev. Lett. 98, 257003 (2007)
Valenzuela, S. O. et al. Microwave-induced cooling of a superconducting qubit. Science 314, 1589–1592 (2006)
Niskanen, A. O., Nakamura, Y. & Pekola, J. P. Information entropic superconducting microcooler. Phys. Rev. B 76, 174523 (2007)
You, J. Q., Liu, Y. & Nori, F. Simultaneous cooling of an artificial atom and its neighboring quantum system. Phys. Rev. Lett. 100, 047001 (2008)
Chiorescu, I. et al. Coherent dynamics of a flux qubit coupled to a harmonic oscillator. Nature 431, 159–162 (2004)
Wallraff, A. et al. Strong coupling of a single photon to a superconducting qubit using circuit quantum electrodynamics. Nature 431, 162–167 (2004)
Johansson, J. et al. Vacuum Rabi oscillations in a macroscopic superconducting qubit LC oscillator system. Phys. Rev. Lett. 96, 127006 (2006)
Sillanpää, M. A., Park, J. I. & Simmonds, R. W. Coherent quantum state storage and transfer between two phase qubits via a resonant cavity. Nature 449, 438–442 (2007)
Majer, J. et al. Coupling superconducting qubits via a cavity bus. Nature 449, 443–447 (2007)
Siddiqi, I. et al. RF-driven Josephson bifurcation amplifier for quantum measurement. Phys. Rev. Lett. 93, 207002 (2004)
Katz, N. et al. Coherent state evolution in a superconducting qubit from partial-collapse measurement. Science 312, 1498–1500 (2006)
Lupaşcu, A. et al. Quantum non-demolition measurement of a superconducting two-level system. Nature Phys. 3, 119–125 (2007)
Mooij, J. E. et al. Josephson persistent-current qubit. Science 285, 1036–1039 (1999)
Orlando, T. P. et al. Superconducting persistent-current qubit. Phys. Rev. B 60, 15398–15413 (1999)
Mark, M. et al. “Stueckelberg interferometry” with ultracold molecules. Phys. Rev. Lett. 99, 113201 (2007)
Astafiev, O. et al. Single artificial-atom lasing. Nature 449, 588–590 (2007)
Rudner, M. S. et al. Quantum phase tomography of a strongly driven qubit. Preprint at 〈http://arxiv.org/abs/0805.1555〉 (2008)
Ashab, S., Johansson, J. R., Zagoskin, A. M. & Nori, F. Two-level systems driven by large-amplitude fields. Phys. Rev. A 75, 063414 (2007)
Wubs, M. et al. Gauging a quantum heat bath with dissipative Landau-Zener transitions. Phys. Rev. Lett. 97, 200404 (2006)
Mark, M. et al. Spectroscopy of ultracold trapped caesium Feshbach molecules. Phys. Rev. A 76, 042514 (2007)
Lang, F. et al. Cruising through molecular bound-state manifolds with radiofrequency. Nature Phys. 4, 223–226 (2008)
Acknowledgements
We thank A. Shytov, J. Bylander, B. Turek, A. J. Kerman and J. Sage for discussions and D. Baker, V. Bolkhovsky, G. Fitch, E. Macedo, P. Murphy, K. Parrillo, R. Slattery and T. Weir at Lincoln Laboratory, MIT, for technical assistance. This work was supported by the Air Force Office of Scientific Research and the Laboratory for Physical Sciences (F49620-01-1-0457) under the Defense University Research Initiative in Nanotechnology programme, and by the US government. The work at Lincoln Laboratory was sponsored by the US Department of Defence under Air Force Contract No. FA8721-05-C-0002.
Author information
Authors and Affiliations
Corresponding author
Supplementary information
Supplementary Information
This file contains Supplementary Discussion, Supplementary Figures 1-8 with legends, and Supplementary References. (PDF 3373 kb)
Rights and permissions
About this article
Cite this article
Berns, D., Rudner, M., Valenzuela, S. et al. Amplitude spectroscopy of a solid-state artificial atom. Nature 455, 51–57 (2008). https://doi.org/10.1038/nature07262
Received:
Accepted:
Issue Date:
DOI: https://doi.org/10.1038/nature07262
This article is cited by
-
Solid-state qubits integrated with superconducting through-silicon vias
npj Quantum Information (2020)
-
Probing the strongly driven spin-boson model in a superconducting quantum circuit
Nature Communications (2018)
-
The flux qubit revisited to enhance coherence and reproducibility
Nature Communications (2016)
-
Ultrafast universal quantum control of a quantum-dot charge qubit using Landau–Zener–Stückelberg interference
Nature Communications (2013)
-
A quantum spectrum analyser
Nature Physics (2011)
Comments
By submitting a comment you agree to abide by our Terms and Community Guidelines. If you find something abusive or that does not comply with our terms or guidelines please flag it as inappropriate.