Abstract
Electronic transport through nanostructures is greatly affected by the presence of superconducting leads1,2,3. If the interface between the nanostructure and the superconductors is sufficiently transparent, a dissipationless current (supercurrent) can flow through the device owing to the Josephson effect4,5. A Josephson coupling, as measured by the zero-resistance supercurrent, has been obtained using tunnel barriers, superconducting constrictions, normal metals and semiconductors. The coupling mechanisms vary from tunnelling to Andreev reflection5,6,7,8. The latter process has hitherto been observed only in normal-type systems with a continuous density of electronic states. Here we investigate a supercurrent flowing through a discrete density of states—that is, the quantized single particle energy states of a quantum dot9, or ‘artificial atom’, placed between superconducting electrodes. For this purpose, we exploit the quantum properties of finite-sized carbon nanotubes10. By means of a gate electrode, successive discrete energy states are tuned on- and off-resonance with the Fermi energy in the superconducting leads, resulting in a periodic modulation of the critical current and a non-trivial correlation between the conductance in the normal state and the supercurrent. We find, in good agreement with existing theory11, that the product of the critical current and the normal state resistance becomes an oscillating function, in contrast to being constant as in previously explored regimes.
This is a preview of subscription content, access via your institution
Access options
Subscribe to this journal
Receive 51 print issues and online access
$199.00 per year
only $3.90 per issue
Buy this article
- Purchase on SpringerLink
- Instant access to full article PDF
Prices may be subject to local taxes which are calculated during checkout
Similar content being viewed by others
References
de Gennes, P. G. Boundary effects in superconductors. Rev. Mod. Phys. 36, 225–237 (1964)
Ralph, D. C., Black, C. T. & Tinkham, M. Spectroscopic measurements of discrete electronic states in single metal particles. Phys. Rev. Lett. 74, 3241–3244 (1995)
von Delft, J. & Ralph, D. C. Spectroscopy of discrete energy levels in ultrasmall metallic grains. Phys. Rep. 345, 61–173 (2001)
Josephson, B. D. Possible new effects in superconductive tunnelling. Phys. Lett. 1, 251–253 (1962)
Tinkham, M. Introduction to Superconductivity (McGraw-Hill, Singapore, 1996)
Andreev, A. F. The thermal conductivity of the intermediate state in superconductors. Sov. Phys. JETP 19, 1228–1231 (1964)
Likharev, K. K. Superconducting weak links. Rev. Mod. Phys. 51, 101–159 (1979)
Blonder, G. E., Tinkham, M. & Klapwijk, T. M. Transition from metallic to tunneling regimes in superconducting micro-constrictions—excess current, charge imbalance, and super-current conversion. Phys. Rev. B 25, 4515–4532 (1982)
Sohn, L. L., Kouwenhoven, L. P. & Schön, G. (eds) Mesoscopic Electron Transport (Kluwer, Dordrecht, 1997)
Dresselhaus, M. S., Dresselhaus, G. & Eklund, P. C. Science of Fullerenes and Carbon Nanotubes (Academic, San Diego, 1996)
Beenakker, C. W. J. & van Houten, H. Single-electron Tunneling and Mesoscopic Devices (eds Koch, H. & Lübbig, H.) see also http://xxx.lanl.gov/abs/cond-mat/0111505 (2001) 175–179 (Springer, Berlin, 1992)
Kouwenhoven, L. & Glazman, L. Revival of the Kondo effect. Phys. World 14, 33–38 (2001)
Jarillo-Herrero, P. et al. Orbital Kondo effect in carbon nanotubes. Nature 434, 484–488 (2005)
Liang, W. J. et al. Fabry-Perot interference in a nanotube electron waveguide. Nature 411, 665–669 (2001)
Buitelaar, M. R., Bachtold, A., Nussbaumer, T., Iqbal, M. & Schonenberger, C. Multiwall carbon nanotubes as quantum dots. Phys. Rev. Lett. 88, 156801 (2002)
Kasumov, A. Y. et al. Supercurrents through single-walled carbon nanotubes. Science 284, 1508–1511 (1999)
Morpurgo, A. F., Kong, J., Marcus, C. M. & Dai, H. Gate-controlled superconducting proximity effect in carbon nanotubes. Science 286, 263–265 (1999)
Buitelaar, M. R., Nussbaumer, T. & Schonenberger, C. Quantum dot in the Kondo regime coupled to superconductors. Phys. Rev. Lett. 89, 256801 (2002)
Haruyama, J. et al. End-bonding multiwalled carbon nanotubes in alumina templates: Superconducting proximity effect. Appl. Phys. Lett. 84, 4714–4716 (2004)
Buitelaar, M. R. et al. Multiple Andreev reflections in a carbon nanotube quantum dot. Phys. Rev. Lett. 91, 057005 (2003)
Takayanagi, H. & Kawakami, T. Superconducting proximity effect in the native inversion layer on InAs. Phys. Rev. Lett. 54, 2449–2452 (1985)
McEuen, P. L. Single-wall carbon nanotubes. Phys. World 13, 31–36 (2000)
Doh, Y. J. et al. Tunable supercurrent through semiconductor nanowires. Science 309, 272–275 (2005)
Liang, W. J., Bockrath, M. & Park, H. Shell filling and exchange coupling in metallic single-walled carbon nanotubes. Phys. Rev. Lett. 88, 126801 (2002)
Sapmaz, S. et al. Electronic excitation spectrum of metallic carbon nanotubes. Phys. Rev. B 71, 153402 (2005)
Galaktionov, A. V. & Zaikin, A. D. Quantum interference and supercurrent in multiple-barrier proximity structures. Phys. Rev. B 65, 184507 (2002)
Joyez, P., Lafarge, P., Filipe, A., Esteve, D. & Devoret, M. H. Observation of parity-induced suppression of Josephson tunneling in the superconducting single-electron transistor. Phys. Rev. Lett. 72, 2458–2461 (1994)
Glazman, L. I. & Matveev, K. A. Resonant Josephson current through Kondo impurities in a tunnel barrier. JETP Lett. 49, 659–662 (1989)
Choi, M. S., Lee, M., Kang, K. & Belzig, W. Kondo effect and Josephson current through a quantum dot between two superconductors. Phys. Rev. B 70, 020502 (2004)
Babic, B. & Schonenberger, C. Observation of Fano resonances in single-wall carbon nanotubes. Phys. Rev. B 70, 195408 (2004)
Acknowledgements
We thank Yu. V. Nazarov, C. W. J. Beenakker, W. Belzig, S. De Franceschi and Y-J. Doh for discussions and C. Dekker for the use of nanotube growth facilities. Financial support was obtained from the Japanese International Cooperative Research Project (ICORP) and the Dutch Fundamenteel Onderzoek der Materie (FOM).
Author information
Authors and Affiliations
Corresponding author
Ethics declarations
Competing interests
Reprints and permissions information is available at npg.nature.com/reprintsandpermissions. The authors declare no competing financial interests.
Supplementary information
Supplementary Notes
This file contains the Supplementary Discussion and Supplementary Figures 1-6.
Rights and permissions
About this article
Cite this article
Jarillo-Herrero, P., van Dam, J. & Kouwenhoven, L. Quantum supercurrent transistors in carbon nanotubes. Nature 439, 953–956 (2006). https://doi.org/10.1038/nature04550
Received:
Accepted:
Issue Date:
DOI: https://doi.org/10.1038/nature04550
This article is cited by
-
Suspended superconducting weak links from aerosol-synthesized single-walled carbon nanotubes
Nano Research (2020)
-
2D materials for quantum information science
Nature Reviews Materials (2019)
-
Geometric quenching of orbital pair breaking in a single crystalline superconducting nanomesh network
Nature Communications (2018)
-
Investigation of Supercurrent in the Quantum Hall Regime in Graphene Josephson Junctions
Journal of Low Temperature Physics (2018)
-
Coherent Charge Transport in Ballistic InSb Nanowire Josephson Junctions
Scientific Reports (2016)
Comments
By submitting a comment you agree to abide by our Terms and Community Guidelines. If you find something abusive or that does not comply with our terms or guidelines please flag it as inappropriate.