Ultrafast non-thermal control of magnetization by instantaneous photomagnetic pulses

Abstract

The demand for ever-increasing density of information storage and speed of manipulation has triggered an intense search for ways to control the magnetization of a medium by means other than magnetic fields1,2,3,4,5. Recent experiments on laser-induced demagnetization6,7,8 and spin reorientation9 use ultrafast lasers as a means to manipulate magnetization, accessing timescales of a picosecond or less. However, in all these cases the observed magnetic excitation is the result of optical absorption followed by a rapid temperature increase. This thermal origin of spin excitation considerably limits potential applications because the repetition frequency is limited by the cooling time10. Here we demonstrate that circularly polarized femtosecond laser pulses can be used to non-thermally excite and coherently control the spin dynamics in magnets by way of the inverse Faraday effect. Such a photomagnetic interaction is instantaneous and is limited in time by the pulse width (200 fs in our experiment). Our finding thus reveals an alternative mechanism of ultrafast coherent spin control, and offers prospects for applications of ultrafast lasers in magnetic devices.

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Figure 1: Magnetic excitations in DyFeO 3 probed by the magneto-optical Faraday effect.
Figure 2: Excitation of the spin oscillations in DyFeO 3 measured at different temperatures in the range between 20 K and 170 K.
Figure 3: Temperature dependence of the frequencies of the observed spin oscillations.

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Acknowledgements

We thank V. N. Gridnev for discussions, and T. Toonen and A. van Etteger for help with measurements. This work was partially supported by the European IST network SPINOSA, the RTN network DYNAMICS, the Russian Foundation for Basic Research (RFBR), de Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), and de Stichting voor Fundamenteel Onderzoek der Materie (FOM).

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Correspondence to Th. Rasing.

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Kimel, A., Kirilyuk, A., Usachev, P. et al. Ultrafast non-thermal control of magnetization by instantaneous photomagnetic pulses. Nature 435, 655–657 (2005). https://doi.org/10.1038/nature03564

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