Abstract
THE safe disposal of large quantities of high-level radioactive wastes from spent power reactor fuels, or reprocessing is a problem of considerable concern because of the danger which may arise from their release into the environment. We describe here a multi-barrier vitrification process which is conducted at moderate temperatures (below 900 °C) and which yields the fixation of radioactive wastes as oxides in a high-silica matrix. Some special characteristics of this process are discussed, including the excellent chemical durability, high thermal and structural stability of the glass, and the possibility of multibarrier protection.
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References
Cohen, B. L. Scient. Am. 236, 21–31 (1977).
McElroy, J. L. et al. Waste Solidification Program Summary Report: Vol. II, BNWL-1667 (Battelle, Pacific Northwest Laboratories, Richland, Washington, 1972).
Melson, W. G. & Thompson, G. Bull. geol. Soc. Am. 84, 703–716 (1973).
Bartlett, J. W. et al. Alternatives for Managing Wastes from Reactors and Post-Fission Operations in the LWR Fuel Cycle Vol. 2, ERDA 76–43 (1976).
Shand, E. B. Glass Engineering Handbook, Ch. 3 (McGraw Hill, New York, 1958).
Keller, W. D. & Huang, W. H. Acta universitatis Carolinae-geol. 4, 309–318 (1971).
Roedder, E. R. & Weiblen, P. W. Proc. 2nd Lunar Sci. Conf. 1, 507–528 (1971).
Shelby, J. E. Bull. Am. ceram. Soc. 57, 358 (1978).
Simmons, J. H., Macedo, P. B., Mohr, R. K. & Gupta, P. K. Molecular Stuffing Process for Making High Silica Glasses With Selected Properties (J. Am. Ceram. Soc. in the press).
Mohr, R. K. et al. Strengthening of Optical Fibers by Molecular Stuffing (J. Am. Ceram. Soc. in the press).
Chu, S. H. & Simmons, J. H. Bull. Am. ceram. Soc. 56, 803 (1977).
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SIMMONS, J., MACEDO, P., BARKATT, A. et al. Fixation of radioactive waste in high silica glasses. Nature 278, 729–731 (1979). https://doi.org/10.1038/278729a0
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DOI: https://doi.org/10.1038/278729a0
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