Article abstract


Nature Physics 4, 319 - 326 (2008)
Published online: 23 March 2008 | doi:10.1038/nphys917

Subject Categories: Condensed-matter physics | Materials physics

Evolution of the electronic excitation spectrum with strongly diminishing hole density in superconducting Bi2Sr2CaCu2O8+delta

J. W. Alldredge1, Jinho Lee1,2, K. McElroy3, M. Wang1, K. Fujita1, Y. Kohsaka1,4, C. Taylor1, H. Eisaki5, S. Uchida6, P. J. Hirschfeld7 & J. C. Davis1,8


Coulomb interactions between the carriers may provide the mechanism for enhanced unconventional superconductivity in the copper oxides. However, they simultaneously cause inelastic quasiparticle scattering that can destroy it. Understanding the evolution of this balance with doping is crucial because it is responsible for the rapidly diminishing critical temperature as the hole density p is reduced towards the Mott insulating state. Here, we use tunnelling spectroscopy to measure the Tright arrow0 spectrum of electronic excitations N(E) over a wide range of hole density p in superconducting Bi2Sr2CaCu2O8+delta. We introduce a parameterization for N(E) based on a particle–hole symmetric anisotropic energy gap Delta(k)=Delta1(cos(kx)-cos(ky))/2 plus an inelastic scattering rate that varies linearly with energy Gamma2(E)=alphaE. We demonstrate that this form of N(E) enables successful fitting of differential tunnelling conductance spectra throughout much of the Bi2Sr2CaCu2O8+delta phase diagram. We find that Delta1 values rise with falling p along the familiar trajectory of excitations to the 'pseudogap' energy, whereas the energy-dependent inelastic scattering rate Gamma2(E)=alphaE seems to be an intrinsic property of the electronic structure and rises steeply for p<16%. Such diverging inelastic scattering may play a key role in suppression of superconductivity in the copper oxides as the Mott insulating state is approached.

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  1. LASSP, Department of Physics, Cornell University, Ithaca, New York 14850, USA
  2. School of Physics and Astronomy, University of St Andrews, North Haugh, St Andrews KY16 9SS, Scotland
  3. Department of Physics, University of Colorado, Boulder, Colorado 8030, USA
  4. Magnetic Materials Laboratory, RIKEN, Wako 351-0198, Japan
  5. NI-AIST, 1-1-1 Central 2, Umezono, Tsukuba, Ibaraki 305-8568, Japan
  6. Department of Physics, University of Tokyo, Tokyo 113-8656, Japan
  7. Department of Physics, University of Florida, Gainesville, Florida 32611, USA
  8. CMP&MS Department, Brookhaven National Laboratory, Upton, New York 11973, USA

Correspondence to: J. C. Davis1,8 e-mail: jcdavis@ccmr.cornell.edu



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