Letter


Nature Physics 3, 91 - 95 (2007)
doi:10.1038/nphys507

Subject Categories: Quantum physics | Atomic and molecular physics | Information theory and computation

Experimental entanglement of six photons in graph states

Chao-Yang Lu1, Xiao-Qi Zhou1, Otfried Gühne2, Wei-Bo Gao1, Jin Zhang1, Zhen-Sheng Yuan1, Alexander Goebel3, Tao Yang1 and Jian-Wei Pan1,3


Graph states1, 2, 3—multipartite entangled states that can be represented by mathematical graphs—are important resources for quantum computation4, quantum error correction3, studies of multiparticle entanglement1 and fundamental tests of non-locality5, 6, 7 and decoherence8. Here, we demonstrate the experimental entanglement of six photons and engineering of multiqubit graph states9, 10, 11. We have created two important examples of graph states, a six-photon Greenberger–Horne–Zeilinger state5, the largest photonic Schrödinger cat so far, and a six-photon cluster state2, a state-of-the-art 'one-way quantum computer'4. With small modifications, our method allows us, in principle, to create various further graph states, and therefore could open the way to experimental tests of, for example, quantum algorithms4, 12 or loss- and fault-tolerant one-way quantum computation13, 14.


Entanglement lies at the heart of quantum mechanics and plays a crucial role in quantum-information processing. Many efforts have been undertaken to create, in particular, multipartite entangled states in different physical systems15, 16, 17, 18, where maximally up to eight ions have been entangled18. In recent years, special types of multipartite entangled states, the graph states1, 2, 3, have become the centre of attention. They can be associated with graphs where each vertex represents a qubit prepared in the state Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com and each edge represents a controlled phase gate having been applied between the two connected qubits. An interesting feature is that many entanglement properties of graph states are closely related to their underlying graphs1. Besides their thought-provoking theoretical structure, the graph states have also provided new insights into studies of non-locality6, 7, 19, 20 and decoherence8 and served as essential resources for various quantum-information tasks3, 4, most prominently as the exceptionally universal resource for one-way quantum computation4. Encouraging progress9, 10, 11, 12, 13, 14, 16 has been achieved in this direction, especially in the linear optics regime. Yet a major challenge ahead lies in the experimental generation of multiqubit graph states.

Of special interest in the graph-state family are the Greenberger–Horne–Zeilinger (GHZ) states and the cluster states. Experimentally, six-atom GHZ states17 and four-photon cluster states16 have been realized. Here, we report the creation of six-photon GHZ states and cluster states with verifiable six-partite entanglement. To do so, we start from three Einstein–Podolsky–Rosen (EPR) entangled photon pairs in the state

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where H and V denote horizontal and vertical polarization, and i and j label the spatial modes of the photons (see Fig. 1a). We superpose photons in mode 2 and 3 (4 and 5) at polarizing beam splitters (PBSs). As the PBS transmits H and reflects V polarization, only if both incoming photons have the same polarization can they go to different outputs21, 22. Thus, a coincidence detection of all six outputs corresponds to the state

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which is a six-photon GHZ state, exhibiting an equal superposition of two maximally different quantum states.

Figure 1: Scheme to generate the six-photon graph states and their representations in the graph-state picture.

Figure 1 : Scheme to generate the six-photon graph states and their representations in the graph-state picture.

a, The six-photon GHZ state (1) and cluster state (2) are created by combining three pairs of entangled photons at PBSs. The Hadamard gate (H) is inserted for generation of the cluster state. bd, Underlying graph of the six-photon graph states and how they are created by post-selected fusion operations. The graph state can be thought of as being constructed by first preparing the qubits at each vertex in the state Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com and then applying controlled phase gates between pairs of neighbouring qubits. Here, we use the post-selected fusion operations, that is, combining photons at PBS, to generate multiqubit graph states efficiently. In the star graph, we refer to the central node as the root and the others as leaves.

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By applying a Hadamard gate on photon 4 before it enters into the PBS (see Fig. 1a), the above scheme can be readily modified to generate a six-photon cluster state. It can be considered in two steps: (1) combine photons 2 and 3, such that, on the basis of a coincidence detection, we get a four-photon GHZ state Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com, where Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com; (2) combine photons 4 and 5, and by a similar reasoning we obtain what we call here a six-photon cluster state

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For an intuitive understanding, in Fig. 1 we show the underlying graph of the above states and how they grow from smaller (two-qubit) graph states. Up to local unitary transformations, the GHZ states correspond to star-shaped graphs, and the cluster states to lattice graphs. The effect of combining two photons at PBS can be described by the operator |HHright fenceleft fenceHH|+|VV right fenceleft fenceVV |, leading to the fusion of two separate graph states into a single one10, 11. Specifically, Fig. 1c (d) shows that when a two-qubit graph state is combined with the root (leaf) node of a four-qubit star graph, a six-qubit GHZ (cluster) state is produced.

A nice feature of the graph-state representation is that many properties of the graph states and their potential use in quantum-information processing can be revealed by their underlying graph. For example, the star-graph states have multiple leaf nodes, which are referred to as microclusters in refs 9,13 and can be used in the so-called parallel fusion for building up large cluster states. The graph of the six-qubit cluster state (2) forms a standard quantum circuit under the one-way computer model4. Moreover, its geometry embodies a tree-shaped graph, which is the basic building block for loss-tolerant one-way quantum computing14. Another interesting feature of the cluster state is that not only itself, but even the remaining mixed four-qubit state after two qubits have been traced out, leads to a GHZ argument for non-locality6, showing a surprisingly strong entanglement persistency.

Let us now proceed with the experimental demonstration. In our experiment, we use spontaneous parametric down-conversion to produce entangled photons23. We made various efforts to prepare high-brightness and stable sources of entangled photons (see the Methods section). The set-up is illustrated in Fig. 2. A pulsed ultraviolet laser successively passes through three beta-barium borate (BBO) crystals to generate entangled photon pairs in spatial modes 1–2, 3–4 and 5–6. The photon pairs are prepared in the state |Phi+right fence with an average two-fold coincidence count of about 9.3times104 s-1 and a visibility of 93% (91%) in the H/V (+/-) basis. We then superpose photons 2 (4) and 3 (5) at the PBS. To achieve good spatial and temporal overlap, the photons are spectrally filtered (DeltalambdaFWHW=3.2 nm) and detected by fibre-coupled single-photon detectors. By making fine adjustments of delay Deltad1 (Deltad2), we are able to observe interference fringes of four-photon entanglement with a visibility of 73% (71%) in mode 1–2–3–4 (3–4–5–6), indicating that the post-selected fusion operations have been successfully implemented (see the Supplementary Information).

Figure 2: Experimental set-up for the generation of six-photon graph states.

Figure 2 : Experimental set-up for the generation of six-photon graph states.

Pumped by a continuous-wave (CW) green laser, the mode-locked Ti:sapphire laser outputs a pulsed infrared laser with a central wavelength of 788 nm, a pulse duration of 120 fs and a repetition rate of 76 MHz, which passes through an LBO crystal (mounted on a motorized translation stage) and is up-converted to ultraviolet (lambda=394 nm). The ultraviolet laser beam is circularized and focused on the three BBO crystals to produce three pairs of entangled photons. The entangled photons are spectrally filtered by narrow-band filters (with a peak transmission rate of approx98%) and then detected by fibre-coupled single-photon detectors (D1T,...,D6R). We use a programmable multichannel coincidence unit to register the multi-fold coincidence events. For polarization analysis, half- and quarter-wave plates (HWP, QWP) together with polarizers or PBSs are used. By changing the angle (theta) of the HWP at path 4, our set-up is tunable to generate the six-photon GHZ states (theta=0°) and cluster state (theta=22.5°).

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Now we analyse the experimental data of six-photon graph states and characterize the entanglement produced here. Let us first discuss to what extent the desired states were produced and the presence of genuine multipartite entanglement. The quality of the states can be judged by the fidelity, that is, the overlap of the produced state with the desired one. The notion of genuine multipartite entanglement characterizes whether generation of the state requires interaction of all parties: a pure state |Psiright fence is called biseparable, whenever a grouping of the six parties into two groups GA and GB can be found, such that the state is a product state, that is Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com, otherwise it is a genuine multipartite entangled state. Consequently, a mixed state is called biseparable, if it is a mixture of biseparable pure states, otherwise it is a genuine multipartite entangled state.

To prove multipartite entanglement, we use the method of entanglement witnesses25. An entanglement witness is an observable that has a positive expectation value on all biseparable states. Thus, a negative expectation value proves the presence of genuine multipartite entanglement. In what follows, we derive efficient entanglement witnesses that are both robust against realistic noise and economical for experimental efforts.

For the six-photon GHZ state (1), we use the witness25

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where I denotes the identity operator. We decompose |G6right fenceleft fenceG6| into locally measurable observables

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where M(n)=cos(npi/6)sigmax+sin(npi/6)sigmay are measurements in the xy plane. To implement this witness, seven measurement settings are required. Figure 3 shows the measurement results, yielding Tr(WGrhoexp)=-0.093plusminus0.025, which is negative by 3.7 standard deviations and thus proves the presence of genuine six-partite entanglement.

Figure 3: Experimental result of the six-photon GHZ state(1).

Figure 3 : Experimental result of the six-photon GHZ state(1).

a, Six-fold coincidence counts in H/V basis in 3 h. b, The expectation values of Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com, each derived from a complete set of 64 six-fold coincidence events in 2 h in measurement basis |Hright fenceplusminuse inpi/6|V right fence. The error bars represent one standard deviation, deduced from propagated poissonian counting statistics of the raw detection events.

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From the expectation value of the witness, we can directly determine the obtained fidelity as FG6=left fenceG6|rhoexp|G6right fence=0.593plusminus0.025, where rhoexp denotes the experimentally produced state. This is a considerable improvement over the fidelity of the six-atom GHZ states17 (F=0.509plusminus0.004).

For the cluster state (2), a possible witness would be WC=I/2-|C6right fenceleft fenceC6| (ref. 26). Similar to the constructions of ref. 26, we use a slightly different witness Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com, the implementation of which requires only six measurements (see the Methods section). Figure 4 shows the measurement results in basis Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com, which together with those of the four other bases Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com and Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com (see the Supplementary Information), gives Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com. Thus, the genuine six-partite entanglement of the cluster state is also proved. Furthermore, from this result, we can obtain a lower bound of the fidelity of our cluster state as FC6greater than or equal to0.595plusminus0.036.

Figure 4: The stabilizer operators and experimental result of the six-photon cluster state(2).

Figure 4 : The stabilizer operators and experimental result of the six-photon cluster state(2).

a, The graph corresponds to the cluster state |C6right fence under H transformations on qubits 1, 3, 4 and 6 and its stabilizer operators gi, where i labels the qubits and X=sigmax,Y =sigmay,Z=sigmaz. The graph state is a common eigenstate of these stabilizer operators, that is, gi|C6right fence=|C6right fence, which describe the correlations in the state. The cluster state is the unique state fulfilling this, which allows for an alternative definition of it. b,c, Six-fold coincidence counts measured in the Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com and Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com basis in 3 h, each signals the observation of an eigenstate of the stabilizer operator (gi) with the corresponding eigenvalue of vj=+1 or -1. From the probabilities of multiphoton detections pj,j=1,2,...,64, we can then compute the expectation values of stabilizer operators by Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com.

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For an investigation of the bipartite entanglement properties of these graph states, we estimate the entanglement of formation from the expectation value of the witness27. Here, different bipartitions arise when the six parties are divided into two groups. The entanglement of formation EF(rho) is an entanglement measure for bipartite systems, quantifying how many EPR pairs are needed for the formation of the state28. For the GHZ state (1), we find that for all bipartitions at least EF(rhoexp)greater than or equal to0.073plusminus0.032. For the cluster state (2), EF(rhoexp) is also always positive, for some bipartitions it is even EF(rhoexp)greater than or equal to0.729plusminus0.106. A full discussion, also for a different entanglement measure, is given in the Supplementary Information.

The imperfections of our graph states are mainly caused by two reasons. First, high-order emissions of entangled photons give rise to the undesired components in the H/V basis (see Fig. 3a). Second, the partial distinguishability of independent photons causes some incoherent mixtures. In spite of the imperfections, genuine entanglements of the six-photon graph states are strictly confirmed. It is possible to improve the fidelity in future experiments, for example, by using photon-number discriminating detectors to filter out the events of double emissions of photon pairs. Moreover, graph states with high purity can be obtained efficiently using the existing entanglement purification scheme29. The linear optical elements such as the PBS may offer a high-accuracy tool for this task30. It leaves a crucial open question of how to reach the noise thresholds for optical cluster-state quantum computation13.

Some further remarks are warranted here. We generate the graph states conditioned on there being one and only one photon in each of the six outputs. This post-selective feature, on the one hand, together with the fusion method, provides a flexible and economical way to create various multiphoton graph states. Slight modifications of our experimental set-up will readily allow the creation of many other graph states, for example, six-qubit linear and Y-shaped graph states (see the Supplementary Information). Such a fascinating capacity creates a useful multiqubit graph-state test-bed. On the other hand, this feature does not prohibit subsequent applications such as tests of quantum non-locality5, 6, 7 and in-principle verifications of linear optical quantum-information processing tasks where photons need to be eventually detected. Finally, concerning the scalability issue, we refer to ref. 11, which has shown that if combined with quantum memory, the post-selection method can even be used for scalable generation of tree-graph states using realistic linear optics. Along this line, however, technically extensive efforts still need to be undertaken to make a quantum memory usable for this purpose.

In summary, we have realized two special graph states, the six-photon GHZ state, the largest photonic Schrödinger cat so far, and the six-photon cluster state—a state-of-the-art one-way quantum computer. We have demonstrated the ability to entangle six photons and to engineer multiqubit graph states, and have created a versatile test-bed for experimental investigations of one-way quantum computation4, quantum error correction3, studies of multiparticle entanglement1 and foundational tests of quantum physics5, 6, 7, 8. Combined with quantum memory, our experimental method could lead to the generation of large-scale tree-graph states11. The high efficiency and flexibility of the six-photon graph-state generation we demonstrated here suggest that photons manipulated with linear optics are promising candidates for engineering of multiqubit graph states. Various applications of our six-photon graph-state test-bed can be imagined. For instance, the six-qubit cluster states allow full implementations of the quantum game of prisoners' dilemma12 and a proof-of-principle demonstration of the basic elements of loss-tolerant one-way quantum computation14. Most remarkably, the six-qubit star-ring graph state corresponds to the codeword and encoding procedure of the five-qubit quantum error-correction code that is able to correct all one-qubit errors3. In addition, our six-photon cluster state also enables a novel test of non-locality, namely a GHZ argument of non-locality for mixed states6. Lastly, the graph-state test-bed is well suited for studies of the stabilities of different types of multiparticle entanglement (for example, GHZ and cluster) under the influence of decoherence, which may provide experimental evidence for the surprising conclusion in ref. 8 that genuine entanglement of a macroscopic number of particles is possible and can persist for timescales that are independent of the size of the system.

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Methods

Optimizing the six-photon set-up

To get high-brightness entangled photons, similarly to ref. 24 we used the high-power Verdi-18/Mira-900F femtosecond laser system that outputs a stable pulsed infrared laser with a power of 2.4 W. In addition, we adopted a new three-BBO-crystal configuration for a more flexible optimization of three independent photon pairs. Moreover, the use of narrow-band filters in our experiment with peak transmission rates as high as 98% considerably improved the collection efficiency. To make our set-up stable, we first made efforts to minimize the fluctuation of the pump power. As shown in Fig. 2, we mounted the LiB3O5 (LBO) crystal on a motorized translation stage controlled by a computer program to avoid damage to the crystal by the focusing laser beam. By doing this, we achieved both good up-conversion efficiency (approx38%) and long life time for LBO, making it a very stable ultraviolet laser source with a power of 0.91 W that typically drops by less than 1.5% over weeks. Our feedback control system has greatly improved the stability of the down-conversion rates: the measured coincidence counts typically fluctuate by approx3% over two weeks, whereas without it the counts drop significantly after about 15 min (see the Supplementary Information for a curve of the measured two-fold coincidences over time). Second, we used a programmable multi-channel coincidence unit that allowed us to simultaneously register any possible coincidence detection between the inputs. Aside from the desired six-fold coincidence events, we also registered other combinations (such as single counts and two-fold coincidences), so we were able to track the performance of our system in real time. Any power drift could be deduced from the recorded count rates, and finally the six-fold coincidences were corrected for their difference. Thus, we were able to achieve a stable set-up, good collection efficiencies and three EPR pairs with high visibilities.

Cluster-state witness construction

The witness for the cluster state (2) can be constructed as follows. Using the results of ref. 26, the observable WC=I/2-|C6right fenceleft fenceC6| is a witness detecting genuine multipartite entanglement around the cluster state. Then, we consider the observable

Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com

where gi denotes the stabilizing operators of the cluster state (see Fig. 4a). Furthermore, we use A0=I-|HHHright fenceleft fenceHHH|-|VVV right fenceleft fenceVVV |, A1=|VVV right fenceleft fenceVVV |-|HHHright fenceleft fenceHHH| and Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com, where M(i) is defined as for the GHZ state (see equation (3)). Finally, Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com denotes a cluster state with different signs, namely Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com.

It is clear that Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com, which implies that Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com is a valid witness26. Furthermore, this implies that the fidelity of the cluster state can be estimated as Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com.

The witness Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com(4) detects genuine entanglement from the states of the form rho(p)=p|C6right fenceleft fenceC6|+(1-p)I/64 for p>0.5. The determination of the expectation value of the witness Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com requires six measurement settings, namely Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com, Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com, Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com and Unfortunately we are unable to provide accessible alternative text for this. If you require assistance to access this image, or to obtain a text description, please contact npg@nature.com. The results are shown in Fig. 4 in the main text and in Supplementary Information, Fig. S3.

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Acknowledgements

We thank H. J. Briegel, D. Browne, L.-M. Duan, T. Rudolph and S. Yu for helpful discussions. This work was supported by the National Natural Science Foundation of China, the Chinese Academy of Sciences. This work was also supported by the Alexander von Humboldt Foundation, the Marie Curie Excellence Grant of the EU, the FWF, the DFG and EU (Scala, Olaqui, Prosecco, QICS, Quprodis).

Competing interests statement:

The authors declare that they have no competing financial interests.

Received 18 September 2006; Accepted 5 December 2006; Published online 14 January 2007.

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  1. Hefei National Laboratory for Physical Sciences at Microscale and Department of Modern Physics, University of Science and Technology of China, Hefei, Anhui 230026, People's Republic of China
  2. Institut für Quantenoptik und Quanteninformation, Österreichische Akademie der Wissenschaften, Technikerstras zlige 21A, A-6020 Innsbruck, Austria
  3. Physikalisches Institut, Universität Heidelberg, Philosophenweg 12, D-69120 Heidelberg, Germany

Correspondence to: Chao-Yang Lu1 e-mail: cylu@mail.ustc.edu.cn

Correspondence to: Jian-Wei Pan1,3 e-mail: jian-wei.pan@physi.uni-heidelberg.de

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