Abstract
Near-infrared lasers are important for optical data communication, spectroscopy and medical diagnosis. Semiconductor nanowires offer the possibility of reducing the footprint of devices for three-dimensional device integration and hence are being extensively studied in the context of optoelectronic devices1,2. Although visible and ultraviolet nanowire lasers have been demonstrated widely3,4,5,6,7,8,9,10,11, progress towards room-temperature infrared nanowire lasers has been limited because of material quality issues and Auger recombination12,13. (Al)GaAs is an important material system for infrared lasers that is extensively used for conventional lasers. GaAs has a very large surface recombination velocity, which is a serious issue for nanowire devices because of their large surface-to-volume ratio14,15. Here, we demonstrate room-temperature lasing in core–shell–cap GaAs/AlGaAs/GaAs nanowires by properly designing the Fabry–Pérot cavity, optimizing the material quality and minimizing surface recombination. Our demonstration is a major step towards incorporating (Al)GaAs nanowire lasers into the design of nanoscale optoelectronic devices operating at near-infrared wavelengths.
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Acknowledgements
The authors acknowledge the Australian Research Council (ARC) for financial support, the National Computational Infrastructure (NCI) for providing the computational resources used for this work, and the Australian Nano Fabrication Facility (ANFF) for technical support. The authors thank M. Lysevych, P. Sajewicz, K. Vora and P. Caroff for fruitful discussions.
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D.S., S.M., H.T. and C.J. conceived and designed the experiments. D.S. and S.M. carried out the modelling and theoretical analysis. N.J. and Q.G. optimized the growth conditions for the nanowires. D.S., S.M. and P.P. carried out the experiments. D.S. and S.M. wrote the manuscript, with contributions from all authors. D.S. and S.M. contributed equally to this work.
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Saxena, D., Mokkapati, S., Parkinson, P. et al. Optically pumped room-temperature GaAs nanowire lasers. Nature Photon 7, 963–968 (2013). https://doi.org/10.1038/nphoton.2013.303
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DOI: https://doi.org/10.1038/nphoton.2013.303
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