Abstract
Optical nonlinearities at the single-photon level are key ingredients for future photonic quantum technologies1. Prime candidates for the realization of the strong photon–photon interactions necessary for implementing quantum information processing tasks2, as well as for studying strongly correlated photons3,4,5,6 in an integrated photonic device setting, are quantum dots embedded in photonic-crystal nanocavities. Here, we report strong quantum correlations between photons on picosecond timescales. We observe (i) photon antibunching upon resonant excitation of the lowest-energy polariton state, proving that the first cavity photon blocks the subsequent injection events, and (ii) photon bunching when the laser field is in two-photon resonance with the polariton eigenstates of the second Jaynes–Cummings manifold7,8, demonstrating that two photons at this colour are more likely to be injected into the cavity jointly than they would otherwise. Together, these results demonstrate unprecedented strong single-photon nonlinearities, paving the way for the realization of a quantum optical Josephson interferometer9 or a single-photon transistor10.
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References
O'Brien, J. L., Furusawa, A. & Vučković, J. Photonic quantum technologies. Nature Photon. 3, 687–695 (2009).
Mabuchi, H. & Doherty, A. C. Cavity quantum electrodynamics: coherence in context. Science 298, 1372–1377 (2002).
Hartmann, M. J., Brandão, F. G. S. L. & Plenio, M. B. Strongly interacting polaritons in coupled arrays of cavities. Nature Phys. 2, 849–855 (2006).
Greentree, A. D., Tahan, C., Cole, J. H. & Hollenberg, L. C. L. Quantum phase transitions of light. Nature Phys. 2, 856–861 (2006).
Angelakis, D. G., Santos, M. F. & Bose, S. Photon blockade induced Mott transitions and XY spin models in coupled cavity arrays. Phys. Rev. A 76, 031805(R) (2007).
Carusotto, I. et al. Fermionized photons in an array of driven dissipative nonlinear cavities. Phys. Rev. Lett. 103, 033601 (2009).
Kubanek, A. et al. Two-photon gateway in one-atom cavity quantum electrodynamics. Phys. Rev. Lett. 101, 203602 (2008).
Schneebeli, L., Kira, M. & Koch, S. W. Characterization of strong light–matter coupling in semiconductor quantum-dot microcavities via photon-statistics spectroscopy. Phys. Rev. Lett. 101, 097401 (2008).
Gerace, D., Türeci, H. E., Imamoğlu, A., Giovannetti, V. & Fazio, R. The quantum optical Josephson interferometer. Nature Phys. 5, 281–284 (2009).
Chang, D. E., Sørensen A. S., Demler, E. A. & Lukin, M. A single-photon transistor using nanoscale surface plasmons. Nature Phys. 3, 807–812 (2007).
Imamoğlu, A., Schmidt, H., Woods, G. & Deutsch, M. Strongly interacting photons in a nonlinear cavity. Phys. Rev. Lett. 79, 1467–1470 (1997).
Brune, M. et al. Quantum Rabi oscillations: a direct test of field quantization in a cavity. Phys. Rev. Lett. 76, 1800–1803 (1996).
Yoshie, T. et al. Vacuum Rabi splitting with a single quantum dot in a photonic-crystal nanocavity. Nature 432, 200–203 (2004).
Reithmaier, J. P. et al. Strong coupling in a single quantum dot–semiconductor microcavity system. Nature 432, 197–200 (2004).
Peter, E. et al. Exciton–photon strong-coupling regime for a single quantum dot embedded in a microcavity. Phys. Rev. Lett. 95, 067401 (2005).
Hennessy, K. et al. Quantum nature of a strongly coupled single quantum dot–cavity system. Nature 445, 896–899 (2007).
Fink, J. M. et al. Climbing the Jaynes–Cummings ladder and observing its nonlinearity in a cavity QED system. Nature 454, 315–318 (2008).
Deppe, F. et al. Two-photon probe of the Jaynes–Cummings model and controlled symmetry breaking in circuit QED. Nature Phys. 4, 686–691 (2008).
Bishop, L. S. et al. Nonlinear response of the vacuum Rabi resonance. Nature Phys. 5, 105–109 (2009).
Birnbaum, K. M. et al. Photon blockade in an optical cavity with one trapped atom. Nature 436, 87–90 (2005).
Dayan, B. et al. A photon turnstile dynamically regulated by one atom. Science 319, 1062–1065 (2008).
Faraon, A. et al. Coherent generation of non-classical light on a chip via photon-induced tunneling and blockade. Nature Phys. 4, 859–863 (2008).
Kasprzak, J. et al. Up on the Jaynes–Cummings ladder of a quantum-dot/microcavity system. Nature Mater. 9, 304–308 (2010).
Moser, S. et al. Scanning a photonic-crystal slab nanocavity by condensation of xenon. Appl. Phys. Lett. 87, 141105 (2005).
Englund, D. et al. Controlling cavity reflectivity with a single quantum dot. Nature 450, 857–861 (2007).
Srinivasan, K. & Painter, O. Linear and nonlinear optical spectroscopy of a strongly coupled microdisk–quantum dot system. Nature 450, 862–866 (2007).
Santori, C. et al. Submicrosecond correlations in photoluminescence from InAs quantum dots. Phys. Rev. B 69, 205324 (2004).
Manson, N. B. & Harrison, J. P. Photo-ionization of the nitrogen-vacancy centre in diamond. Diam. Rel. Mater. 14, 1705–1710 (2005).
Mohan, A. et al. Polarization-entangled photons produced with high-symmetry site-controlled quantum dots. Nature Photon. 4, 302–306 (2010).
Gallo, P. et al. Integration of site-controlled pyramidal quantum dots and photonic-crystal membrane cavities. Appl. Phys. Lett. 92, 263101 (2008).
Bennett, A. J. et al. Giant Stark effect in the emission of single semiconductor quantum dots. Appl. Phys. Lett. 97, 031104 (2010).
Duan, L-M. & Kimble, H. J. Scalable photonic quantum computation through cavity-assisted interactions. Phys. Rev. Lett. 92, 127902 (2004).
Acknowledgements
This work was supported by the National Centre of Competence in Research, Quantum Photonics (NCCR QP), a research instrument of the Swiss National Science Foundation (SNSF), and a European Research Council (ERC) Advanced Investigator Grant (A.I.). The authors thank I. Carusotto for helpful discussions.
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A.R. and T.V. conducted the experiments, analysed the data and performed the simulations. M.W. made essential contributions to the experiment in its early stages. A.B., K.J.H. and E.L.H. fabricated the structure that ensures maximal dot–cavity coupling. A.R., T.V. and A.I. conceived the experiment, discussed the results and wrote the manuscript.
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Reinhard, A., Volz, T., Winger, M. et al. Strongly correlated photons on a chip. Nature Photon 6, 93–96 (2012). https://doi.org/10.1038/nphoton.2011.321
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DOI: https://doi.org/10.1038/nphoton.2011.321
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