Letter abstract


Nature Nanotechnology 4, 30 - 33 (2009)
Published online: 7 December 2008 | doi:10.1038/nnano.2008.365

Subject Categories: Nanomaterials | Synthesis and processing

Gram-scale production of graphene based on solvothermal synthesis and sonication

Mohammad Choucair1, Pall Thordarson1 & John A. Stride1,2


Carbon nanostructures have emerged as likely candidates for a wide range of applications, driving research into novel synthetic techniques to produce nanotubes, graphene and other carbon-based materials. Single sheets of pristine graphene have been isolated from bulk graphite in small amounts by micromechanical cleavage1, and larger amounts of chemically modified graphene sheets have been produced by a number of approaches2, 3, 4, 5, 6, 7. Both of these techniques make use of highly oriented pyrolitic graphite as a starting material and involve labour-intensive preparations. Here, we report the direct chemical synthesis of carbon nanosheets in gram-scale quantities in a bottom-up approach based on the common laboratory reagents ethanol and sodium, which are reacted to give an intermediate solid that is then pyrolized, yielding a fused array of graphene sheets that are dispersed by mild sonication. The ability to produce bulk graphene samples from non-graphitic precursors with a scalable, low-cost approach should take us a step closer to real-world applications of graphene.

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  1. School of Chemistry, University of New South Wales, Sydney 2052, Australia
  2. Bragg Institute, Australian Nuclear Science and Technology Organisation, PMB 1, Menai, New South Wales 2234, Australia

Correspondence to: John A. Stride1,2 e-mail: j.stride@unsw.edu.au



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