Article abstract


Nature Materials 7, 203 - 208 (2008)
Published online: 17 February 2008 | doi:10.1038/nmat2123

There is an Erratum (21 February 2008) associated with this Article.

Subject Categories: Electronic materials | Semiconductors | Optical, photonic and optoelectronic materials | Magnetic materials

Zero-field optical manipulation of magnetic ions in semiconductors

R. C. Myers1, M. H. Mikkelsen1, J.-M. Tang2,3, A. C. Gossard1, M. E. Flatté2 & D. D. Awschalom1


Controlling and monitoring individual spins is desirable for building spin-based devices, as well as implementing quantum information processing schemes. As with trapped ions in cold gases, magnetic ions trapped on a semiconductor lattice have uniform properties and relatively long spin lifetimes. Furthermore, diluted magnetic moments in semiconductors can be strongly coupled to the surrounding host, permitting optical or electrical spin manipulation. Here we describe the zero-field optical manipulation of a few hundred manganese ions in a single gallium arsenide quantum well. Optically created mobile electron spins dynamically generate an energy splitting of the ion spins and enable magnetic moment orientation solely by changing either photon helicity or energy. These polarized manganese spins precess in a transverse field, enabling measurements of the spin lifetimes. As the magnetic ion concentration is reduced and the manganese spin lifetime increases, coherent optical control and readout of single manganese spins in gallium arsenide should be possible.

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  1. Center for Spintronics and Quantum Computation, University of California, Santa Barbara, California 93106, USA
  2. Optical Science and Technology Center and Department of Physics and Astronomy, University of Iowa, Iowa City, Iowa 52242, USA
  3. Present address: Department of Physics, University of New Hampshire, Durham, New Hampshire 03824, USA

Correspondence to: D. D. Awschalom1 e-mail: awsch@physics.ucsb.edu



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