Abstract
One leading candidate theory of high-temperature superconductivity in the copper oxide systems is the interlayer tunnelling (ILT) mechanism1. In this model, superconductivity is created by tunnelling of electron pairs between the copper oxide planes — contrasting with other models in which superconductivity first arises by electron pairing within each plane. The ILT model predicts that the superconducting condensation energy is approximately equal to the gain in kinetic energy of the electron pairs due to tunnelling. Both these energies can be determined independently2,3,4, providing a quantitative test of the model. The gain in kinetic energy of the electron pairs is related to the interlayer plasma frequency, ωJ, of electron pair oscillations, which can be measured using infrared spectroscopy. Direct imaging of magnetic flux vortices also provides a test5, which is performed here on the same samples. In the high-temperature superconductor Tl2Ba2CuO6, both the sample-averaging optical probe and the local vortex imaging give a consistent value of ωJ ≈ 28 cm−1 which, when combined with the condensation energy, produces a discrepancy of at least an order of magnitude with deductions based on the ILT model.
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Acknowledgements
We thank M. Bhushan and M. Ketchen for assistance with the development of the scanning SQUID microscope; P. W. Anderson for comments; and P. Stamp for reading the manuscript. K.A.M. acknowledges the support of an R. H. Dicke postdoctoral fellowship. This work was supported by the Netherlands Foundation for Fundamental Research on Matter (FOM) with financial aid from the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO). A.A.T. acknowledges the support of NWO, RFBR and the Russian Superconductivity Program. The work performed at SUNY-Buffalo was partly supported by NYSERDA.
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Tsvetkov, A., van der Marel, D., Moler, K. et al. Global and local measures of the intrinsic Josephson coupling in Tl2Ba2CuO6 as a test of the interlayer tunnelling model. Nature 395, 360–362 (1998). https://doi.org/10.1038/26439
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DOI: https://doi.org/10.1038/26439
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