Abstract
Recently discovered Weyl semimetals have received considerable research interest due to the exotic Weyl fermion-like excitations and the nontrivial π Berry phase near the band degenerate points. Here we show that by constructing a Weyl semimetal p–n–p junction and restricting Weyl fermions into closed orbits with electric and magnetic confinements, the Berry phase acquired by the Weyl fermions can be controlled flexibly. This brings out two effects on electron transport through the junction: when the Berry phase is integer multiples of π an obvious phase shift is observed in the transmission map, whereas for non-integer ones of Berry phase the transmission shows strong chirality dependence and a large chiral or valley-level splitting can be induced. Utilizing this chirality splitting, we further propose a new method to measure the Berry phase in Weyl semimetals, which shows accuracy for various potential profiles and has practical applications in experiments.
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Introduction
Quasi-particles in solid-state physics with dressed exotic properties have deep analogies with particle physics. The discovery of Weyl fermions in topological Weyl semimetals (WSMs) is one such case1,2,3,4,5,6,7,8. WSMs are characterized by the linear band crossing points in momentum space, known as the Weyl nodes. Excitations near the Weyl node can be described by a massless Weyl Hamiltonian \(H = \mathop {\sum}\limits_i {v_i} \hat p_i\sigma _i\) (i = x, y, z) with σi the Pauli matrix and vi the Fermi velocity. Here, the sign of \(\mathop {\prod}\limits_i {v_i}\) determines the chirality of the node. Weyl nodes with opposite chirality always appear or annihilate in pairs according to the Nielsen–Ninomiya theorem9 and are topologically robust against translational symmetry invariant perturbations10. Similar to the chiral anomaly in quantum field theory11,12, when applying a parallel magnetic field B and electric field E, an electron flow between different Weyl nodes can be induced, manifesting as a quadratic negative magnetoresistance in transport experiments13,14,15,16,17,18. Besides, any two-dimensional cross-section between the Weyl nodes with opposite chirality obtains a nonzero Chern number, resulting in the Fermi arc states in the surface Brillouin zone1. Observing these Fermi arc states has been an important way to identify WSMs in angle-resolved photoemission spectroscopy measurements19,20,21,22,23.
In addition to the chiral anomaly and topological Fermi arcs, the nontrivial Berry phase is another important characteristic of WSMs associated to their topological properties24,25,26,27. As the Weyl node with positive (negative) chirality acts like a source (drain) of Berry curvature in momentum space, Weyl fermions moving around one loop enclosing the Weyl node would acquire a π Berry phase. Experimentally detecting this π Berry phase can provide evidence for the existence of Weyl nodes. One commonly used way is to measure the magnetic Shubnikov-de Haas (SdH) oscillation in three-dimensional (3D) semimetals and extrapolate the phase shift by plotting the inverse magnetic field 1/B as a function of the Landau level index n28,29. However, distinguishing the peak position from the resistance oscillation is nontrivial and may lead to inaccurate results30. Furthermore, to reach the quantum limit a relatively high magnetic field is demanded, which increases the difficulty of experimental implementations29.
In this paper, we investigate the electron transport through a WSM p–n–p junction and propose a new method to measure the Berry phase and to generate the chirality-polarized current in WSMs. We show that by confining the Weyl fermions into closed orbits using both electric and magnetic fields, the Berry phase of the Weyl fermions with different chiralities has opposite signs and shows significant influence on the transport properties. When the Weyl fermions move in the plane which is perpendicular with the magnetic filed, the Berry phase undergoes a π jump as varying the incident angle and an obvious phase shift can be observed in the transmission spectrum, which is similar to the graphene p–n–p junction case31,32. However, when the Weyl fermions have nonzero momentum component parallel with the magnetic field, the Berry phase takes non-integer multiples of π and would induce a large chiral or valley-level splitting. We give a semiclassical analysis for this chirality-dependent transport based on the Einstein–Brillouin–Keller (EBK) quantization rule33,34 and propose a new method to measure the Berry phase utilizing the chirality (valley) splitting. Compared with the traditional SdH oscillation measurement, this method is accurate for various potential profiles and does not require a high magnetic field, which can work as a practical way to explore the nontrivial Berry phase in 3D semimetals in real expermiments.
Results
Theoretical model
We consider a WSM p–n–p junction shown in Fig. 1a. The central n region with length 2L is defined by a potential well U(x) and a uniform magnetic field B is applied in the z-direction to tune the real-space orbit of the Weyl fermions. The Weyl fermions are then confined inside the junction as shown in Fig. 1b (blue region). The Hamiltonian of the pristine WSM can be written in the two-band form35: \(\hat H = \mathop {\sum}\limits_{\mathbf{k}} {c_{\mathbf{k}}^\dagger } H({\mathbf{k}})c_{\mathbf{k}}\), with ck = (ck↑, ck↓)T being the annihilation operator with wave vector k and H(k) = tz(2 − coskxa − coskya − coskza) · σz + txsinkxa · σx + tysinkya · σy. Here, ti with i = x, y, z is the hopping energy in the i-direction, a is the lattice constant, and σ = (σx, σy, σz) is the Pauli matrix vector acting on the spin space. The system we consider satisfies the inversion symmetry but breaks the time-reversal symmetry and only harbors two Weyl nodes in the first Brillouin zone, which are located at K± = (0, 0, ±π/2a).
Expanding H(k) around the two Weyl nodes, we obtain the low-energy effective Hamiltonian for the Weyl fermions:
Here τ = ± 1 denotes the Weyl node with positive (negative) chirality or different valleys and \(\tilde k_z = k_z - \tau \pi /2a\) is the displacement of kz component measured from K±. The Fermi velocity is defined with vi = tia/ħ and for simplicity we just set ti = t and vi = v = ta/ħ in the following calculations. Note that the following results in this paper applies to the small Fermi energy range where the above linear expansion on the Hamiltonian H(k) works. For the Fermi energy away from the Weyl nodes, the chirality is ill-defined and the effective Hamiltonian Hτ(k) can not well describe the quasi-particle excitations.
Considering the presence of the potential well U(x) and magnetic filed B, and substituting the wave vector ki by the momentum operator \(\hat p_i/\hbar = - i\frac{\partial }{{\partial i}}\), the low-energy effective Hamiltonian can be written into the following form:
where the vector potential A = (0, Bx, 0) has been included through the minimal coupling. As the system has translational symmetry along y and z directions, the eigen-wavefunction can be written as \(\Psi ({\mathbf{r}}) = {\mathrm{e}}^{ip_yy/\hbar }{\mathrm{e}}^{ip_zz/\hbar }\varphi (x)\), where r = (x, y, z) and φ(x) is the x-component of Ψ(r). The Weyl equation \(\hat H_\tau \Psi ({\mathbf{r}}) = E\Psi ({\mathbf{r}})\) can be reduced to the differential equation \(\hat H_{\tau ,x}\varphi (x) = E\varphi (x)\) with
where Πy = py + eBx is the kinetic momentum in the y direction.
Semiclassical analysis
Before performing a quantum mechanical calculation, we first make the semiclassical analysis on Hamiltonian \(\hat H_{\tau ,x}\) and estimate the bound levels inside the p–n–p junction using the EBK quantization rule33,34. The Berry phase’s role in affecting the chiral levels can be seen clearly here.
To apply the quantization rule, we first substitute the operator −iħ∂x in Eq. (3) into symbol px using the Weyl correspondence36,37 and then arrive at the classical Hamiltonian matrix:
Solving the eignenvalues of the matrix Hτ, we get the following Hamiltonian–Jacobi equation:
where the ± sign corresponds to the electron or hole solution. The above equation determines the classical turning points xin and xout in the x-direction where the momentum px = 0. The Weyl fermions confined inside the p–n–p junction make back and forth movement between xin and xout, and form a closed loop C in the classical phase space. Here, the specific form of potential well U(x) should not influence the main results of this paper (see the Supplementary Note 1), as long as the potential varies slowly spatially so that the inter-node scattering can be ignored if the separation of the Weyl nodes is not too close with each other38,39,40. For concreteness we set U(x) = κx2Θ(L − |x|) + U0Θ(|x| − L) in the following calculations, where Θ(x) is the Heaviside function and U0 = κL2.
Due to the closure of the loop C, the kinetic momentum Π = (Πx, Πy, Πz) with Πi = p_i+ eAi, i = x, y, z also exhibits an enclosed trajectory CΠ in the momentum space [see the closed curves in Fig. 2a]. Note that unlike the canonical momentum py, the kinetic momentum Πy = py + eBx is x dependent and not conserved along the CΠ. The Berry phase Γ accumulated along the trajectory for Weyl fermions with positive chirality can be determined by the Π-dependent Hamiltonian H(Π) = vσ · Π and is calculated from the following integral along CΠ41:
with |Π〉 the eigen-vector of H(Π).
Figure 2a gives the distribution of the Berry curvature BΠ (BΠ = i∇ × 〈Π|∂Π|Π〉) for the conduction band of H(Π) and shows the momentum trajectories of Weyl fermions under different magnetic fields. Here, the pz component is set to be 0.5p* and for simplicity we define the new units with E* = (κv2ħ2)1/3, x* = ħv/E*, \(B_ \ast = \hbar /ex_ \ast ^2\), and p* = E*/v. From Eq. (6) we know that the Berry curvature flux through the closed trajectory CΠ is the Berry phase acquired for the Weyl fermions. Increasing the magnetic field, the trajectory becomes enlarged, as if the magnetic field provides a momentum Lorentz force pointing outside the trajectory and pulls the closed trajectory outward. As a result, the momentum trajectory CΠ encloses more Berry curvature flux and accumulates a larger Berry phase.
After obtaining the Berry phase, we use the following EBK equation:
to calculate the chiral bound levels inside the p–n–p junction. Here, n is an integer number and γ = 0.75 is the Maslov index. As the spin direction is parallel (anti-parallel) to the momentum for Weyl fermions with positive (negative) chirality, the Berry phase or the spin procession angle accumulated for different chirality is opposite over the same real-space orbit [see Fig. 1b]. This sign difference is reflected by τ in Eq. (7). Solving the semiclassical EBK equation, we get the two chiral energy levels as functions of the magnetic field B, which are shown in Fig. 2b. For zero magnetic field, the Berry phase of both chiral Weyl fermions is zero, resulting in the degenerate chiral levels. Increasing the magnetic field, the Berry phase increases and the two chiral levels split with each other. Note that this level splitting can be large and approaches the level spacing of the quantized levels when B = B*. Here we mainly discuss the type-I WSM with no band tilting. For the type-II WSM, the chiral level splitting would exhibit strong anisotropy with respect to the band tilting direction (see Supplementary Note 2).
Quantum mechanical results
In this part, we solve the Weyl equation \(\hat H_\tau {\mathrm{\Psi }}_\tau ({\boldsymbol{r}}) = E{\mathrm{\Psi }}_\tau ({\boldsymbol{r}})\) (τ = ±1) microscopically and calculate the quantum transmission coefficient through the WSM p–n–p junction. Considering a plane wave with momentum py and pz incident from the left p region (x < − L), its wave function can be written as \(\Psi _\tau ^{{\mathrm{in}}}({\boldsymbol{r}}) = {\mathrm{e}}^{ip_yy/\hbar }{\mathrm{e}}^{ip_zz/\hbar }\varphi _\tau ^{{\mathrm{in}}}(x)\). The outgoing wave function in the right p region (x > L) can be written as \(\Psi _\tau ^{{\mathrm{out}}}({\boldsymbol{r}}) = {\mathrm{e}}^{ip_yy/\hbar }{\mathrm{e}}^{ip_zz/\hbar }t_\tau (E,p_y,p_z)\varphi _\tau ^{{\mathrm{out}}}(x)\) with tτ(E, py, pz) the transmission amplitude. Here we assume that the electrostatic potential in the p regions is very large, whereas the magnetic field is relatively small in the whole system. Then the momentum q = (U0 − E)/v in the p regions changes little by the magnetic field. For this reason, we only consider the magnetic field existing in the central n region and make the zero-magnetic field approximation in p regions. In fact, the results can well remain the same even if the magnetic field exists in p regions (see Supplementary Note 3). Then \(\varphi _\tau ^{{\mathrm{in}}}(x)\) can be written as:
where px satisfies \(\sqrt {p_x^2 + (p_y - eBL)^2 + p_z^2} = q\). The outgoing wave function is
with \(p_x^\prime\) satisfying \(p_x^{\prime 2} = q^2 - (p_y + eBL)^2 - p_z^2\). Then the transmission coefficient through the p–n–p junction for the chirality τ is Tτ(E, py, pz) = |tτ(E, py, pz)|2 and we define the total transmission coefficient as T = (T+ + T−)/2.
The transmission coefficient T is solved using the transfer matrix method. Figure 3 shows T as a function of the energy E and the momentum py. The peak position shows the bound energy levels inside the p–n–p junction. Here the magnetic field is set to B/B* = 0.2 and the momentum pz/p* = 0.3. As expected from the semiclassical analysis, the chiral or valley levels show explicit splitting behaviors. For a large momentum py (e.g., py/p* = 1.5), the two chiral levels almost degenerate and the Berry phases for different chiral Weyl fermions are very small. Decreasing the py component, the level splitting becomes larger because of the increase of the Berry phase. Here the chiral levels obtained from the EBK quantization rule are also plotted with solid (dashed) lines for the positive (negative) chirality as a comparison. One can see that the peak positions of the transmission map fit the semiclassical results quite well, which verifies the Berry phase’s role on inducing the chiral level splitting.
Experimental observable
To observe the above-mentioned unusual chiral level splitting, we design an experimental p–n–p junction device as shown in Fig. 4a. A scanning tunneling microscope (STM) or transmission electron microscope tip on top of the WSM can inject a beam of well-collimated Weyl fermions into the junction with a definite direction42. The electron beam can be described by a Gaussian wavepacket that takes the form
Here, A denotes the amplitude of the wavepacket, \({\mathrm{\Delta }}_{p_{y(z)}}\) is the momentum broadening, and py(z)0 is the average momentum. The outgoing electron beam in the bottom p region can be described by
The currents following into and out from the WSM are calculated as \(I^{{\mathrm{in}}} = \mathop {\sum}\limits_\tau {\langle \psi _{g\tau }^{{\mathrm{in}}}({\mathbf{r}})|\hat j_x|\psi _{g\tau }^{{\mathrm{in}}}({\mathbf{r}})\rangle }\) and \(I^{{\mathrm{out}}} = \mathop {\sum}\limits_\tau {\langle \psi _{g\tau }^{{\mathrm{out}}}({\mathbf{r}})|\hat j_x|\psi _{g\tau }^{{\mathrm{out}}}({\mathbf{r}})\rangle }\), with \(\hat j_x = - ev\sigma _x\) being the current operator.
We use the polar angle θ and the azimuthal angle φ in the sphere coordinate to describe the incident direction of the wave packet and they satisfy the following relations:
with \(p_{x0} = - \sqrt {q^2 - (p_{y0} - eBL)^2 - p_{z0}^2}\). Experimentally, one can fix the value of the incident current Iin and rotate the sample beneath the STM tip (or rotate the STM tip) with angle (θ, ϕ) to measure the outgoing current Iout. Figure 4b shows Iout as a function of the incident energy E and the azimuthal angle ϕ, where the polar angle θ is fixed to π/2, i.e., the incident electron beam is injected in the x–y plane. We see that in the presence of the magnetic field, the transmission map shows a fish-bone shape and remarkably the peak position of the transmission current has a sharp shift at a critical ϕ (see the white arrows). This phenomenon is similar to the graphene p–n–p junction case31 and arises from the π Berry phase jump of the Weyl fermion. Note that the two chiral bound levels degenerate and the current is chiral unpolarized in this case, because the Berry phase takes an integer multiple of π and its sign does not lead to any physical effect. Tilting the sample with a small angle by setting θ = π/2 + π/180, the chiral energy levels show obvious splitting for small ϕ as a result of the non-integer multiple π’s Berry phase [see Fig. 4c]. With a large angle ϕ, the chiral levels degenerate, indicating the vanishing Berry phase. Here we define the chirality polarization as \(P \equiv \frac{{I_ + - I_ - }}{{I_ + + I_ - }}\) with \(I_ \pm = \langle \psi _{g, \pm 1}^{{\mathrm{out}}}({\mathbf{r}})|\hat j_x|\psi _{g, \pm 1}^{{\mathrm{out}}}({\mathbf{r}})\rangle\) being the outgoing current for the positive/negative chirality. Figure 4d gives the chirality polarization calculated on the dashed line cut in Fig. 4c. We see that even in such a small tilting angle θ, the chirality polarization can be high. Figure 4c, d also show that a chiral or valley-polarized current can be generated in the present device by tuning the tip orientation or the magnetic field, which provides a platform for investigating the chirality or valley degree of freedom in WSMs.
Measuring the Berry phase
The semiclassical EBK quantization formula in Eq. (7) tells us that the Berry phase difference 2|Γ| between two chiral Weyl fermions would lead to a chiral level splitting. Next, we show that this chiral splitting can be used to measure the Berry phase by merely reading the resonant level positions from the transmission spectrum. We take Fig. 4c as an example. From the angle–momentum relations (Eq. (12)), one can transform the angle-dependent transmission map into the momentum-dependent one, as shown in Fig. 5a. Here, to enhance the discriminability of the peak position, we have shown the second derivative −∂2T/∂E2 of the the transmission coefficient. By making a line cut py0/p* = 0.2 in Fig. 5a, one can read out the n-th resonant levels \(\epsilon _{n \pm }\) for the positive (negative) chirality. Taking the average \(\epsilon _n = (\epsilon _{n + } + \epsilon _{n - })/2\), the opposite Berry phase cancels and one gets the quantized energy levels including no Berry phase. Here we define the level spacing as \({\mathrm{\Delta }}_n \equiv \epsilon _n - \epsilon _{n - 1}\), and from the EBK quantization rule in Eq. (7) we see that as the Berry phase Γ = ±π, the chiral level splitting equals to Δn. Whereas for the zero Berry phase, the different chiral levels degenerate and the level splitting becomes zero. For simplicity, we assume that the level splitting varies linearly with the Berry phase and then the Berry phase for the n-th level can be calculated from the following formula:
We first give the actual Berry phase of the resonant levels calculated with the semiclassical EBK method. The results are labeled by circular solid dots in Fig. 5b, c. The Berry phases obtained using Eq. (13) are also shown in Fig. 5c with diamond points for comparison. One can see that the two results fit well, which shows that our method is effective and accurate. Experimentally, the p–n–p junction can be constructed by the electrical or chemical doping43,44. By tuning the electrostatic potential offset between the p and n regions into 0.18 eV and setting the length of the central n region to 270 nm, an electrostatic potential profile that can be approximated with a parabolic function45 with the strength κ ≈ 10 eV μm−2 is obtained inside the p–n–p junction. If we take the Fermi velocity v = 3 × 105 ms−146, the splitting magnetic field 0.2B* is then estimated to be 0.18 T, which is far less than the filed strength to reach the quantum limit in the SdH oscillation. Besides, we also test our method for other kinds of potential profiles U(x) in Supplementary Note 1 and the results also show accuracy. Thus, the strategy proposed here could provide a convenient and practical way to measure the Berry phase in WSMs in real experiments.
Discussion
Before we only consider the inversion symmetric WSMs with two Weyl nodes in the Brillouin zone. For the time-reversal symmetrical one47,48, there exist at least two pairs of Weyl nodes with different chirality, which are related by the time-reversal symmetry. The connections between different Weyl nodes with opposite chirality would become complicated in this case, but the results should be the same since the Berry phase for Weyl fermions is only chirality dependent and we have ignored the inter-node scattering between different Weyl nodes (see Supplementary Note 4). Besides, the Dirac semimetals49,50 in which the Dirac nodes are composed of two decoupled chiral Weyl points should also manifest the similar property. Thus, our results obtained above can be extended to topological semimetal p–n–p junctions.
In conclusion, we investigate the transport property of a WSM p–n–p junction and find two unusual phenomena due to the Berry phase effect: when the Weyl fermions acquire an integer multiple π’s Berry phase, a sharp level shift can be observed in the transmission spectrum, whereas for non-integer ones of Berry phase, the chiral or valley levels show explicit splitting and a chirality (valley)-polarized current can be generated through the junction. We give a semiclassical analysis on these phenomena using the EBK quantization rule and propose a new method to measure the Berry phase in topological semimetals, which is accurate and can be applied in real experiments.
Methods
Calculating the Berry phase
To obtain the Berry phase, we discretize the momentum trajectory CΠ into N = 1000 sites and label them by Πj with j = 1, 2, …N. A periodic boundary condition Π1 = ΠN is required to ensure the closed feature of the orbit. Each site corresponds to one vector |Πj〉, which is the eigenstate of H(Πj) = vσ · Πj. Then the Berry phase can be calculated by51
Calculating the quantum transmission coefficient
In using the transfer matrix method, we divide the central region (−L < x < L) of the p–n–p junction into M intervals and in every interval approximate the electrostatic potential by a constant local value Un = U(xn) and set the vector potential An = (0, Bxn, 0), with xn = −L + nh and h = 2L/N. Then, in each interval xn−1 < x < xn, the one-dimensional Hamiltonian \(\hat H_{\tau ,x}\) in Eq. (3) can be written as: \(\hat H_{\tau ,n} = v[ - i\hbar \partial _x\sigma _x + (p_y + eBx_n)\sigma _y + \tau p_z\sigma _z] + U_n\). The solutions of \(\hat H_n\) (for simplicity, we have omitted the τ index) have a right-propagating mode denoted by φn→(x) and a left-propagating one denoted by φn←(x). The wavefunction fn(x) in the interval n can be written as a composition of φn→ and φn←: fn(x) = Anφn→ + Bnφn← = Sn(x)[An, Bn]T, where Sn = (φn→, φn←) is a 2 × 2 matrix.
At the interface x = xn, we have the following matching condition:
The iteration relation for [An, Bn]T is:
Finally, the relation between the outgoing mode and the incoming mode is obtained as \([A_{M + 1},B_{M + 1}]^T = \mathop {\prod}\limits_{i = 0}^M {S_{M + 1 - i}^{ - 1}} (x_{M - i})\cdot S_{M - i}(x_{M - i})[A_0,B_0]^T\). By setting [A0, B0]T = [1, 0]T, the transmission coefficient through the p–n–p junction is T = |AM+1|2.
Data availability
The data generated or analyzed in this work are included in this published article (and its Supplementary Material).
Code availability
The code that support the findings of this study has been deposited in figshare with the identifier: https://doi.org/10.6084/m9.figshare.8305997.
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Acknowledgements
This work was financially supported by National Key R and D Program of China (Grant No. 2017YFA0303301), NBRP of China (Grant No. 2015CB921102), NSF-China (Grant No. 11574007), the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB28000000), and Beijing Municipal Science & Technology Commission No. Z181100004218001.
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Z.H., Y.-F.Z. and N.-X.Y. wrote this paper together. Q.-F.S. initiated and supervised the project.
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Hou, Z., Zhou, YF., Yang, NX. et al. Chirality-dependent electron transport in Weyl semimetal p–n–p junctions. Commun Phys 2, 86 (2019). https://doi.org/10.1038/s42005-019-0186-9
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DOI: https://doi.org/10.1038/s42005-019-0186-9
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